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Physical Review A

Adiabatic and nonadiabatic Berry phases for two-level atoms

D J Moore, G E Stedman

Published Jan 1, 1992• 16 citations
Publisher

Abstract

A formalism for calculating Berry phases for nonadiabatic systems containing an additional adiabatic time dependence is developed. This is then applied to a two-level atom in a strong resonant polarized laser, where the laser polarization provides the adiabatic parameter. It is found that, when the laser polarization is kept constant, judicious polarization choices allow one to eliminate either the rotating-wave or non-rotating-wave part of the interaction. Furthermore, the adiabatic Berry phasor obtained when the laser polarization is varied is found to be complex. This can be compared to the case of purely adiabatic time-reversal even systems, which can only have real Berry phasors.

DOI
10.1103/physreva.45.513

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A formalism for calculating Berry phases for nonadiabatic systems containing an additional adiabatic time dependence is developed. This is then applied to a two-level atom in a strong resonant polarized laser, where the laser polarization provides the adiabatic parameter. It is found that, when the laser polarization is kept constant, judicious polarization choices allow one to eliminate either the rotating-wave or non-rotating-wave part of the interaction. Furthermore, the adiabatic Berry phasor obtained when the laser polarization is varied is found to be complex. This can be compared to the case of purely adiabatic time-reversal even systems, which can only have real Berry phasors.
The exact adiabatic representation scheme of Nguyen-Dang [J. Chem. Phys. 90, 2657 (1989)] is applied to time evolution of the general laser-driven two- and three-level systems. It leads to exact formal results that do not assume a specific shape of the pulse and do not invoke the rotating-wave approximation (RWA). These results are a generalization of the corresponding RWA results because the former depend on an effective pulse area that varies with the detuning and involves a Rabi frequency modulated by a phase cphi(t). In addition, the exact adiabatic representation scheme is applied to N-level systems exhibiting various dynamic symmetries and, as in the previous cases, leads to results that do not invoke the RWA and depend on an effective pulse area. Time-reversal analysis on two- and three-level systems leads to quantization of the effective pulse area for time-symmetric pulses. This quantization leads to localized asymptotic population distributions.
The adiabatic variation of a Hamiltonian can cause the wavefunction, governed by the Hamiltonian, to acquire an unexpected phase. The existence of this phase (Berry's phase) is an additional element in the well-known quantum adiabatic theorem. Berry's phase is observable in the interference between two identically prepared systems only one of which is adiabatically varied. We show that a single quantum system prepared in a superposition of the eigenstates of its Hamiltonian leads to observable Berry phase effects at all times. We examine this principle within the context of two-level optical resonance.
A formalism is developed for calculating Berry phases for nonadiabatic time-periodic quantum systems when a dynamical invariant is known. It is found that, when the invariant is periodic and has a nondegenerate spectrum, this method allows a convenient way to obtain generalized Berry phases and the proper cyclic initial states. The method is applied to the generalized harmonic oscillator and the two-level system, where the invariant operators are explicitly constructed. Formulae for the conventional Berry's phases are readily obtained by taking the adiabatic limit of the exact results.
Quantum mechanical phases arising from a periodically varying Hamiltonian are considered. These phases are derived from the eigenvalues of a stationary, ``dressed'' Hamiltonian that is able to treat internal atomic or molecular structure in addition to the time variation. In the limit of an adiabatic time variation, the usual Berry phase is recovered. For more rapid variation, nonadiabatic corrections to the Berry phase are recovered in perturbation theory, and their explicit dependence on internal structure emerges. Simple demonstrations of this formalism are given, to particles containing interacting spins, and to molecules in electric fields.
A theoretical analysis of Berry's phases, which is based on the Cartan subalgebra, is given for three-level atomic systems. The analysis is developed under the adiabatic approximation and is related to topological fibre bundle theories. The topological Berry's phases derived in the present study, are related to phase shifts and can be applied, also, for partial cycles. Some possible applications of the present theory are discussed, for three-level and two-level atomic systems, interacting with nearly resonant monochromatic fields, under the semiclassical and rotating-wave approximations.