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Journal of Optics B Quantum and Semiclassical Optics

Mapping a quantum state of light onto atoms

Jan Hald, Eugene Simon Polzik

Published Feb 1, 2001• 22 citations
Publisher

Abstract

We derive a theory for mapping a quantum state of nonclassical light onto a collective, excited atomic state via complete absorption of the light. We allow for an arbitrary polarization-squeezed state of light and an arbitrary spin of the atomic ground state. The present derivation thereby generalizes the results of Kuzmich et al . We compare the theory to the recently published experimental results on atomic spin squeezing.

DOI
10.1088/1464-4266/3/1/365

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We derive a theory for mapping a quantum state of nonclassical light onto a collective, excited atomic state via complete absorption of the light. We allow for an arbitrary polarization-squeezed state of light and an arbitrary spin of the atomic ground state. The present derivation thereby generalizes the results of Kuzmich et al . We compare the theory to the recently published experimental results on atomic spin squeezing.
We propose an experimentally feasible way to generate spin squeezing in an ensemble of V-type atoms. The proposal involves absorption of a squeezed light beam, and it does not require a large solid angle to be occupied by squeezed light. 50% of the amount of squeezing of the optical field can be transferred onto spin squeezing of the excited atomic states. The analogy with the input-output theory for quantum fields is used to elucidate this result. An experimental setup for generation and detection of spin squeezing within magnetic or hf manifolds is outlined.
We consider an ensemble of trapped atoms interacting with a continuous-wave laser field. For sufficiently polarized atoms and for a polarized light field, we may approximate the nonclassical components of the collective spin angular momentum operator for the atoms and the Stokes vectors of the field by effective position and momentum variables for which we assume a Gaussian state. Within this approximation, we present a theory for the squeezing of the atomic spin by polarization rotation measurements on the probe light. We derive analytical expressions for the squeezing with and without inclusion of the noise effects introduced by atomic decay and by photon absorption. The theory is readily adapted to the case of inhomogeneous light-atom coupling [A. Kuzmich and T.A.B. Kennedy, Phys. Rev. Lett. 92, 030407 (2004)]. As a special case, we show how to formulate the theory for an optically thick sample by slicing the gas into pieces, each having only small photon absorption probability. Our analysis of a realistic probing and measurement scheme shows that it is the maximally squeezed component of the atomic gas that determines the accuracy of the measurement.
In this thesis I explore the use of collective spin angular momentum as a platform for quantum information processing. Such systems have several nice features that make them excellent choices for such protocols, especially ones where information is also stored in photonic variables. The longer coherence times of atoms makes it possible to store information from light in atoms for future use, and it is generally easier to couple atomic variables than to create nonlinear interactions of light. Above and beyond the advantages of atomic systems, collective atomic systems have additional strengths. In the limit of a large number of atoms, the collective variables of atomic systems have a natural connection to the bosonic algebra of light (known as the Holstein-Primakoff or HP approximation) where components of the collective spin angular momentum effectively act as quadratures, making them natural systems for coupling to light. Also, collectively addressing the atoms allows one to access a large state space without individual addressing of the atoms. A natural first step towards control of these collective variables is generating large amounts of atomic spin squeezing. In the HP approximation going from rotations to squeezing corresponds to going from linear to quadratic interactions in the atomic quadratures; for extremely large squeezing one should see the breakdown of the HP approximation and the ability to generate arbitrary collective atomic states. I have sought to improve previous schemes for the spin squeezing of atomic ensembles, such as the proposal of Takeuchi et. al. based on coherent quantum feedback. In this scheme a beam of linearly polarized light passes through the atomic ensemble (prepared in a coherent state), coupling to the atoms through a state-dependent index of refraction (the Faraday effect). The light is then passed through a wave-plate and reflected back through the atoms for a second pass. This double-pass scheme leads to an effective nonlinearity as the atomic fluctuations are mapped onto the light on the first pass and then back on to the atoms in the second pass. The light acts as a bus coupling each atom to each of the others. This nonlinear interaction forms a shearing of the atomic coherent state that results in squeezing. The light is entangled to the atoms through these interactions, and remains entangled as it escapes the system. This leads to decoherence of the atoms as the light is lost to the environment, reducing the amount of spin squeezing achieved. The first step towards improving the double-pass scheme was to add a quantum eraser step in which the light is disentangled from the squeezed atoms. By first measuring one quadrature of the light, and then performing a measurement-dependent rotation on the atomic ensemble, it is possible to decouple the atoms and light so that the loss of the light does not reduce the atomic squeezing. This results in an improvement of the rate of atomic spin squeezing. The nonlinear shearing interaction that remains still falls short of the exponential squeezing seen in optical parametric amplification. The reason for this can be seen by decomposing the shearing interaction into squeezing along a given quadrature followed by a rotation. The rotation leads to a constantly changing axis along which the squeezing occurs, and thus the squeezing builds up more slowly. This can be corrected for by breaking up the light pulse into a sequence of small pulses, and performing a small phase matching rotation after each pulse. The squeezing then adds up along a constant direction, rather than along a constantly varying direction. This results in still further improvement of the rate of atomic spin squeezing. A complete model includes the effects of photon-atom scattering and other noise and loss effects on the overall rate of squeezing. Previous derivations of noise due to photon-atom scattering have started with the unjustified assumptions that the atomic and photonic decoherence channels were both Gaussian and independent of correlations between the two subsystems. They then proceed with very general statistical arguments that rely upon these simplifications. My work begins with the more fundamental master equation picture in which I find the Linblad jump operators. I find that in general the photonic and atomic loss channels are not independent, with the intensity of the light dictating the details of this dependence, and find the conditions under which the Gaussian approximation holds. Squeezing and loss is initially treated assuming ensembles of spin-1/2 atoms, but this work is further extended to higher dimensional subsystems. For a higher spin case, preparing the atoms in spin coherent states is not optimal. One can engineer a stronger interaction by preparing the atoms in an atomic "cat state", i.e., a superposition of the two stretch states along the direction of propagation of the light beam. The fluctuations of such a state are more strongly coupled to the light, resulting in a stronger nonlinearity. This leads to strong correlations between the atoms, but they are not immediately useful for squeezing; the cat state must be coherently mapped to a coherent state to achieve atomic spin squeezing. The state created in this manner is ultimately more squeezed than that achieved with the same interaction but prepared initially in a coherent state.
We investigate the generation of entanglement (spin squeezing) in an optical-transition atomic clock through the coupling to an optical cavity in its vacuum state. We show that if each atom is prepared in a superposition of the ground state and a long-lived electronic excited state, and viewed as a spin-1/2 system, then the collective vacuum light shift entangles the atoms, resulting in a squeezed distribution of the ensemble collective spin, without any light applied. This scheme reveals that even an electromagnetic vacuum can constitute a useful resource for entanglement and quantum manipulation. By rotating the spin direction while coupling to the vacuum, the scheme can be extended to implement two-axis twisting resulting in stronger squeezing.