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arXiv:1811.10583 · Physical Review A

Nonlinear quantum behavior of ultrashort-pulse optical parametric oscillators

Tatsuhiro Onodera, Edwin Ng, Chris Gustin, Niels Lörch, Atsushi Yamamura, Ryan Hamerly, Peter L. McMahon, Alireza Marandi, Hideo Mabuchi

Published Mar 11, 2022• 12 citations
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Abstract

The quantum features of ultrashort-pulse optical parametric oscillators (OPOs) are investigated theoretically in the nonlinear regime near and above threshold. Viewing the pulsed OPO as a multimode open quantum system, we rigorously derive a general input-output model that features nonlinear coupling among many cavity (i.e., system) signal modes and a broadband single-pass (i.e., reservoir) pump field. Under appropriate assumptions, our model produces a Lindblad master equation with multimode nonlinear Lindblad operators describing two-photon dissipation and a multimode four-wave-mixing Hamiltonian describing a broadband, dispersive optical cascade, which we show is required to preserve causality. To simplify the multimode complexity of the model, we employ a supermode decomposition to perform numerical simulations in the regime where the pulsed supermodes experience strong single-photon nonlinearity. We find that the quantum nonlinear dynamics induces pump depletion as well as corrections to the below-threshold squeezing spectrum predicted by linearized models. We also observe the formation of non-Gaussian states with Wigner-function negativity and show that the multimode interactions with the pump, both dissipative and dispersive, can act as effective decoherence channels. Finally, we briefly discuss some experimental considerations for potentially observing such quantum nonlinear phenomena with ultrashort-pulse OPOs on nonlinear nanophotonic platforms.

