Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Applied Physics Letters

Generation of broadband frequency-entangled photons using plasmon nanoantenna

Hisaki Oka

Published Oct 21, 2013• 8 citations
Publisher

Abstract

A scheme for the generation of frequency-entangled photons using a plasmon nanoantenna system is proposed. The nanoantenna system consists of two large metallic nanostructures confined in a one-sided microcavity with high spontaneous emission factor. Two input photons are converted into an entangled photon pair via the saturation effect of the nanoantenna. The degree of entanglement of the resultant entangled photons is evaluated using the entropy of entanglement, E. We show that broadband frequency-entangled photons with E up to ≈0.45 are generated owing to rapid plasmon radiative decay.

DOI
10.1063/1.4826646

Related papers

Generation of broadband ultraviolet frequency-entangled photons using cavity quantum plasmonics

Hisaki Oka

Application of quantum entangled photons is now extending to various fields in physics, chemistry and biology. In particular, in terms of application to molecular science, broadband ultraviolet frequency-entangled photons are desired because molecules inducing photochemical reactions of interest often have electronic transition energies in the ultraviolet region. Recent standard method for generating such entangled photons is a chirped quasi-phase-matching method, however this method is not suitable for the generation of ultraviolet frequency-entangled photons because it requires down-conversion of a photon with a wavelength shorter than ultraviolet into an entangled photon pair. Here we propose a simple method for generating broadband ultraviolet frequency-entangled photons using cavity quantum plasmonics, in which conventional cavity quantum electrodynamics theory is applied to quantum plasmonics. We introduce a cavity-plasmon system in which localised surface plasmon (LSP) is coupled to the cavity fields of a state-of-the-art microcavity. Using this system, we theoretically show that broadband ultraviolet frequency-entangled photons can be generated simply by utilising the absorption saturation effect of LSP.

Scientific Reports•Aug 8, 2017•3 citations

General framework for two-photon spontaneous emission near plasmonic nanostructures

S. Smeets, Björn Maes, Gilles Rosolen

The authors develop a framework for efficient calculation of two-photon spontaneous emission in arbitrary nanostructures using one-photon Purcell factors. The formalism will aid the design of entangled two-photon sources for various applications, including quantum technologies and spectroscopy.

Physical Review A•Jun 27, 2023•12 citations

Dissipation-driven entanglement between qubits mediated by plasmonic nanoantennas

Jiamin Hou, Karolina Słowik, F. Lederer +1 more

A scheme is proposed to generate a maximally entangled state between two qubits by means of a dissipation-driven process. To this end, we entangle the quantum states of qubits that are mutually coupled by a plasmonic nanoantenna. Upon enforcing a weak spectral asymmetry in the properties of the qubits, the steady-state probability to obtain a maximally entangled, subradiant state approaches unity. This occurs despite the high losses associated with the plasmonic nanoantenna that are usually considered as being detrimental. The entanglement scheme is shown to be quite robust against variations in the transition frequencies of the quantum dots and deviations in their prescribed position with respect to the nanoantenna. Our work paves the way for applications in the field of quantum computation in highly integrated optical circuits.

arXiv:1403.0794•Physical Review B•Jun 12, 2014•49 citations

Two-Photon Spontaneous Emission in Atomically Thin Plasmonic Nanostructures

Yunuhen Muñiz, Alejandro Manjavacas, Carlos Farina +2 more

The ability to harness light-matter interactions at the few-photon level plays a pivotal role in quantum technologies. Single photons-the most elementary states of light-can be generated on demand in atomic and solid state emitters. Two-photon states are also key quantum assets, but achieving them in individual emitters is challenging because their generation rate is much slower than competing one-photon processes. We demonstrate that atomically thin plasmonic nanostructures can harness two-photon spontaneous emission, resulting in giant far field two-photon production, a wealth of resonant modes enabling tailored photonic and plasmonic entangled states, and plasmon-assisted single-photon creation orders of magnitude more efficient than standard one-photon emission. We unravel the two-photon spontaneous emission channels and show that their spectral line shapes emerge from an intricate interplay between Fano and Lorentzian resonances. Enhanced two-photon spontaneous emission in two-dimensional nanostructures paves the way to an alternative efficient source of light-matter entanglement for on-chip quantum information processing and free-space quantum communications.

arXiv:2006.15219•Physical Review Letters•Jul 15, 2020•34 citations

Generation of long-time maximum entanglement between two dipole emitters via a hybrid photonic-plasmonic resonator

Siping Liu, Jiahua Li, Rong Yu +1 more

We explore the entanglement generation between two dipole emitters via a hybrid photonic-plasmonic resonant structure which consists of two metal nanoparticles (MNPs) and a high-$Q$ whispering-gallery-mode (WGM) microcavity. Because the coupling strength between the dipole emitter and the cavity can be substantially enhanced with the help of MNPs and maintained by the WGM cavity, the maximum entanglement plateau between two dipole emitters can be deterministically created even in the presence of the spontaneous emission of the dipole emitters and the decay induced by the microcavity and MNPs. The width of the plateau depends on the coupling strengths (or the radii of the MNPs) and the initial state, but is insensitive to the dipole-cavity detuning. These results are useful in real experiments.

