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Ferroelectrics

Optical Bistability from Ferroelectric Fabry-Perot Interferometer

Abdel-Baset M.A. Ibrahim, David Reginald Tilley, Junaidah Osman

Published Sep 4, 2007• 7 citations
Publisher

Abstract

We study the nonlinear optical bistability and multistability of a nonlinear ferroelectric (FE) Fabry-Perot (FP) interferometer assumed coated with partial dielectric mirrors on its interfaces. The FE material is considered to have an intensity-dependent refractive index where the third order nonlinear susceptibility χ ilmn (3) acts like Kerr coefficient. The nonlinear response of the FE medium is modeled by the Landau-Khalatnikov (LK) dynamical equation. Within a single frequency approximation, the nonlinear wave equation is written in terms of polarization P rather than the electric field E as the dependent variable. The resulting nonlinear polarization equation is numerically integrated across the FP film using the fourth order Runge-Kutta method. The behavior of the resulting polarization and transmission as a function of the field input intensity is investigated.

DOI
10.1080/00150190701517598

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We study the nonlinear optical bistability and multistability of a nonlinear ferroelectric (FE) Fabry-Perot (FP) interferometer assumed coated with partial dielectric mirrors on its interfaces. The FE material is considered to have an intensity-dependent refractive index where the third order nonlinear susceptibility χ ilmn (3) acts like Kerr coefficient. The nonlinear response of the FE medium is modeled by the Landau-Khalatnikov (LK) dynamical equation. Within a single frequency approximation, the nonlinear wave equation is written in terms of polarization P rather than the electric field E as the dependent variable. The resulting nonlinear polarization equation is numerically integrated across the FP film using the fourth order Runge-Kutta method. The behavior of the resulting polarization and transmission as a function of the field input intensity is investigated.
Ferroelectric oxides with perovskite structure such as PbLaTiO3 (PLT), BaTiO3, PbTiO3, SrBi2Ta2O9 and LiNbO3 are very attractive class of materials which possess numerous useful properties such as high dielectric constant, large spontaneous polarization, and remarkable optical nonlinearity. Potential applications of these materials include real-time holography, correlation filtering and various novelty filter applications (Sutherland 1996 and Eaton 1991). They are also popular materials for the fabrication of nonvolatile memories (Ramesh 2001). Over the past few years, ferroelectric oxides have been widely investigated for various nonlinear optical applications (Shi 2006; Xuan 1998; Zhang 1999; Zhao 1996) especially for optical switches. Optical switches are devices invented to perform multiplexing at very fast speeds and with less delay than the customary switches works with electronic signals. A ferroelectric optical switch is expected to allow the processing of millions of signals at a speed of terahertz. To obtain optical bistability phenomenon, two ingredients are necessary, a nonlinear process and a feedback mechanism (Gibbs, 1977, 1979, and 1985). In all optical systems, the feedback can be “distributed”, “extrinsic” or “intrinsic”. In multilayer systems with alternating nonlinear materials, the feedback is “distributed”; it arises from the interaction of the propagating wave with many cross-sections of a nonlinear medium. In a Fabry-Perot (FP) resonator, the feedback is “extrinsic”; it arises as a result of reflection from the mirrors placed at its interface. In a single nonlinear layer, the feedback can be “intrinsic” or “mirrorless”; it arises in each elementary oscillator due to the strong local nonlinear response of an individual atom or molecule. In the usual or the standard analysis to study the optical bistability (Marburger 1978, Gupta 1987, Biran 1990, Danckaert 1989, Shen 1984, and Haelterman 1989) in nonlinear optics, the governing equation for optical propagation within the nonlinear medium is a nonlinear wave equation in the electric field derived from Maxwell’s equations. The usual constitutive relation between the nonlinear polarization and the electric field is then obtained by expanding the nonlinear polarization as a Taylor series in the electric field. The usefulness of this constitutive relation is that the polarization is a natural source term in the Maxwell’s
We present a model calculation of optical bistability and polarisation evolution in optically birefringent media based on the interaction of three waves.Second-order optical nonlinearity (described by the third rank susceptibility tensor) is assumed to be dominant.A bistable light transmission is analysed in terms of standard Fabry-Perot model of feedback, and is a direct consequence of the results obtained for a semi-infinite medium.A second effect considered in the paper is evolution of polarisation state of the waves involved in these processes.We derived a closed formula for intensity-dependent refractive index, which corresponds to that used in the case of third-order nonlinear media.As a result, we calculated both intensity • and Stokes parameters of transmitted light.
A nonlinear thin film bounded by two dielectric media could act as an optical switching and bistability device, owing to two physical mechanisms at work near the total internal reflection state. One is the simple intensity-dependent index change induced by the finite optical field in the film before transmission occurs, and the other is the nonlinear Fabry-Perot interference associated with the high reflectivities at the two interfaces when transmission takes place. We present a detailed theory for these two mechanisms and for the case in which the nonlinearity is also nonlocal (e.g., in a liquid-crystal film). The results for multiple switchings and hysteresis hold in general for any nonlinear thin film.