DOI
10.1103/physreva.105.033508

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The quantum features of ultrashort-pulse optical parametric oscillators (OPOs) are investigated theoretically in the nonlinear regime near and above threshold. Viewing the pulsed OPO as a multimode open quantum system, we rigorously derive a general input-output model that features nonlinear coupling among many cavity (i.e., system) signal modes and a broadband single-pass (i.e., reservoir) pump field. Under appropriate assumptions, our model produces a Lindblad master equation with multimode nonlinear Lindblad operators describing two-photon dissipation and a multimode four-wave-mixing Hamiltonian describing a broadband, dispersive optical cascade, which we show is required to preserve causality. To simplify the multimode complexity of the model, we employ a supermode decomposition to perform numerical simulations in the regime where the pulsed supermodes experience strong single-photon nonlinearity. We find that the quantum nonlinear dynamics induces pump depletion as well as corrections to the below-threshold squeezing spectrum predicted by linearized models. We also observe the formation of non-Gaussian states with Wigner-function negativity and show that the multimode interactions with the pump, both dissipative and dispersive, can act as effective decoherence channels. Finally, we briefly discuss some experimental considerations for potentially observing such quantum nonlinear phenomena with ultrashort-pulse OPOs on nonlinear nanophotonic platforms.
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The theoretical description of broadband, multimode quantum pulses undergoing a second-order χ(2)χ^{(2)}χ(2)-nonlinear interaction can be quite intricate, due to the large dimensionality of the underlying phase space. However, in many cases only a few broadband (temporal) modes are relevant before and after the nonlinear interaction. Here we present an efficient framework to calculate the relation between the quantum states at the input and output of a nonlinear element in their respective relevant modes. Since the number of relevant input and output modes may differ, resulting in an open quantum system, we introduce the generalized Bloch-Messiah decomposition (GBMD), reducing the description to an equal number of input and output modes. The GBMD enables us to calculate the multimode Wigner function of the output state by convolving the rescaled Wigner function of the reduced input quantum pulse with a multivariate Gaussian phase-space function. We expand on this result by considering two examples input states: A Fock state in a single broadband mode and a two-mode squeezed vacuum, both in the THz-frequency regime, up-converted to a single output broadband mode of optical frequencies. We investigate the effect, the convolution and thermalization due to entanglement breakage have on the output Wigner function by calculating the von Neumann entropy of the output Wigner function. The methods presented here can be used to optimize the amplification or frequency conversion of broadband quantum states, opening an avenue to the generation and characterization of optical quantum states on ultrafast time scales.
Multimode nonclassical states of light are an essential resource in quantum computation with continuous variables [1]. They can be generated either by mixing different squeezed light sources using linear optical operations [2], or directly in a multimode optical device [3, 4]. Synchronously Pumped Optical Parametric Oscillators (SPOPO) — which correspond to an OPO pumped by a train of ultrashort pulses that are synchronized with the cavity round-trip time — have been theoretically shown to be promising devices for the generation of multimode nonclassical frequency combs, since a SPOPO is a sole optical cavity acting as an assembly of independent squeezers in a particular basis called the supermodes basis [5]. The supermodes are optical frequency combs with specific spectrum and phase profiles that are determined by the length of the intracavity nonlinear crystal and the pulse shape of the pump.
We study the emergence of non-Gaussian quantum features in pulsed squeezed light generation with a mesoscopic number (i.e., dozens to hundreds) of pump photons. Due to the strong optical nonlinearities necessarily involved in this regime, squeezing occurs alongside significant pump depletion, compromising the predictions made by conventional semiclassical models for squeezing. Furthermore, nonlinear interactions among multiple frequency modes render the system dynamics exponentially intractable in naïve quantum models, requiring a more sophisticated modeling framework. To this end, we construct a nonlinear Gaussian approximation to the squeezing dynamics, defining a “Gaussian interaction frame” in which non-Gaussian quantum dynamics can be isolated and concisely described using a few dominant (i.e., principal) supermodes. Numerical simulations of our model reveal non-Gaussian distortions of squeezing in the mesoscopic regime, largely associated with signal-pump entanglement. We argue that state of the art in nonlinear nanophotonics is quickly approaching this regime, providing an all-optical platform for experimental studies of the semiclassical-to-quantum transition in a rich paradigm of coherent, multimode nonlinear dynamics. Mesoscopic pulsed squeezing, thus, provides an intriguing case study of the rapid rise in dynamic complexity associated with semiclassical-to-quantum crossover, which we view as a correlate of the emergence of new information processing capacities in the quantum regime.
We introduce two approaches to modeling the quantum dynamics of optical χ(3)χ^{(3)}χ(3) solitons. Taking an open-system viewpoint, we project the underlying quantum field into system (soliton) and residual reservoir components. The reservoir is treated as either (i) a discrete ``Lanczos supermode'' (LSM) expansion which localizes dynamics to a few-supermode basis, or (ii) a non-local environment which can be traced out by deriving a Markovian master equation (ME). Using these methods, we analyze and identify the quantum structure of both the soliton's stability and its hierarchy of perturbations. Through numerical simulations, we confirm both methods effectively capture quantum-induced soliton phase shifts in a concise few-mode (single-mode for ME) basis, and the LSM approach also captures photon loss which arises from non-Markovian dispersive couplings. As neither method is limited to the linearized regime, our approaches provide powerful computational tools to analyze complex non-Gaussian quantum dynamics of solitons where other commonly-used methods fail, providing insight into such non-perturbative regimes. We also investigate radiation that occurs in the presence of higher-order dispersion with ultrashort pulses, deriving a ME that predicts photon loss consistent with classical theory, but find that both classical and ME theory dramatically underestimate the actual amount of dissipation, which we explain in terms of dispersive coupling-induced soliton broadening.
Abstract Parametric down-conversion in a nonlinear crystal is a widely employed technique for generating quadrature squeezed light with multiple modes, which finds applications in quantum metrology, quantum information and communication. Here we study the generation of temporally multimode femtosecond pulsed squeezed light in a synchronously pumped optical parametric oscillator (SPOPO) operating below the oscillation threshold, while considering the presence of non-compensated intracavity group-velocity dispersion. Based on the developed time-domain model of the system, we show that the dispersion results in mode-dependent detuning of the broadband supermodes of the pulsed parametric process from the cavity resonance due to temporal Gouy phase, as well as linear coupling between these supermodes. With perturbation theory up to the second order in the coupling coefficients between modes, we obtained a solution for the amplitudes of multiple supermodes given an arbitrary sub-threshold pump level. The dispersion affects the quantum state of the supermodes by influencing their squeezing level and the rotation of the squeezing ellipse. It also affects the entanglement among the supermodes, leading to reduced suppression of shot noise level as measured in the balanced homodyne detection scheme. Furthermore, our study highlights the potential of SPOPO with group-velocity dispersion as a testbench for experimental investigations of multimode effects in linearly evanescent coupled parametric oscillators.