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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Towards integration of quantum interference in alkali atoms on a chip

Holger Schmidt, Dongliang Yin, Wenge Yang, Donald B. Conkey, John P. Barber, Aaron R. Hawkins, Bin Wu

Published Feb 9, 2006• 4 citations
Publisher

Abstract

We discuss a new integrated approach to realizing optical quantum interference effects such as electromagnetically induced transparency (EIT), slow light, and highly efficient nonlinear processes on a semiconductor chip. An ensemble of alkali atoms represents one of the canonical systems that exhibit slow light and related phenomena. At the same time, it would be desirable to build slow-light and related devices on a semiconductor platform in order to move to practical applications. We review progress towards combining the large magnitude of quantum interference effects in alkali vapors with the convenience of integrated optics in the form of hollow-core antiresonant reflecting optical waveguides (ARROWs). We discuss the benefits and challenges of this integrated approach with special emphasis on nonlinear optics. We present strategies to optimize the optical waveguides and discuss the current status of building rubidium-filled optical waveguides on a chip. Recent results on optimization of waveguide loss and transfer of rubidium atoms through hollow microchannels on a chip are presented.

DOI
10.1117/12.660175

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We discuss a new integrated approach to realizing optical quantum interference effects such as electromagnetically induced transparency (EIT), slow light, and highly efficient nonlinear processes on a semiconductor chip. An ensemble of alkali atoms represents one of the canonical systems that exhibit slow light and related phenomena. At the same time, it would be desirable to build slow-light and related devices on a semiconductor platform in order to move to practical applications. We review progress towards combining the large magnitude of quantum interference effects in alkali vapors with the convenience of integrated optics in the form of hollow-core antiresonant reflecting optical waveguides (ARROWs). We discuss the benefits and challenges of this integrated approach with special emphasis on nonlinear optics. We present strategies to optimize the optical waveguides and discuss the current status of building rubidium-filled optical waveguides on a chip. Recent results on optimization of waveguide loss and transfer of rubidium atoms through hollow microchannels on a chip are presented.
We review the current status of integrating optical quantum interference effects such as electromagnetically induced transparency (EIT), slow light, and highly efficient nonlinear processes on a semiconductor chip. A necessary prerequisite for combining effects such as slow light and related phenomena with the convenience of integrated optics is the development of integrated alkali vapor cells. Here, we describe the development of integrated rubidium cells based on hollow-core antiresonant reflecting optical waveguides (ARROWs). Hollow-core waveguides were fabricated on a silicon platform using conventional microfabrication and filled with rubidium vapor using different methods. Rubidium absorption through the waveguides was successfully observed which opens the way to integrated atomic and molecular on a chip. The realization of quantum coherence effects requires additional surface treatment of the waveguide walls, and the effects of the surface coating on the waveguide properties are presented.
Atomic vapors of alkali metals are widely used to slow and stop light in tabletop experiments. In order to take advantage of the underlying quantum interference effects in future commercial devices, highly reactive alkali atoms must be incorporated into small volumes with integrated optical access. With integration in mind, we describe the development of a hollow-core waveguide technology based on the combination of vapor-filled hollow waveguides and conventional solid-core waveguides on a silicon chip. We discuss the underlying principles of the waveguide design, the development of different approaches to building on-chip vapor cells, the demonstration of linear and nonlinear rubidium spectroscopy on a chip, and the prospects for quantum interference effects such as slow light and giant Kerr nonlinearities using this approach. Ultrasmall active vapor volumes on the order of 100 picoliters with simultaneously high optical density in excess of two illustrate the potential of planar hollow-core waveguides for linear and nonlinear optical spectroscopy of atoms confined on a chip.
The demonstration of slow, fast, and stopped light1 has helped generate considerable interest in quantum interference effects. In addition to producing intriguing physical phenomena, these effects will be valuable for future optical communications. Buffers using slow-light modules will be important elements in alloptical data networks. Cryptography systems may also be expected to use quantum interference effects for photon creation and detection. But if slow-light buffers and quantum cryptography are to be practical in real-world applications, wemust create miniaturized, stand-alone quantum interference modules. This is the aim of research involving on-chip atomic vapor cells integrated with optical waveguides Slow-light effects are a product of a medium with large, frequency-dependent gain or absorption features that then give rise to large dispersion characteristics. Our work employs quantum interference effects in atomic vapor to create large dispersion. At present, atomic vapor can provide excellent dispersion characteristics, but it usually requires a large system footprint. In classical optical setups, which beam a laser through a transparent vapor cell, there is also a constant trade-off between focal depth and beamwidth. By using on-chip hollow-core optical antiresonant reflecting optical waveguides (ARROWs), we are able to direct light down vapor-filled cores, maintaining large optical intensities over long distances. This is particularly beneficial for nonlinear optical effects that can be exploited for single-photon generation and detection. In addition, ARROW-based platforms also require only a small footprint (1×1cm). ARROWs are constructed by growing alternating layers of silicon oxide and silicon nitride around a sacrificial core on a silicon wafer. The alternating dielectric materials with specific thicknesses confine and guide light through antiresonance. After etching out the sacrificial core, we are left with a hollow channel into which we can introduce various gases and liquids for optical experiments. Solid waveguides etched into the silicon on Figure 1. A rubidium (Rb)-loaded ARROW atomic vapor cell.
The focus of this work is the integration of alkali vapor atomic vapor cells into common silicon wafer microfabrication processes. Such integrated platforms enable the study of quantum coherence effects such as electromagnetically induced transparency, which can in turn be used to demonstrate slow light. Slow and stopped light devices have applications in the optical communications and quantum computing fields. This project uses hollow core anti-resonant reflecting optical waveguides (ARROWs) to build such slow light devices. An explanation of light-matter interactions and the physics of slow light is first provided, as well as a detailed overview of the fabrication process. Following the discovery of a vapor transport issue, a custom capillary-based testing platform is developed to quantify the effect of confinement, temperature, and wall coatings on rubidium transport. A mathematical model is derived from the experimental results and predicts long transport times. A new design methodology is presented that addresses the transport problem by increasing the number of rubidium entry points. This design also improves chip durability and decreases environmental susceptibility through the use of a single copper reservoir and buried channel waveguides (BCWs). New chips are successfully fabricated, loaded, and monitored for rubidium spectra. Absorption is observed in several chips and absorption peaks depths in excess of 10% are reported. The chip lifetime remains comparable to previous designs. This new design can be expanded to a multi-core platform suitable for slow and stopped light experimentation.
We analyze the integration of electromagnetically induced transparency in alkali atoms on a semiconductor chip. We propose the use of antiresonant reflecting optical waveguides with hollow cores to realize the necessary waveguiding capability and optical mode areas of a few square micrometers. We derive the scaling laws and limitations for the reduction in group velocity and single-photon phase shifts as a function of waveguide dimension. We show that miniaturization leads to a large enhancement of single-photon cross-phase modulation, despite the presence of additional limitations due to coherence dephasing and waveguide loss.