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Soviet Physics Uspekhi

Nonlinear Narrow Molecular Resonances Induced by Laser Radiation, and Their Application in Spectroscopy and Quantum Electronics

Vladilen S Letokhov

Published May 31, 1973• 1 citation
Publisher
DOI
10.1070/pu1973v015n05abeh005045

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Нелинейные узкие молекулярые резонансы, индуцируемые лазерным излучением, и их применение в спектроскопии и квантовой электронике, Летохов В.С.
This paper investigates nonlinear processes in transitions to the continuum, and their manifestations in the photoabsorption, polarization, and angular distribution of the electrons, as well as in the nonlinear susceptibility in the case of frequency gases. Change of photoabsorption line shape by strong laser radiation upon transition to the continuum is examined. Conditions for the appearance of an induced autoionizing-like resonance in absorption are described, and allowance for the energy dependence of the matrix elements of the transitions to the continuum are examined. A discussion of narrow nonlinear resonances in ionization and recombination is presented. Induction of nonlinear resonances in a continuum when strong/radiation interacts with several close-lying discrete states is described. A presentation is given on the use of laser to induce nonlinear autoionizinglike resonances in a continuum to generate coherent radiation on the basis of frequency mixing in gases. Doppler broadening of nonlinear resonance is discussed. Phase modulation, frequency modulation and amplitude-phase modulation are outlined.
The forces acting on a resonance particle in the fields of laser radiation sources can be large. Acceleration, heating, and cooling of atoms by using these forces are discussed. Since the forces are of a resonance type, one can employ them to separate isotopes and excited atoms from unexcited atoms. Light pressure can play an important role in the spectroscopy of narrow atomic and molecular resonances. The quantum features of the motion of particles in a standing light wave are manifested in a fine structure of the absorption coefficient. This review is concerned with analyzing the resonance light-pressure forces and discussing the application of them in optics and quantum electronics.