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Europhysics Letters (EPL)

Quantum Correlation between Fundamental and Second Harmonic in SHG

R. J. Horowicz

Published Nov 15, 1989• 24 citations
Publisher

Abstract

It is shown theoretically that nonclassical correlations between the fundamental and the second-harmonic mode exist for second-harmonic generation in a resonant optical cavity. The fluctuations in the sum of the intensities are reduced relative to the corresponding shot-noise level, even beyond the value expected for two uncorrelated sub-Poissonian beams.

DOI
10.1209/0295-5075/10/6/006

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It is shown theoretically that nonclassical correlations between the fundamental and the second-harmonic mode exist for second-harmonic generation in a resonant optical cavity. The fluctuations in the sum of the intensities are reduced relative to the corresponding shot-noise level, even beyond the value expected for two uncorrelated sub-Poissonian beams.
We consider the process of second-harmonic generation (SHG) in a cavity that is resonant for both the fundamental- and second-harmonic modes. It has been previously shown that such a system displays a phase instability leading to self-pulsing and that one gets important intensity squeezing on both the fundamental- and second-harmonic mode for pump intensities close to but below, this instability threshold. Such a squeezing has been recently observed. We have analytically calculated the intensity-noise spectrum of the frequency-doubled field above such an instability threshold, using a semiclassical input-output technique for the treatment of quantum fluctuations.1 Such a method, introduced to deal with fluctuations around a stable solution, has been generalized to the self-pulsing domain. As expected, the instability brings excess noise to the output beams, especially around the zero-frequency, the self-oscillation frequency, and its harmonics. Remarkably, some regions exist in which where the noise increase is small; squeezing still occurs in this frequency range far in the instability domain.
The mutual influence of second-harmonic generation and nondegenerate downconversion inside the same cavity is studied. The threshold behavior and the stability of a semiclassical solution with all four modes oscillating resonantly is investigated. It is shown that under certain conditions the self-pulsing instability that occurs in second-harmonic generation is absent in the combined system. The squeezing spectra for the quadrature-phase amplitudes in the second harmonic and the fundamental, as well as the photon statistics in the downconverted modes, are derived analytically. As one of the various nonclassical features of this system, the second harmonic is found to exhibit excellent noise suppression at very large frequencies, with the frequency component of best squeezing being tunable by the pump parameter. The intricate interaction of the two nonlinear processes can give rise to twin beams of correlated photons, with sub-Poissonian statistics in each beam. These results are contrasted with the results for each nonlinear process by itself.
We investigate theoretically the spatial quantum correlations of the light produced by spontaneous emission in type-I second-harmonic generation in the traveling-wave configuration. It is first shown that spontaneous emission occurs at both fundamental and second-harmonic frequency. Considering the quantum fluctuations of the intensities collected in symmetrical parts of the far-field plane, nonclassical correlations below the shot noise are predicted not only at fundamental frequency, but also at second-harmonic frequency. The latter cannot be traced back to any twin-photon emission mechanism, but are generated by a secondary process acting on twin photons. This mechanism also creates correlations between fundamental and second-harmonic field, at a given transverse wave number, and at opposite wave numbers. The analysis of a simplified few-mode model, on a quantum level, provides a good qualitative understanding of these correlations.
The interaction of doubly resonant second harmonic generation and nondegenerate down-conversion in a cavity is shown to generate light with excellent noise suppression in two symmetrical dips moving away from zero frequency with increasing pump strength. This feature emerges not only in the amplitude noise of fundamental and second harmonic, but also in the single beam and the sum intensity fluctuation spectra of the twin beams produced by down-conversion, which makes this system a potentially useful source for quantum cryptography or optical quantum correlation experiments.
The input-output theory, originally developed for a linear coupling between cavity mode a and a bath, is extended to a coupling that is quadratic in the cavity mode operator a. We then apply this to second-harmonic generation, in a cavity that is resonant at the fundamental frequency and has an active laser medium working at the fundamental frequency. We find intensity squeezing of 50% below the shot-noise level in the output light at the second-harmonic frequency, whether or not the cavity is resonant at the second-harmonic frequency. To compare the singly resonant cavity to the doubly resonant cavity, we develop in an appendix a general technique for extracting a single mode from a continuum.