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Physical review. B, Condensed matter

Quantum tunneling with dissipation: Possible enhancement by dissipative interactions

Kazuo Fujikawa, Satoshi Iso, Misao Sasaki, Hiroshi Suzuki

Published Oct 15, 1992• 24 citations
Publisher

Abstract

The macroscopic quantum tunneling in a double-well potential with dissipation is formulated without referring to instantons. This formulation, in the domain of small dissipation, goes beyond the instanton approximation which corresponds to the two-state truncated system (or, the so-called spin-boson Hamiltonian). It is first confirmed that our formulation, when applied to the two-state truncated system, reproduces all the known results of the instanton approximation. It is then shown that the ground state is mixed with excited states by dissipative interactions and this effect tends to enhance the ground-state quantum tunneling. In the Ohmic dissipation case this enhancement factor, even for a shallow double-well potential, can be at most comparable to the suppression factor which has been known from the work by Caldeira and Leggett. In the super-Ohmic case, however, the enhancement factor generally exceeds the suppression factor and the two-state approximation fails. A salient feature in the choice of counter terms in macroscopic quantum tunneling, which is essential to the above conclusion, is emphasized.

DOI
10.1103/physrevb.46.10295

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The macroscopic quantum tunneling in a double-well potential with dissipation is formulated without referring to instantons. This formulation, in the domain of small dissipation, goes beyond the instanton approximation which corresponds to the two-state truncated system (or, the so-called spin-boson Hamiltonian). It is first confirmed that our formulation, when applied to the two-state truncated system, reproduces all the known results of the instanton approximation. It is then shown that the ground state is mixed with excited states by dissipative interactions and this effect tends to enhance the ground-state quantum tunneling. In the Ohmic dissipation case this enhancement factor, even for a shallow double-well potential, can be at most comparable to the suppression factor which has been known from the work by Caldeira and Leggett. In the super-Ohmic case, however, the enhancement factor generally exceeds the suppression factor and the two-state approximation fails. A salient feature in the choice of counter terms in macroscopic quantum tunneling, which is essential to the above conclusion, is emphasized.
We suggest taking the fluctuation-dissipation theorem of Callen and Welton [Phys. Rev. 83, 34 (1951)] as a basis to study quantum dissipative phenomena (such as macroscopic quantum tunneling) in a manner analogous to the Nambu-Goldstone theorem for spontaneous symmetry breakdown [Phys. Rev. 122, 345 (1961); Nuovo Cimento 19, 154 (1961)]. It is shown that the essential physical contents of the Caldeira-Leggett model [Phys. Rev. Lett. 46, 211 (1981); Ann. Phys. (N.Y.) 149, 374 (1983)] such as the suppression of quantum coherence by Ohmic dissipation are derived from general principles only, namely, the fluctuation-dissipation theorem and unitarity and causality (i.e., dispersion relations), without referring to an explicit form of the Lagrangian. An interesting connection between quantum tunneling with Ohmic dissipation and Anderson's orthogonality theorem is also noted.
For the realistic theoretical descriptions of quantum devices, we have to take the unavoidable coupling to their surrounding environment into account. A lot of effort in theoretical physics has been made to describe decoherence effects and the corresponding quantum to classical transition in the past. In these studies, baths are coupled to certain observables making their behavior more classical. In the most general case, a quantum device is affected by environments coupled to different observables. In this thesis, we study the differences emerging from coupling the bath to different observables. In particular, we investigate the situation, where two baths are coupled simultaneously to two conjugate variables (e.g. xˆ and pˆ, denoted dissipative frustration). We study how the interplay of these two baths can lead to interesting effects. After an introduction of the topic, we discuss the results of this thesis in Part II and Part III. In Part II, we study the effect of quantum tunneling in presence of a dissipative interaction with two Ohmic environments to the position xˆ and/or to the momentum pˆ of a particle. In chapter 2, we consider a symmetric double well potential which is important in the context of coherent state preparation, as its ground state is a superposition of being in the left and in the right well. Using the semiclassical approximation to calculate instanton paths within the path integral method, we find that momentum dissipation enhances the coherent tunnel splitting. In presence of dissipative couplings to xˆ and pˆ, the momentum dissipation acts in favor of the delocalization of the particle shifting the critical coupling strength of the dissipative phase transition induced by the position