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Physical Review A

Spectral modification of the Stokes line of a Raman-coupled three-level system in a cavity

Gautam Gangopadhyay, Deb Shankar Ray

Published Feb 1, 1992• 4 citations
Publisher

Abstract

We have investigated the spectral modification of the Raman Stokes line in the cavity version of Raman scattering where a three-level system in the \ensuremath{\Lambda} configuration interacts with an externally driven pump mode and a Stokes mode in a cavity. Anti-Stokes modes are eliminated by the cavity-resonance condition. At very low intensities the spectrum consists of a single-peak structure (Raman Stokes) that splits into a doublet when the external pump field is sufficiently intense so that the effective Rabi frequency exceeds the rate of spontaneous emission. At very high intensity, however, a triplet structure appears where the strong sidebands are symmetrically separated from the central weak band.

DOI
10.1103/physreva.45.1843

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We have investigated the spectral modification of the Raman Stokes line in the cavity version of Raman scattering where a three-level system in the \ensuremath{\Lambda} configuration interacts with an externally driven pump mode and a Stokes mode in a cavity. Anti-Stokes modes are eliminated by the cavity-resonance condition. At very low intensities the spectrum consists of a single-peak structure (Raman Stokes) that splits into a doublet when the external pump field is sufficiently intense so that the effective Rabi frequency exceeds the rate of spontaneous emission. At very high intensity, however, a triplet structure appears where the strong sidebands are symmetrically separated from the central weak band.
The general method developed in a previous paper (see ibid., vol.10, p.345 (1977)) is applied to the problem of resonance Raman scattering in very intense laser fields. At very low intensities the spectrum consists of three monochromatic lines (Rayleigh, Raman Stokes and anti-Stokes) which split into a triplet and two doublets when the laser light, tuned on one of the two transitions connecting the upper state to the two lower sublevels, has a sufficiently high intensity to saturate this transition but not the second one. The Raman and Rayleigh lines are completely mixed when the intensity becomes so high that both transitions are saturated. The corresponding evolution of the spectrum is determined. Optical-pumping effects leading to asymmetries in the fluorescence spectrum are taken into account.
The theory of coherent anti-Stokes Raman scattering (CARS) is extended to include the effect of pump fluctuations. The intensities and spectra of lines in resonant CARS are calculated to all orders in fields assuming a phase-diffusion model for waves at the two pump frequencies. The bandwidth of the two lasers enters in a much more complicated way than following a simple scaling of T1{T}_{1}T1​ or T2{T}_{2}T2​. Various resonances in CARS spectra due to dynamic splitting of the energy levels are discussed for a range of detunings, field intensities, and bandwidths. In contrast to the usual spectra in strong fields, the Rabi sidebands appear as dispersion-shaped structures. The laser linewidth is shown to change dramatically the CARS line shape. The case of no saturation is also treated, thus allowing for the inclusion of more general line shapes and fluctuations of the pump waves and the nonlinear susceptibility tensor ${\ensuremath{\chi}}^{(3)}$. Gaussian statistics of the pump field are shown to lead to enhancement factors in CARS intensity, similar to those appearing in the context of multiphoton absorption processes.
We consider a two-channel \ensuremath{\Lambda}-type three-level atom interacting simultaneously with two quantized cavity fields and a classically described cw laser field, all of different frequencies. The effective interactions are of the Raman type, in which the two cavity fields are regarded as Stokes and anti-Stokes modes, and the classical field acts as the pump mode, so that both the pump-Stokes and the pump--anti-Stokes transitions are included. We present the analytic solution of the system evolution operator. We also study the time dependence of the atomic inversion and the statistical properties of the cavity fields. We show that strongly correlated photons can be generated in our model.
The quantum theory of Stokes--anti-Stokes processes in a degenerate system in a cavity is developed. The Raman transition is pumped by a coherent field. Effects of many atoms, cavity losses, and thermal photons are included in the theory. An exact solution for the model is obtained. An explicit expression for the reduced density matrix of the cavity field is given. The spectrum of the cavity field is obtained and is interpreted in terms of the eigenstates of the effective Hamiltonian describing Stokes--anti-Stokes processes. The spectrum develops sidebands due to strong Raman coupling.
We discuss the frequency dependence of the spontaneous-emission rate (power) in a Fabry-Perot microcavity containing a Lorentz dielectric, with emphasis on modifications of the spectrum under the circumstances of the strong medium-cavity coupling. With the standard-cavity tuning, the total spontaneous-emission power spectrum consists of a multiwave version of the familiar low-frequency vacuum Rabi split peak and a broad structure on the high-frequency side coming from the enhanced spontaneous emission into the continuum of the obliquely propagating waves. This form of the spectrum derives from the properties of the (single-wave) radiation-intensity spectrum of the molecule. Depending on the observation direction, the radiation-intensity spectrum exhibits either a double-peak structure characteristic of the vacuum Rabi splitting, as observed in light transmisssion and reflection experiments, or a single-peak structure describing the enhanced spontaneous emission at the corresponding cavity resonant frequency.
I study the coherent interaction of a three-level atom in the lambda configuration with pump, Stoke, and anti-Stokes laser fields. The pump laser field drives transitions from the two non-degenerate lower levels to the excited state which is highly detuned for either transition. This excited state is also coupled to each of the lower states by Stokes or anti-Stokes transitions so that this system may represent a model of four-wave mixing. Assuming large detunings, the excited state is adiabatically eliminated from obtaining an effective two-level system with Raman coupling between the levels. Optical Bloch equations are obtained for this effective two-level system, and phenomenological damping terms are added for collisional dephasing of the Raman transitions. The equations are solved for the steady-state as well as by the method of adiabatic following. From these solutions we obtain the polarization.