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Journal of Physics A Mathematical and General

Steady propagation of a coherent light pulse in a dielectric medium. II. The effect of spatial dispersion

Kensuke S. Ikeda, O. Akimoto

Published Jul 1, 1979• 16 citations

Abstract

For pt.I see ibid., vol.10, p.425 (1977). The effect of spatial dispersion or exciton formation on the steady propagation of a coherent light pulse in a dielectric medium is studied. The optical Bloch equation for a lattice of atomic dipoles coupled to one another by an exchange-type interaction is solved simultaneously with the Maxwell equation by the method of power-series expansion developed in the preceding paper. Two kinds of pulse solutions are obtained in general: one propagating by the medium of the radiation field and the other by excitation transfer between atomic dipoles. The former solution is SIT-like in the short pulse limit, but a polariton-soliton or a standing wave of non-linear polariton if the pulse width is long. The latter is an exciton-soliton containing little photon component. When the pulse width is extremely long, there appears a polariton-soliton of a new type in which the two propagation mechanisms are mixed. It is found that the spatial dispersion prevents the polariton-soliton solutions from existing in a certain frequency range. This effect is explained on the basis of the functional behavior of the dispersion relation of the non-linear polariton.

DOI: 10.1088/0305-4470/12/7/027

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For pt.I see ibid., vol.10, p.425 (1977). The effect of spatial dispersion or exciton formation on the steady propagation of a coherent light pulse in a dielectric medium is studied. The optical Bloch equation for a lattice of atomic dipoles coupled to one another by an exchange-type interaction is solved simultaneously with the Maxwell equation by the method of power-series expansion developed in the preceding paper. Two kinds of pulse solutions are obtained in general: one propagating by the medium of the radiation field and the other by excitation transfer between atomic dipoles. The former solution is SIT-like in the short pulse limit, but a polariton-soliton or a standing wave of non-linear polariton if the pulse width is long. The latter is an exciton-soliton containing little photon component. When the pulse width is extremely long, there appears a polariton-soliton of a new type in which the two propagation mechanisms are mixed. It is found that the spatial dispersion prevents the polariton-soliton solutions from existing in a certain frequency range. This effect is explained on the basis of the functional behavior of the dispersion relation of the non-linear polariton.

The phenomenon of self-induced transparency (SIT) in the exciton range of the spectrum consists of the propagation through the crystal of solitary wave packets of coherent excitons and photons with anomalous small losses. In the running frame of reference at the site occupied by the soliton a single aperiodic transformation of photons into excitons and a reverse motion of the energy into the field takes place. The solutions of the SIT equations have been received in the slowly-varying amplitude approximation. Taking into account the phase modulation, the authors have shown the appearance of the branch of the carrier wave frequency with anomalous dispersion not only at the given pulse width but at the given pulse amplitude. They have also found the exact solution of the above mentioned equations taking into account the effect of saturation of the dipole momentum transition from the crystal ground state to the exciton state. It leads to the increasing of the soliton time width, to the decreasing of its amplitude and worsens the SIT observation.

We determine the dispersion law of the carrier wave of an exciton-photon pulse which propagates as a solitary wave. For short pulses, four branches $\ensuremath{\Omega}=\ensuremath{\Omega}$ ($\stackrel{\ensuremath{\rightarrow}}{\mathrm{K}}$) appear: a branch which goes through the intersection point $\ensuremath{\hbar}cK={E}_{o}+\frac{{\ensuremath{\hbar}}^{2}{K}^{2}}{2M}$ of the uncoupled modes of the free exciton and the free light field, two polaritonlike branches and an excitonlike branch. The polaritonlike branches have a normal dispersion, whereas the branch which goes through the intersection point of the free modes has an anomalous dispersion for sufficiently short pulse width. This branch contains the solution of McCall and Hahn as a special case. For very short pulses the branch with anomalous dispersion continues into the two polaritonlike branches. For increasing pulse width a forbidden energy gap appears at $\stackrel{\ensuremath{\rightarrow}}{\mathrm{K}}=0$. For long pulses, only the two polaritonlike solutions exist.

The present paper has the dual purposes. As the first purpose, it is demonstrated that the boson description of Wannier excitons introduced in the preceding paper is suitable also to discussion of non-linear coherent interaction of Wannier excitons with the radiation field. The second purpose is to discuss the possibility of self-induced transparency due to Wannier excitons on the basis of the boson description by making clear the difference between a two-level atomic system and a system of excitons which can propagate in a crystal as polariton. As a result, stable pulse propagation of the radiation field is shown to be prevented by the polariton effect of excitons.

The dynamics of pulses with durations comparable to the inverse transition frequency that propagate in an optical medium is studied in terms of two integrable systems of Maxwell-Bloch equations. The first model describes the field interaction with a nondegenerate medium with a permanent dipole moment and permanent external pumping. A general formula is derived for the N -soliton solution. Particular solutions are used as examples to investigate the effect of permanent dipole moment and pumping on the soliton dynamics. The second model describes the interaction between two-component electric-field pulses and a two-level degenerate medium with permanent upper-level pumping. For different initial magnetic-sublevel populations, soliton solutions are used as examples to show that pumping causes a change in polarization dynamics. A two-soliton solution is used to analyze the interaction of solitons in a two-level medium with external pumping.