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Russian Microelectronics

Quantum memory based on ensemble states of NV centers in diamond

Alexander V. Tsukanov

Published May 1, 2013• 13 citations
Publisher

Abstract

In this study, the main results of experimental and theoretical investigations that substantiate the possibility of the development of quantum computational systems with a separate structure are considered and analyzed. These systems involve the operational part and the memory, as well as the communication quantum network, which performs the data exchange between them. We are starting to get knowledge about such hybrid quantum devices from studying the solid-state systems, in which the macroscopic number (ensemble) of NV centers in diamond is used as the memory element, while superconducting mesoscopic structures play the role of the operational element and quantum network.

DOI
10.1134/s1063739713030086

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•Jan 1, 2017•1 citation
In this study, the main results of experimental and theoretical investigations that substantiate the possibility of the development of quantum computational systems with a separate structure are considered and analyzed. These systems involve the operational part and the memory, as well as the communication quantum network, which performs the data exchange between them. We are starting to get knowledge about such hybrid quantum devices from studying the solid-state systems, in which the macroscopic number (ensemble) of NV centers in diamond is used as the memory element, while superconducting mesoscopic structures play the role of the operational element and quantum network.
Hybrid quantum systems, which combines the advantages of different quantum systems, play an essential role in the realisation of quantum computation, especially as quantum memory. This thesis discusses the very promising hybrid quantum system based on the ensemble of negatively charged nitrogen-vacancy centers (NV-centers) in diamond and superconducting microwave cavities. The decoherence of this system, due to the inhomogeneous spin broadening, seems to be the major obstacle of utilising the NV-centers as a quantum information storage. This works focuses on the study of the dynamics of our NV-center spin ensemble strongly coupled to a superconducting resonator driven by pulse sequences with a carrier frequency equaling the cavity frequency. A precise knowledge of the spin broadening, which has a non-Lorentzian distribution, led to the observation of the so called 'cavity protection effect'. Furthermore this work demonstrates the enhancement of the damped Rabi oscillations between the spin ensemble and the cavity mode through appropriate chosing of the microwave pulses, which could change in the order of two magnitudes. Last we also confirmed the theoretical analysis of the crossover from markovian to non-markovian dynamics for our system, which is achieved for increasing coupling strength.
Quantum entanglement is a kernel of quantum computation and quantum communication. We introduce a theoretical scheme to achieve the entanglement between two separated quantum nodes in a hybrid system. The proposed hybrid system based on diamond nitrogen-vacancy (NV) center spin ensemble is coherently coupled to a superconducting quantum circuit consisting of two quantum nodes and a quantum channel. Each node in our setup is composed of an NV center spin ensemble magnetically coupled to a superconducting coplanar resonator. The NV center spin ensemble composed of N identical and non-interacting NV spins, is placed in the magnetic field antinode of the superconducting coplanar resonator where the coupling is maximized. An array of superconducting quantum interference devices (SQUIDs) is inserted in the central conductor of resonator to make its frequency tunable with the magnetic flux threading through the SQUID loops. This flux is generated by passing current through an on-chip wire, so that the resonator can be brought in resonance with the NV center spins without changing their Zeeman splitting. Quantum qubits encoded into two separate nodes are connected by a vacuum superconducting coplanar resonator that is used as a quantum channel. This setup can potentially take the best elements of each individual system:NV center spin ensemble with longer coherence time capable of preparing, storing and releasing photonic quantum information, and the superconducting quantum circuits are easy to manipulate externally and can perform quantum logic gates to control quantum information rapidly. In order to realize the entanglement between two separated quantum nodes, firstly, we make a canonical transformation and obtain the Hamiltonian of the system that is reduced to two NV center spin ensembles resonantly coupled to a single mode of the superconducting coplanar resonator. Then we put forward the hybrid NV center spin-photon qubit encoding. In this hybrid encoding, the NV center spin and photon degrees of freedom enter on an equal footing into the definition of the qubit, in which case, quantum channel will switch on when three superconducting coplanar resonators are in resonance with each other, and all the manipulations can perform simply by tuning the frequencies of the superconducting coplanar resonators. Under the precise control of the evolution time, high fidelity entanglement between two separated quantum nodes is achieved. We show that this proposal can provide high fidelity quantum entanglement under realistic conditions, both in the resonant and the dispersive interaction cases. This hybrid quantum system will exhibit long coherence time and possess features like easy fabrication, integratability, and potential scalability. Furthermore, the quantum node composed of an NV center spin ensemble magnetically coupled to a superconducting coplanar resonator can be respectively integrated, which has practical applications in the realization of quantum information transmission and quantum entanglement among multiple quantum nodes.
