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Physica A Statistical Mechanics and its Applications

Influence of the counter-rotating terms on the spontaneous emission from a two-level hydrogenic atom: non-Markovian solution for atomic population-inversion expectation value and the radiative line shape

JOSIP SEKE, Wolfgang N. Herfort

Published Nov 1, 1991• 11 citations
Publisher
DOI
10.1016/0378-4371(91)90038-e

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For the first time to the authors' knowledge a mathematically rigorous method is used for treating finite-time deviations from the exponential decay in the case of spontaneous Lyman-\ensuremath{\alpha} transitions in a two-level hydrogenic atom. First, in the so-called Weisskopf-Wigner model (where the rotating-wave approximation is implied) finite-time deviations with a rigorous validity range, based on accurate error estimations, are derived. Second, in order to obtain the frequency shift (Lamb shift), counter-rotating terms are taken into account by using a projection-operator method developed a decade ago by one of the present authors [J. Seke, Phys. Rev. A 21, 2156 (1980)]. By means of this method, equations of motion for dipole-moment expectation values are derived without employing the usual Born approximation. These equations are solved by using the method of the Laplace transform and its inverse. Again finite-time deviations from the exponential decay of the dipole-moment expectation values with a definite validity range are obtained. Finally, it should be emphasized that all the results presented in this paper contain accurate error estimates which are absolutely necessary in a rigorous mathematical method.

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Virtual Photons, Causality and Atomic Dynamics in Spontaneous Emission

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The time-dependent electric energy density surrounding a two-level atom fixed at r = 0 is studied, the atom being taken in its excited state at t = 0 and the field being initially in the vacuum state. The atom-field coupling includes both rotating and counter-rotating terms. The energy density of the spontaneously emitted field in the rotating wave approximation is shown to behave non-causally, while in the presence of the complete coupling it is shown to vanish outside a sphere of radius r = ct centred on the atom. The deviations of atomic dynamics from the exponential Wigner-Weisskopf behaviour during spontaneous decay are shown to be deeply influenced by the counter-rotating terms. It is concluded that the virtual photons induced by the counter-rotating terms in the atom-field coupling are essential in order to ensure causality and cannot be neglected in any accurate treatment of spontaneous emission.

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It is pointed out that the usual Heisenberg equations-of-motion or Liouvillian superoperator perturbation-theory approaches to systems with arbitrary statistical ensembles can give spurious, nonconvergent results when attempts are made to calculate the expectation value for certain operators which commute with the zeroth-order Hamiltonian. The non-Markovian, long-time tail of the Weisskopf-Wigner spontaneous-emission decay of a two-level atom is presented as an example of this failure. The general reason for such failures is elucidated and a new method applicable to arbitrary equilibrium or nonequilibrium statistical ensembles is formulated. The new method is applied to the same example of spontaneous emission to derive the correct short- and long-time behavior. The physical model of a two-level atom is discussed and some mathematical techniques of general usefulness are presented. The present results are also briefly discussed in the context of previous work on nonexponential decay. A fully quantum-mechanical definition of time-dependent spectral line shape is given in terms of the response of a two-level---atom detector with variable frequency interacting with electromagnetic radiation. The non-Lorentzian line shape recorded by such a detector for the spontaneous emission of a source two-level atom is calculated as another example of a problem for which the usual methods give incorrect results. The extension of the present method to Liouvillian or master-equation approaches is discussed.
For the first time to the authors' knowledge a mathematically rigorous method is used for treating finite-time deviations from the exponential decay in the case of spontaneous Lyman-\ensuremath{\alpha} transitions in a two-level hydrogenic atom. First, in the so-called Weisskopf-Wigner model (where the rotating-wave approximation is implied) finite-time deviations with a rigorous validity range, based on accurate error estimations, are derived. Second, in order to obtain the frequency shift (Lamb shift), counter-rotating terms are taken into account by using a projection-operator method developed a decade ago by one of the present authors [J. Seke, Phys. Rev. A 21, 2156 (1980)]. By means of this method, equations of motion for dipole-moment expectation values are derived without employing the usual Born approximation. These equations are solved by using the method of the Laplace transform and its inverse. Again finite-time deviations from the exponential decay of the dipole-moment expectation values with a definite validity range are obtained. Finally, it should be emphasized that all the results presented in this paper contain accurate error estimates which are absolutely necessary in a rigorous mathematical method.
The time-dependent electric energy density surrounding a two-level atom fixed at r = 0 is studied, the atom being taken in its excited state at t = 0 and the field being initially in the vacuum state. The atom-field coupling includes both rotating and counter-rotating terms. The energy density of the spontaneously emitted field in the rotating wave approximation is shown to behave non-causally, while in the presence of the complete coupling it is shown to vanish outside a sphere of radius r = ct centred on the atom. The deviations of atomic dynamics from the exponential Wigner-Weisskopf behaviour during spontaneous decay are shown to be deeply influenced by the counter-rotating terms. It is concluded that the virtual photons induced by the counter-rotating terms in the atom-field coupling are essential in order to ensure causality and cannot be neglected in any accurate treatment of spontaneous emission.