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The European Physical Journal B

Regular reflection of pressure broadened resonance lines

Wolfgang Heering

Published Mar 1, 1975• 6 citations
Publisher
DOI
10.1007/bf01313914

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We report an observation of \ensuremath{\Delta}m=2 ground-state coherences in selective-reflection spectra at a glass--metal-vapor interface. The coherence was created by a linearly polarized laser beam tuned to a sub-Doppler resonance in the selective-reflection spectrum of the cesium D2{\mathit{D}}_{2}D2​ line and detected through the magnetorotation of the plane of polarization of the reflected beam. The coherence effect appears as a dispersive shaped resonance of subnatural width. The dependence of the width on the intensity of the optical field shows a saturation behavior. For vanishing light intensity and cesium vapor pressure the linewidth is limited by transverse time-of-flight broadening, whereas its pressure dependence indicates an additional contribution from the finite longitudinal interaction time.
Three-photon excitation and multiphoton ionization techniques have been used to measure self-broadening for several resonance lines in xenon and krypton. Tabulations of widths and shifts of the xenon lines at 146.9, 129.6, 119.2, and 117.0 nm were made for pressures between 50 and 900 Torr. Similar measurements were made for the krypton resonance line at 116.5 nm. For pressures less than 500 Torr the widths were found to be in reasonable agreement with theoretical results, which were extrapolated into regions of concentration where the criteria for their validity are at best questionable. We have also found the lines to be shifted to the high-energy side of the unperturbed line. For four of the five lines studied, the blue shifts increased nearly linearly with increasing pressure. In the four cases where the shift could be measured the ratio of shift to width was close to (1/2. Our experimental technique is very simple, but it has yielded what we believe to be the first resonance broadening data based on absorption under conditions where there is strong trapping of the resonance radiation.