Physical Review A•Apr 4, 2013•23 citations

Spontaneous photon-pair generation from a dielectric nanoantenna

Giuseppe Marino, Alexander S. Solntsev, Lei Xu +13 more

Optical nanoantennas have shown a great capacity for efficient extraction of photons from the near to the far-field, enabling directional emission from nanoscale single-photon sources. However, their potential for the generation and extraction of multi-photon quantum states remains unexplored. Here we demonstrate experimentally the nanoscale generation of two-photon quantum states at telecommunication wavelengths based on spontaneous parametric down-conversion in an optical nanoantenna. The antenna is a crystalline AlGaAs nanocylinder, possessing Mie-type resonances at both the pump and the bi-photon wavelengths and when excited by a pump beam generates photonpairs with a rate of 35 Hz. Normalized to the pump energy stored by the nanoantenna, this rate corresponds to 1.4 GHz/Wm, being one order of magnitude higher than conventional on-chip or bulk photon-pair sources. Our experiments open the way for multiplexing several antennas for coherent generation of multi-photon quantum states with complex spatial-mode entanglement and applications in free-space quantum communications and sensing.

arXiv:1903.06956•Optica•Oct 31, 2019•166 citations
A scheme for the generation of frequency-entangled photons using a plasmon nanoantenna system is proposed. The nanoantenna system consists of two large metallic nanostructures confined in a one-sided microcavity with high spontaneous emission factor. Two input photons are converted into an entangled photon pair via the saturation effect of the nanoantenna. The degree of entanglement of the resultant entangled photons is evaluated using the entropy of entanglement, E. We show that broadband frequency-entangled photons with E up to ≈0.45 are generated owing to rapid plasmon radiative decay.
Application of quantum entangled photons is now extending to various fields in physics, chemistry and biology. In particular, in terms of application to molecular science, broadband ultraviolet frequency-entangled photons are desired because molecules inducing photochemical reactions of interest often have electronic transition energies in the ultraviolet region. Recent standard method for generating such entangled photons is a chirped quasi-phase-matching method, however this method is not suitable for the generation of ultraviolet frequency-entangled photons because it requires down-conversion of a photon with a wavelength shorter than ultraviolet into an entangled photon pair. Here we propose a simple method for generating broadband ultraviolet frequency-entangled photons using cavity quantum plasmonics, in which conventional cavity quantum electrodynamics theory is applied to quantum plasmonics. We introduce a cavity-plasmon system in which localised surface plasmon (LSP) is coupled to the cavity fields of a state-of-the-art microcavity. Using this system, we theoretically show that broadband ultraviolet frequency-entangled photons can be generated simply by utilising the absorption saturation effect of LSP.
A scheme is proposed to generate a maximally entangled state between two qubits by means of a dissipation-driven process. To this end, we entangle the quantum states of qubits that are mutually coupled by a plasmonic nanoantenna. Upon enforcing a weak spectral asymmetry in the properties of the qubits, the steady-state probability to obtain a maximally entangled, subradiant state approaches unity. This occurs despite the high losses associated with the plasmonic nanoantenna that are usually considered as being detrimental. The entanglement scheme is shown to be quite robust against variations in the transition frequencies of the quantum dots and deviations in their prescribed position with respect to the nanoantenna. Our work paves the way for applications in the field of quantum computation in highly integrated optical circuits.
The ability to harness light-matter interactions at the few-photon level plays a pivotal role in quantum technologies. Single photons-the most elementary states of light-can be generated on demand in atomic and solid state emitters. Two-photon states are also key quantum assets, but achieving them in individual emitters is challenging because their generation rate is much slower than competing one-photon processes. We demonstrate that atomically thin plasmonic nanostructures can harness two-photon spontaneous emission, resulting in giant far field two-photon production, a wealth of resonant modes enabling tailored photonic and plasmonic entangled states, and plasmon-assisted single-photon creation orders of magnitude more efficient than standard one-photon emission. We unravel the two-photon spontaneous emission channels and show that their spectral line shapes emerge from an intricate interplay between Fano and Lorentzian resonances. Enhanced two-photon spontaneous emission in two-dimensional nanostructures paves the way to an alternative efficient source of light-matter entanglement for on-chip quantum information processing and free-space quantum communications.
We explore the entanglement generation between two dipole emitters via a hybrid photonic-plasmonic resonant structure which consists of two metal nanoparticles (MNPs) and a high-QQQ whispering-gallery-mode (WGM) microcavity. Because the coupling strength between the dipole emitter and the cavity can be substantially enhanced with the help of MNPs and maintained by the WGM cavity, the maximum entanglement plateau between two dipole emitters can be deterministically created even in the presence of the spontaneous emission of the dipole emitters and the decay induced by the microcavity and MNPs. The width of the plateau depends on the coupling strengths (or the radii of the MNPs) and the initial state, but is insensitive to the dipole-cavity detuning. These results are useful in real experiments.
Optical nanoantennas have shown a great capacity for efficient extraction of photons from the near to the far-field, enabling directional emission from nanoscale single-photon sources. However, their potential for the generation and extraction of multi-photon quantum states remains unexplored. Here we demonstrate experimentally the nanoscale generation of two-photon quantum states at telecommunication wavelengths based on spontaneous parametric down-conversion in an optical nanoantenna. The antenna is a crystalline AlGaAs nanocylinder, possessing Mie-type resonances at both the pump and the bi-photon wavelengths and when excited by a pump beam generates photonpairs with a rate of 35 Hz. Normalized to the pump energy stored by the nanoantenna, this rate corresponds to 1.4 GHz/Wm, being one order of magnitude higher than conventional on-chip or bulk photon-pair sources. Our experiments open the way for multiplexing several antennas for coherent generation of multi-photon quantum states with complex spatial-mode entanglement and applications in free-space quantum communications and sensing.