dissipation. Chapter 3 contains a study of the escape rate out of a metastable well in presence of dissipation. Here we find that the incoherent tunneling rate is exponentially enhanced in presence of momentum dissipation. We further show that the influence of momentum dissipation depends on the slope of the part of barrier the particle escaping through. In presence of both dissipative couplings, we find a non-monotonic behavior of the escape rate as a function of the dissipative couplings strengths. In Part III, we show that it is possible to realize the situation of "dissipative frustration" in Josephson junction chains. In particular, we introduce charge dissipation as a physical realization of the afore introduced momentum coupling. After presenting the circuit elements needed for charge dissipation, we study a chain of Josephson junctions affected by Ohmic baths coupled to the charge and/or the phase. Using a self-consistent harmonic approximation, we determine the phase diagram at zero temperature which exhibits a quantum phase transition between an ordered phase, corresponding to the superconducting state, and a disordered phase, corresponding to the insulating state with localized superconducting charge. Interestingly, we find that the critical line separating the two phases has a non-monotonic behavior as a function of the dissipative coupling strength. Moreover, within the self-consistent harmonic approximation, we analyze the dissipation induced crossover between a first and second order phase transition, showing that dissipative frustration increases the range in which the phase transition is second order. The non-monotonic behavior is also reflected in the purity of the system that quantifies the degree of correlation between the system and the environment, and in the logarithmic negativity as an entanglement measure that encodes the internal quantum correlations in the chain.
The real-time dynamics of a quantum-mechanical particle in a dissipative double-well potential at finite temperatures is solved ab initio by means of a multisite spin-hopping analysis. Both the macroscopic-quantum-coherence and macroscopic-quantum-tunneling regimes are covered. The theory gives a unified picture of tunneling transport and vibrational relaxation. The analysis is based on the Ohmic-model Hamiltonian [A. O. Caldeira and A. J. Leggett, Ann. Phys. (N.Y.) 149, 374 (1983); R. Zwanzig, J. Stat. Phys. 9, 215 (1973)] or the equivalent ``particle-on-a-string'' model [H. Dekker, Phys. Rev. A 31, 1067 (1985)]. The reduced quantum Liouville equation for the particle is derived and written in the energy representation. The usual truncation to the ground-state doublet of the vibrational ladder is not made. The interdoublet vibrational dynamics considerably simplifies upon coarse-graining and in the harmonic-well approximation. The intradoublet pseudospin dynamics is treated in the ``noninteracting-blip approximation'' [A. J. Leggett et al., Rev. Mod. Phys. 59, 1 (1987)]. The coarse-grained vibrational processes give rise to a Markovian one-step spin hopping between adjacent doublets (or sites). Inter alia ``inhomogeneous broadening'' and ``motional narrowing'' [P. E. Parris and R. Silbey, J. Chem. Phys. 83, 5619 (1985)] are discussed as special cases.
By using a variation method we study the ground state of a tunneling particle coupled to many bosons in a double-well potential. The boson system is assumed to have dense low-energy excitations, just as taken by Chakravarty and Leggett to discuss the dissipative effect in macroscopic quantum phenomena. We examine reduction of the tunneling matrix and eventual localization of the particle due to boson excitations for arbitrary strengths of tunneling and coupling parameters. Ground state energy is evaluatied. Continuous as well as discontinuous changes from tunneling to localized states are found when the coupling parameter increases. The results are related to the orthogonality of many-particle ground states, as known for many-electron system as Anderson's theorem.
We present a comprehensive study of the effect of a transverse magnetic field on the macroscopic quantum tunneling of two identical coupled particles with dissipation. Two coupled particles of identical masses but opposite charges in the plane, in the presence of a constant transverse external magnetic field and an external potential interacting with a bath of harmonic oscillators are studied. In this case, the problem cannot be mapped to a one-dimensional problem, it strictly remains two-dimensional. We calculate the exact effective action both for the case of linear coupling to the bath and without a linear coupling to the bath using imaginary time path integral and Leggett's prescription at T=0. In the limit of zero magnetic field we recover a two dimensional version of the result found in \cite{em1} for the case of two identical particles. We find that in the limit of weak and strong dissipation, the effective action reduces to a two dimensional version of the Caldeira-Leggett form in terms of the reduced mass and magnetic field. The case of Ohmic dissipation with the motion of the two particles damped by the Ohmic frictional constant η\etaη is studied in detail.