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The Journal of Chemical Physics

Time evolution of a single spin inhomogeneously coupled to an interacting spin environment

Zhen Huang, Gehad Sadiek, Sabre Kais

Published Apr 12, 2006• 17 citations
Publisher

Abstract

We study the time evolution of a single spin coupled by exchange interaction to an environment of interacting spin bath modeled by the XY Hamiltonian. By evaluating the spin correlator of the single spin, we observed that the decay rate of the spin oscillations strongly depends on the relative magnitude of the exchange coupling between the single spin and its nearest neighbor J(') and coupling among the spins in the environment J. The decoherence time varies significantly based on the relative coupling magnitudes of J and J('). The decay rate law has a Gaussian profile when the two exchange couplings are of the same order J(') approximately J but converts to exponential and then a power law as we move to the regimes of J(')>J and J(')<J. We also show that the spin oscillations propagate from the single spin to the environmental spins with a certain speed. The effect of varying the anisotropic parameter, external magnetic field, and temperature on the decaying rate of the spin state is also discussed.

DOI
10.1063/1.2192778

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We study the time evolution of a single spin coupled by exchange interaction to an environment of interacting spin bath modeled by the XY Hamiltonian. By evaluating the spin correlator of the single spin, we observed that the decay rate of the spin oscillations strongly depends on the relative magnitude of the exchange coupling between the single spin and its nearest neighbor J(') and coupling among the spins in the environment J. The decoherence time varies significantly based on the relative coupling magnitudes of J and J('). The decay rate law has a Gaussian profile when the two exchange couplings are of the same order J(') approximately J but converts to exponential and then a power law as we move to the regimes of J(')>J and J(')<J. We also show that the spin oscillations propagate from the single spin to the environmental spins with a certain speed. The effect of varying the anisotropic parameter, external magnetic field, and temperature on the decaying rate of the spin state is also discussed.
The time evolution of a spin-12\frac{1}{2}21​ particle under the influence of a locally applied external magnetic field, and interacting with anisotropic spin environment in thermal equilibrium at temperature TTT is studied. The exact analytical form of the reduced density matrix of the central spin is calculated explicitly for a finite number of bath spins. The case of an infinite number of environmental spins is investigated using the convergence of the rescaled bath operators to normal Gaussian random variables. In this limit, we derive the analytical form of the components of the Bloch vector for antiferromagnetic interactions within the bath, and we investigate the short-time and long-time behavior of reduced dynamics. The effect of the external magnetic field, the anisotropy, and the temperature of the bath on the decoherence of the central spin are discussed.
We study the dynamics of entanglement for the XY-model, one-dimensional spin systems coupled through the nearest neighbor exchange interaction and subject to an external time-dependent magnetic field. Using the two-site density matrix, we calculate the time-dependent entanglement of formation between nearest neighbor qubits. We investigate the effect of varying the temperature, the anisotropy parameter and the external time-dependent magnetic field on the entanglement. We have found that the entanglement can be localized between nearest neighbor qubits for certain values of the external time-dependent magnetic field. Moreover, as known for the magnetization of this model, the entanglement shows nonergodic behavior, it does not approach its equilibrium value at the infinite time limit.
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We study the decoherence of two coupled spins that interact with a spin-bath environment. It is shown that the connectivity and the coupling strength between the spins in the environment are of crucial importance for the decoherence of the central system. For the anisotropic spin bath, changing the connectivity or coupling strength changes the decoherence of the central system from Gaussian to exponential decay law. The initial state of the environment is shown to affect the decoherence process in a qualitatively significant manner.
Decoherence of a central spin coupled to an interacting spin bath via inhomogeneous Heisenberg coupling is studied by two different approaches, namely an exact equations of motion (EOMs) method and a Chebyshev expansion technique (CET). By assuming a wheel topology of the bath spins with uniform nearest-neighbor XXXXXX-type intrabath coupling, we examine the central spin dynamics with the bath prepared in two different types of bath initial conditions. For fully polarized baths in strong magnetic fields, the polarization dynamics of the central spin exhibits a collapse-revival behavior in the intermediate-time regime. Under an antiferromagnetic bath initial condition, the two methods give excellently consistent central spin decoherence dynamics for finite-size baths of $N\ensuremath{\le}14$ bath spins. The decoherence factor is found to drop off abruptly on a short time scale and approach a finite plateau value which depends on the intrabath coupling strength nonmonotonically. In the ultrastrong intrabath coupling regime, the plateau values show an oscillatory behavior depending on whether N/2N/2N/2 is even or odd. The observed results are interpreted qualitatively within the framework of the EOM and perturbation analysis. The effects of anisotropic spin-bath coupling and inhomogeneous intrabath bath couplings are briefly discussed. Possible experimental realization of the model in a modified quantum corral setup is suggested.
We study the time dynamics of a single boson coupled to a bath of two-level systems (spins 1/2) with different excitation energies, described by an inhomogeneous Dicke model. Analyzing the time-dependent Schr\"odinger equation exactly, we find that at resonance the boson decays in time to an oscillatory state with a finite amplitude characterized by a single Rabi frequency if the inhomogeneity is below a certain threshold. In the limit of small inhomogeneity, the decay is suppressed and exhibits a complex (mainly Gaussian-like) behavior, whereas the decay is complete and of exponential form in the opposite limit. For intermediate inhomogeneity, the boson decay is partial and governed by a combination of exponential and power laws.