In recent years, NV centers in diamond has attracted significant attention as a candidate for quantum information devices. The negatively charged NV center, in particular, has been intensely investigated [1-3]. NV- centers host both an electron spin qubit and a nitrogen nuclear spin, in our case a nuclear spin-1/2 of 15N is imbedded. The ground state of the electron spin qubit has a long coherence time and an optical transition at 637nm. The nuclear spins may be considered as a long-lived quantum memory, which has been experimentally demonstrated [2]. Because of these preferable quantum properties, NV centers have been considered as a good candidate for implementation of quantum information processing and there has been a number of theoretically propose designs for quantum information processing [3].
A fully functional quantum computer must contain at least two important components: a quantum memory for storing and manipulating quantum information and a quantum data bus to securely transfer information between quantum memories. Typically, a quantum memory is composed of a matter system, such as an atom or an electron spin, due to their prolonged quantum coherence. Alternatively, a quantum data bus is typically composed of some propagating degree of freedom, such as a photon, which can retain quantum information over long distances. Therefore, a quantum computer will likely be a hybrid quantum device, consisting of two or more disparate quantum systems. However, there must be a reliable and controllable quantum interface between the memory and bus in order to faithfully interconvert quantum information. The current engineering challenge for quantum computers is scaling the device to large numbers of controllable quantum systems, which will ultimately depend on the choice of the quantum elements and interfaces utilized in the device. In this thesis, we present and characterize a hybrid quantum device comprised of single nitrogen-vacancy (NV) centers embedded in a high quality factor diamond mechanical oscillator. The electron spin of the NV center is a leading candidate for the realization of a quantum memory due to its exceptional quantum coherence times. On the other hand, mechanical oscillators are highly sensitive to a wide variety of external forces, and have the potential to serve as a long-range quantum bus between quantum systems of disparate energy scales. These two elements are interfaced through crystal strain generated by vibrations of the mechanical oscillator. Importantly, a strain interface allows for a scalable architecture, and furthermore, opens the door to integration into a larger quantum network through coupling to an optical interface.There are a few important engineering challenges associated with this device. First, there have been no previous demonstrations of a strain-mediated spin-mechanical interface and hence the system is largely uncharacterized. Second, fabricating high quality diamond mechanical oscillators is difficult due to the robust and chemically inert nature of diamond. Finally, engineering highly coherent NV centers with a coherent optical interface in nanostructured diamond remains an outstanding challenge. In this thesis, we theoretically and experimentally address each of these challenges, and show that with future improvements, this device is suitable for future quantum-enabled applications. First, we theoretically and experimentally demonstrate a dynamic, strain-mediated coupling between the spin and orbital degrees of freedom of the NV center and the driven mechanical motion of a single-crystal diamond cantilever. We employ Ramsey interferometry to demonstrate coherent, mechanical driving of the NV spin evolution. Using this interferometry technique, we present the first demonstration of nanoscale strain imaging, and quantitatively characterize the previously unknown spin-strain coupling constants. Next, we use the driven motion of the cantilever to perform deterministic control of the frequency and polarization dependence of the optical transitions of the NV center. Importantly, this experiment constitutes the first demonstration of on-chip control of both the frequency and polarization state of a single photon produced by a quantum emitter. In the final experiment, we use mechanical driving to engineer a series of spin ``clock" states and demonstrate a significant increase in the spin coherence time of the NV center. We conclude this thesis with a theoretical discussion of prospective applications for this device, including generation of non-classical mechanical states and spin-spin entanglement, as well as an evaluation of the current limitations of our devices, including a possible avenues for improvement to reach the regime of strong spin-phonon coupling.