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Journal of the Korean Physical Society

Quantum phase transitions in 1/3 plateau of the quantum spin tube

Kouichi Okunishi, Masahiro Sato, Tôru Sakai, Kiyomi Okamoto, Chigaku Itoi

Published Aug 1, 2013• 0 citations
Publisher

Abstract

We study quantum phase transitions in the 1/3 plateau state of the three-leg spin-1/2 tube, where the low-energy effective chirality degree of freedom plays an essential role. Using the density matrix renormalization group and the effective chirality model, we find that, as the leg coupling increases, the chirality liquid, a novel spin imbalance phase and the vector-spin-chirality ordered phase emerge without closing the plateau spin gap. We also clarify the role of the S 3-symmetry of the spin tube, behind these quantum phase transitions.

DOI
10.3938/jkps.63.596

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We study quantum phase transitions in the 1/3 plateau state of the three-leg spin-1/2 tube, where the low-energy effective chirality degree of freedom plays an essential role. Using the density matrix renormalization group and the effective chirality model, we find that, as the leg coupling increases, the chirality liquid, a novel spin imbalance phase and the vector-spin-chirality ordered phase emerge without closing the plateau spin gap. We also clarify the role of the S 3-symmetry of the spin tube, behind these quantum phase transitions.
We study the magnetization plateau state of the three-leg spin-12\frac{1}{2}21​ tube in the strong rung coupling region, where S3{S}_{3}S3​ symmetry breaking and the low-energy chirality degree of freedom play crucial roles. On the basis of the effective chirality model and density matrix renormalization group, we clarify that, as the leg coupling increases, the chirality liquid with gapless nonmagnetic excitations, the spin-imbalance phase, and the vector-spin-chirality ordered phase emerge without closing the plateau spin gap. The relevance of these results to experiments is also discussed.
We investigate the S = 1/2 three-leg spin tube, which is the simplest spin nanotube, using the density matrix renormalization group (DMRG) and the numerical exact diagonalization (ED), conbined with a finite-size scaling analysis. Particularly, we intruduce the lattice distortion from the regular triangle unit to the isosceles one. In our previous works, we revealed that the S = 1/2 isosceles triangle spin tube exhibits following exotic quantum phenomena: the quantum phase transition between the spin gapped and gapless spin liquid phases, the 1/3 magnetization plateau due to two different mechanisms, and a new phase between the two plateau phases where the translational symmetry is spontaneously broken. We briefly review these results and show our new calculation of the expectation value of the magnetization at each site to specify the spin structure in the new field induced phase.
We investigate the properties of a three-leg quantum spin tube using several techniques such as the density-matrix renormalization-group (DMRG) method, strong-coupling approaches and the nonlinear sigma model. For integer SSS, the model proves to exhibit a particularly rich phase diagram consisting of an ensemble of 2S2S2S phase transitions. They can be accurately identified by the behavior of a nonlocal string order parameter associated to the breaking of a hidden symmetry in the Hamiltonian. The nature of these transitions is further elucidated within the different approaches. We carry a detailed DMRG analysis in the specific cases S=1S=1S=1. The numerical data confirm the existence of two Haldane phases with broken hidden symmetry separated by a trivial singlet state. The study of the gap and of the von Neumann entropy suggest a first-order phase transition but at the close proximity of a tricritical point separating a gapless and a first-order transition line in the phase diagram of the quantum spin tube.
Motivated by the recent discovery of the spin tube [(CuCl2tachH)3Cl]Cl2[{(\mathrm{Cu}{\mathrm{Cl}}_{2}\mathrm{tach}\mathrm{H})}_{3}\mathrm{Cl}]{\mathrm{Cl}}_{2}[(CuCl2​tachH)3​Cl]Cl2​, we investigate the properties of a frustrated three-leg spin tube with antiferromagnetic intra- and inter-ring couplings. We pay special attention to the evolution of the properties from weak to strong inter-ring coupling and show on the basis of extensive density matrix renormalization group and exact diagonalization calculations that the system undergoes a first-order phase transition between a dimerized gapped phase at weak coupling that can be described by the usual spin-chirality model and a gapless critical phase at strong coupling that can be described by an effective spin-3∕23∕23∕2 model. We also show that there is a magnetization plateau at 1∕31∕31∕3 in the whole gapped phase and slightly beyond. The implications for [(CuCl2tachH)3Cl]Cl2[{(\mathrm{Cu}{\mathrm{Cl}}_{2}\mathrm{tach}\mathrm{H})}_{3}\mathrm{Cl}]{\mathrm{Cl}}_{2}[(CuCl2​tachH)3​Cl]Cl2​ are discussed, with the conclusion that this system behaves essentially as a spin-3∕23∕23∕2 chain.
Recent developments of theoretical studies on spin nanotubes are reviewed, especially focusing on the S = 1/2 three-leg spin tube. In contrast to the three-leg spin ladder, the tube has a spin gap in the case of the regular-triangle unit cell when the rung interaction is sufficiently large. The effective theory based on the Hubbard Hamiltonian indicates a quantum phase transition to a gapless spin liquid due to the lattice distortion to an isosceles triangle. This is also supported by the numerical diagonalization and the density matrix renormalization group analyses. Furthermore, combining analytical and numerical approaches, we reveal several novel magnetic-field-induced phenomena: Néel, dimer, chiral and/or inhomogeneous orders, a new mechanism for the magnetization plateau formation, and others. The recently synthesized spin tube materials are also briefly introduced.
Recently some quantum spin systems on tube lattices, so called spin nanotubes, have been synthesized. They are expected to be interesting low-dimensional systems like the carbon nanotubes. As the first step of theoretical study on the spin nanotube, we investigate the S=1/2 three-leg spin tube, which is the simplest one, using the numerical exact diagonalization and the finite-size scaling analysis. In our previous works the quantum phase transition between the spin-gap and gapless phases was revealed to occur due to the asymmetric lattice distortion. In addition the transition between the magnetization plateau and gapless phases at 1/3 of the saturation magnetization induced by the same distortion. Recently we found that the Tomonaga-Luttinger liquid is realized in the 1/3 magnetization plateau phase for the symmetric three-leg spin tube.