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Physical Review Letters

Excitation Spectrum of a Dimerized Next-Neighbor Antiferromagnetic Chain

B. Sriram Shastry, Bill Sutherland

Published Sep 28, 1981• 328 citations
Publisher

Abstract

The excitation spectrum of an antiferromagnetic chain exhibiting the effects of both dimerization and frustration is studied. The method used is based on an exact solution for the doubly degenerate ground state, and views the excitations as propagating defect boundaries between the two exact ground states. These excitations are analogous to "solitons," and can bind into a second type of excitation, analogous to "breathers."

DOI
10.1103/physrevlett.47.964

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The excitation spectrum of an antiferromagnetic chain exhibiting the effects of both dimerization and frustration is studied. The method used is based on an exact solution for the doubly degenerate ground state, and views the excitations as propagating defect boundaries between the two exact ground states. These excitations are analogous to "solitons," and can bind into a second type of excitation, analogous to "breathers."
The excitation spectrum is studied around the degenerate point at the Ising limit in the one-dimensional anisotropic Heisenberg antiferromagnets with next-nearest-neighbor interactions. Solitons are found as propagation modes in the N\'eel state and in the (2,2) antiphase state, while triplet-dimer excitations are found propagating in the dimer state. These excitations determine the shape of dynamical spin-correlation functions, which are calculated by an exact diagonalization for finite chains. The phase diagram is determined from the condition that the energy gap vanishes in the excitation spectrum.
We study the antiferromagnetic spin chain with both dimerization and frustration. The classical ground state has three phases, a Néel phase, a spiral phase and a collinear phase, which we study through a nonlinear sigma-model approach. In the spiral phase, the field theory becomes and Lorentz invariant at long distances, a model which is exactly solvable. The low-energy spectrum is doubly degenerate with massive `elementary' spin-1/2 particles and `two-particle' triplet and singlet physical excitations. The field theory also supports solitons which lead to a double degeneracy of the ground state for half-integer spins (when there is no dimerization).
Starting from the exact result of Majumdar and Ghosh for the dimerized ground state of a Heisenberg linear-chain antiferromagnet with competing next-nearest-neighbor interaction J2{\mathit{J}}_{2}J2​=1/2J1{\mathit{J}}_{1}J1​, it is shown that this state is an exact eigenstate of the same Hamiltonian with couplings extended up to fourth-nearest neighbors, if the relations J1{\mathit{J}}_{1}J1​-2J2{\mathit{J}}_{2}J2​+J3{\mathit{J}}_{3}J3​=0 and J3{\mathit{J}}_{3}J3​=2J4{\mathit{J}}_{4}J4​ hold. Furthermore, it is proved to all orders in perturbation theory that this state is the ground state of this Hamiltonian in a finite interval of values of the parameter \ensuremath{\lambda}==1/2-j2{\mathit{j}}_{2}j2​ around \ensuremath{\lambda}=0. The actual extension of this interval is computed numerically for finite chains and is shown to be significant.
We have studied the low-energy excitation spectrum of a dimerized and frustrated antiferromagnetic Heisenberg chain. We use an analytic approach, based on a description of the excitations as triplets above a strong-coupling singlet ground state. The quasiparticle spectrum is calculated by treating the excitations as a dilute Bose gas with infinite on-site repulsion. Additional singlet (S=0)(S=0)(S=0) and triplet (S=1)(S=1)(S=1) modes are found as two-particle bound states of the elementary triplets. We have also calculated the contributions of the elementary and collective excitations into the spin structure factor. Our results are in excellent agreement with exact diagonalizations and dimer series expansions data as long as the dimerization parameter \ensuremath{\delta} is not too small $(\ensuremath{\delta}>0.1),$ i.e., while the elementary triplets can be treated as localized objects.
Ground-state phase diagram and low-lying excitation spectrum of the one-dimensional S =1 anisotropic Heisenberg antiferromagnetic chain with nearest neighbor and next nearest neighbor interactions are studied by means of an approximate mapping of the original S =1 spin Hamiltonian to the effective fermion Hamiltonian, which describes the dynamics of spin zero defects in antiferromagnetic environments (domain walls in the Néel state). We find that the frustration due to the next nearest neighbor interactions works cooperatively with quantum fluctuation in the Haldane state and stabilizes it. This is naturally explained in terms of the spin zero defect. In addition, we discuss characteristic features of the excitation spectrum in connection with its ground-state properties.
The phase diagram of a frustrated S=1/2 antiferromagnetic spin ladder with additional next-nearest neighbor exchanges, both diagonal and inchain, is studied by a weak-coupling effective field theory approach combined with exact diagonalization for finite systems. In addition to two known phases with rung-singlet and Haldane-type ground states, we observe two new phases with dimerization along the chains. Furthermore, the transitions between the different phases are studied and shown to be either first order or to belong to the universality class of the two-dimensional Ising model. The nature of elementary excitations is discussed briefly.