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Optics Communications

Stimulated collision-induced fluorescence and stimulated Raman scattering in barium vapor pumped by XeCl laser radiation

Yunsheng Huo, Qihong Lou

Published Aug 1, 1988• 2 citations
Publisher
DOI
10.1016/0030-4018(88)90031-4

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The stimulated collision-induced fluorescence (SOF) at wavelengths of 472.6nm, 582.6nm and 648.3nm, as well as Raman-shifted radiation at wavelength of 475nm were observed in barium vapor pumped by broadband pulse of the XeOl laser. The SCF was found to be self-termination short pulses with FWHM of 8 ns, and its internsity inoreased with buffer-gas pressure. There existed time delay aa long as 20 ns between the front edges of the pump pulse and of the Raman-shifted pulse, and the Raman conversion efficiency decreased significantly as the buffer-gas pressure increasing.
An experimental investigation was made of stimulated Raman scattering (STRS) of excimer laser radiation in barium, thulium, and europium vapors. The energy of XeF* laser radiation ( λ = 351 nm) converted to the yellow range (585 nm) in barium vapor was 6 mJ and the conversion efficiency was ∼39%. The spectral composition of the converted radiation is governed by the STRS, by four-wave parametric processes, and also by lasing due to the natural barium transition. Selection of the pump frequencies is required to concentrate the converted radiation at a single frequency and to reduce its divergence. Stimulated Raman scattering of XeCl* laser radiation ( λ = 308 nm) was achieved in thulium vapor at λ = 422 nm. In europium vapor in quasiresonance with the 6 s 2 8 S 0 1/2 –5 d 2 10 P 0 11/2 forbidden transition, stimulated emission was obtained due to the natural 5 d 2 10 P 0 11/2 –6 s 6 p 10 P 11/2 and 5 d 2 10 P 0 11/2 –6 s 6 p 10 P 3/2 transitions.