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Physical Review A

Resonant cascaded down-conversion

Christian Weedbrook, Ben Perrett, Karen V. Kheruntsyan, P. D. Drummond, Raphael C. Pooser, Olivier Pfister

Published Mar 20, 2012• 4 citations
Publisher

Abstract

We analyze an optical parametric oscillator (OPO) in which cascaded down-conversion occurs inside a cavity resonant for all modes but the initial pump. Due to the resonant cascade design, the OPO presents two ${\ensuremath{\chi}}^{(2)}$-level oscillation thresholds that are therefore much lower than for a ${\ensuremath{\chi}}^{(3)}$ OPO. This is promising for reaching the regime of an effective third-order nonlinearity well above both thresholds. Such a ${\ensuremath{\chi}}^{(2)}$ cascaded device also has potential applications in frequency conversion to far-infrared regimes. But, most importantly, it can generate novel multipartite quantum correlations in the output radiation, which represent a step beyond squeezed or entangled light. The output can be highly non-Gaussian and therefore not describable by any semiclassical model. In this paper, we derive quantum stochastic equations in the positive-$P$ representation and undertake an analysis of steady-state and dynamical properties of this system.

DOI
10.1103/physreva.85.033821

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We analyze an optical parametric oscillator (OPO) in which cascaded down-conversion occurs inside a cavity resonant for all modes but the initial pump. Due to the resonant cascade design, the OPO presents two \ensuremathχ(2){\ensuremath{\chi}}^{(2)}\ensuremathχ(2)-level oscillation thresholds that are therefore much lower than for a \ensuremathχ(3){\ensuremath{\chi}}^{(3)}\ensuremathχ(3) OPO. This is promising for reaching the regime of an effective third-order nonlinearity well above both thresholds. Such a \ensuremathχ(2){\ensuremath{\chi}}^{(2)}\ensuremathχ(2) cascaded device also has potential applications in frequency conversion to far-infrared regimes. But, most importantly, it can generate novel multipartite quantum correlations in the output radiation, which represent a step beyond squeezed or entangled light. The output can be highly non-Gaussian and therefore not describable by any semiclassical model. In this paper, we derive quantum stochastic equations in the positive-PPP representation and undertake an analysis of steady-state and dynamical properties of this system.
We analyze an optical parametric oscillator (OPO) in which cascaded down-conversion occurs inside a cavity resonant for all modes but the initial pump. Due to the resonant cascade design, the OPO present two χ^2 level oscillation thresholds that are therefore remarkably lower than for a χ^3 OPO. This is promising for reaching the regime of an effective third-order nonlinearity well above both thresholds. Such a χ^2 cascaded device also has potential applications in frequency conversion to far infra-red regimes. But, most importantly, it can generate novel multi-partite quantum correlations in the output radiation, which represent a step beyond squeezed or entangled light. The output can be highly non-Gaussian, and therefore not describable by any semi-classical model.
We propose and analyze a cascaded optical parametric system which involves three interacting modes across two octaves of frequency difference. Our system, combining degenerate optical parametric oscillation (OPO) with second harmonic generation (SHG), promises to be a useful source of squeezed and entangled light at three differing frequencies. We show how changes in damping rates and the ratio of the two concurrent nonlinearities affect the quantum correlations in the output fields. We analyze the threshold behavior, showing how the normal OPO threshold is changed by the addition of the SHG interactions. We also find that the inclusion of the OPO interaction removes the self-pulsing behavior found in normal SHG. Finally, we show how the Einstein-Podolsky-Rosen correlations can be controlled by the injection of a coherent seed field at the lower frequency.
We investigate production of three-photon states in cascaded parametric down-conversion (PDC). The analysis includes preparation of Greenberger-Horne-Zeilinger polarization-entangled states in cascaded type-II and type-I PDC in the framework of considering the dual-grid structure that involves two periodically poled crystals. Considering cascaded optical parametric oscillator (OPO) driven by a sequence of laser pulses with Gaussian time-dependent envelopes, we investigate quantum statistical properties of high intensity mode generated in intracavity three-photon splitting. Calculating the normalized third-order correlation function below-and at the generation threshold, we demonstrate that in the pulsed regime, depending on the duration of pulses and the time-interval separations between them, the degree of three-photon-number correlation essentially exceed the analogous one for the case of continuous pumping.
The quantum features of ultrashort-pulse optical parametric oscillators (OPOs) are investigated theoretically in the nonlinear regime near and above threshold. Viewing the pulsed OPO as a multimode open quantum system, we rigorously derive a general input-output model that features nonlinear coupling among many cavity (i.e., system) signal modes and a broadband single-pass (i.e., reservoir) pump field. Under appropriate assumptions, our model produces a Lindblad master equation with multimode nonlinear Lindblad operators describing two-photon dissipation and a multimode four-wave-mixing Hamiltonian describing a broadband, dispersive optical cascade, which we show is required to preserve causality. To simplify the multimode complexity of the model, we employ a supermode decomposition to perform numerical simulations in the regime where the pulsed supermodes experience strong single-photon nonlinearity. We find that the quantum nonlinear dynamics induces pump depletion as well as corrections to the below-threshold squeezing spectrum predicted by linearized models. We also observe the formation of non-Gaussian states with Wigner-function negativity and show that the multimode interactions with the pump, both dissipative and dispersive, can act as effective decoherence channels. Finally, we briefly discuss some experimental considerations for potentially observing such quantum nonlinear phenomena with ultrashort-pulse OPOs on nonlinear nanophotonic platforms.
Abstract Photon pairs and heralded single photons, obtained from cavity-assisted parametric down conversion (PDC), play an important role in quantum communications and technology. This motivated a thorough study of the spectral and temporal properties of parametric light, both above the optical parametric oscillator (OPO) threshold, where the semiclassical approach is justified, and deeply below it, where the linear cavity approximation is applicable. The pursuit of a higher two-photon emission rate leads into an interesting intermediate regime, between above OPO threshold and very low pump power, where the OPO still operates considerably below the threshold but the nonlinear cavity phenomena cannot be neglected anymore. Here, we investigate this intermediate regime and show that the spectral and temporal properties of the photon pairs, as well as their emission rate, may significantly differ from the widely accepted linear model. The observed phenomena include frequency pulling and broadening in the temporal correlation for the down-converted optical fields. These factors need to be taken into account when devising practical applications of the high-rate cavity-assisted spontaneous PDC sources.
The process of cascaded down-conversion and sum-frequency generation inside an optical cavity has been predicted to be a potential source of three-mode continuous-variable entanglement. When the cavity is pumped by two fields, the threshold properties have been analyzed, showing that these are more complicated than in well-known processes such as optical parametric oscillation. When there is only a single pumping field, the entanglement properties have been calculated using a linearized fluctuation analysis, but without any consideration of the threshold properties or critical operating points of the system. In this work we extend this analysis to demonstrate that the singly pumped system demonstrates a rich range of threshold behavior when quantization of the pump field is taken into account and that asymmetric polychromatic entanglement is available over a wide range of operational parameters.