We have experimentally studied the dynamics of rubidium atoms in a magneto-optical trap employing optical σ+ σ--molasses with controlled time phase differences in a vapour cell. We find that the action of radiation pressure vortices gives rise to a novel long-range interaction between the atoms which may explain the irregular atomic-density distributions possible in such traps even at perfect alignment. We have also recorded absorption spectra of trapped low-density atomic samples which include time-phase-dependent narrow Raman and Rayleigh resonances.
We have experimentally studied the dynamics of rubidium atoms in a magneto-optical trap employing optical σ+ σ--molasses with controlled time phase differences in a vapour cell. We find that the action of radiation pressure vortices gives rise to a novel long-range interaction between the atoms which may explain the irregular atomic-density distributions possible in such traps even at perfect alignment. We have also recorded absorption spectra of trapped low-density atomic samples which include time-phase-dependent narrow Raman and Rayleigh resonances.
We have studied the behavior of clouds of neutral atoms contained in a spontaneous force optical trap. Because of the low temperatures of the atoms (<1 mK) we have observed a variety of new phenomena which involve both short and long range interactions between the atoms. The short range interactions are manifested in two body collisions which are notable because of the very long collision times. This time scale causes the dynamics to be profoundly affected by absorption and spontaneous emission during the collision. An interesting assortment of collective behaviors are observed when the trapped atom cloud contains more than 105 atoms. These include the expansion of the cloud as the number is increased and dramatic changes in the distribution of the atoms at higher numbers. We can explain much of the collective behavior using a simple model that includes a 1/r2 force between the atoms arising from the multiple scattering of photons. Finally, we discuss the optical trapping of atoms directly from a low pressure vapor in a small glass cell. We have used these optically trapped atoms to load a magnetostatic trap in the same cell. This provided a high density sample of atoms with a temperature of less than 2 μK.
A cloud of ultracold atoms confined in a magneto-optical trap (MOT) has a temperature greater than that of a low-density vapour in the same light field. It has been observed (Drewsen M. et al., Appl. Phys. B , 59 (1994) 283) that this temperature excess is proportional to the cube root of the total number of trapped atoms ( N 1/3 ). We present an explanation for this effect in terms of the scattering which arises when photons spontaneously emitted by atoms have an appreciable probability of being reabsorbed within the cloud. This hypothesis has been tested by time-of-flight measurements of the temperature of clouds of atoms released from a MOT into 1-dimensional and 3-dimensional optical molasses in the σ + -σ - and lin ⊥ lin configuration.
This thesis describes theoretical and experimental work concerning radiation forces on atoms, with particular reference to rubidium atoms confined in a magneto-optical trap. After a short history of the field of laser cooling, a review of the semiclassical theory of mechanical interactions between two-level atoms and electromagnetic radiation is given. Different formulations of the semiclassical theory are discussed, including a new formulation in terms of momentum transfer amongst the plane wave modes of the electromagnetic field. Two important applications of light forces on atoms, namely 'optical molasses' and the 'magneto-optical trap', are then described with emphasis on experimental parameters. Three sub-Doppler cooling mechanisms, 'sisyphus cooling', 'motion-induced orientation cooling' and the 'magnetically-assisted sisyphus effect', are described and their role in optical molasses and the magneto-optical trap is discussed. A new study of the polarisation gradients which occur in 3-D monochromatic light fields is presented and quantifies their relative presence in different light field configurations. Polarisation gradient parameters are developed and shown to be directly related to the relativistic spin tensor of the light field. Implications of this polarisation gradient study for laser cooling work are discussed. The design, construction from scratch, operation and testing of a magneto-optical trap for rubidium are described, including novel designs for two vacuum cells. Preliminary experiments to characterise the trap are described and results are presented; they primarily concern the number and distribution of atoms in the trap. Finally. the theory of time domain spectroscopy is reviewed. The construction and testing of a pulsed dye laser for study of coherent transients in samples of laser-cooled atoms and a proposed experiment to measure the temperature of cold atoms using coherent transients are described. Factors expected to influence the shape of coherent transients in cold atoms are discussed.
An overview of the theory of the magneto-optical trap is presented, along with measurements of the effect of an imbalance in the intensities of the trapping beams. This investigation tests the theory of the spring constant of the trap and confirms that the confining force at the center of the trap results from an induced orientation of the atomic ground state. The experimental results give the magnitude of this force, which has not yet been calculated accurately. We calculate the radiation field in the three-dimensional molasses, finding that the relative time phase of the orthogonal standing waves is significant, and we give some insight into the phenomenon of interference fringes when the beams are misaligned. We also discuss the limitation of the trapped atomic density resulting from photon scattering within the cloud, predicting that densities above 1013 atoms/cm3 could be achieved in a trap operating at low saturation of the atomic transition. Finally, we briefly consider collisional loss at low densities, finding an especially large contribution from resonant dipole–dipole scattering.
NOTE: Text or symbols not renderable in plain ASCII are indicated by [...]. Abstract is included in .pdf document. Investigations of optical processes for laser cooled and trapped atoms are described. Fluorescence from Cs atoms in a magneto-optical trap is detected under conditions of very low atomic density. Discrete steps are observed in the fluorescent signal versus time and are associated with the arrival and departure of individual trapped atoms. Histograms of the frequency of occurrence of a given level of fluorescence exhibit a series of uniformly spaced peaks that are attributed to the presence of N = 0, 1, 2 atoms in the trap. In addition, numerical absorption and emission spectra for three-level [...], [...], and V systems under intense radiations are calculated. Absorption spectra for a [...] system is used to explain the probe-wave amplification and absorption spectra recorded for Cs atoms cooled and confined in a magneto-optical trap, in which novel spectral features of narrow frequency widths with single-pass gain exceeding 20% are observed. The consequence of the optical gain is demonstrated to lead to negative radiation pressure, which is investigated together with other mechanical forces in the trap. Various alternative trapping schemes in three-level and two-level atoms are proposed as possible means to compress an atomic sample and demonstrated for a two-level magneto-optical trap.
This thesis reports on the design, setup, and operation of a new atom trap apparatus, which is developed to confine few rubidium atoms in ultrahigh vacuum by means of taylored and dynamically variable light potentials (dipole traps), thus making the atoms available for spectroscopy and controlled manipulations. To maintain low background pressure, atoms of a vapour cell are transferred into a cold atomic beam by laser cooling techniques, and accumulated by a magneto-optic trap (MOT) in a separate part of the vacuum system. The laser cooled atoms are then transferred into dipole traps made of focused far-off-resonant laser fields in single or crossed-beam geometry, which are superimposed with the center of the MOT. Gaussian as well as hollow Laguerre-Gaussian (LG01) beam profiles are used with red-detuned and blue-detuned light. Microfabricated dielectric phase objects allow the efficient and robust mode conversion of Gaussian into Laguerre-Gaussian laser beams. Trap geometries can easily be changed due to the highly flexible experimental setup. The dipole trap laser beams have powers up to several hundred milliwatts and are focused to around 10 m. At a detuning of several tens of nanometers from the atomic resonance, the resulting traps are a few millikelvin deep, and the trapped atoms exhibit motional frequencies near 30 kHz, trap light scattering rates of a few hundred photons per second per atom, and storage times of several seconds. The number of dipole-trapped atoms ranges from more than ten thousand to below ten. The dipole-trapped atoms are detected either by a photon counting system with efficient straylight discrimination, or by recapture into the MOT, which is imaged onto a sensitive photodiode and a CCD-camera. Due to the strong AC-Stark shift imposed by the high-intensity trapping light, energy-selective resonant excitation and detection of the stored atoms is possible. The measured energy distribution is consistent with a harmonic potential shape and allows for the determination of temperatures and heating rates. From initial measurements, the thermal energy is found to be about 10 % of the trap depth. Using a crossed-beam geometry with red-detuned laser light, efficient transfer of atoms between the beams is observed. Optimum transfer occurs when the two beams cross at a radial offset, which can qualitatively be understood when the particle energy and geometrical properties of the two-beam trapping potential are considered. Numerical simulations reproduce the general features of the measured transfer efficiency vs. radial beam offset. This experiment is a first step towards dynamically variable potentials. Atoms have been radially confined in a blue-detuned hollow beam, and their decay time has been determined. This configuration is currently extended to a three-dimensionally confining blue-detuned dipole trap. For advanced laser cooling, state manipulation and spectroscopy of trapped atoms, a system of two diode lasers has been set up which are phase-coherently locked with a difference frequency near 6.834 GHz, to drive Raman transitions between the hyperfine-split ground states of 87Rb atoms. Resonances of such a transition have been recorded in a buffer gas loaded rubidium vapour cell with linewidths below 100 Hz.