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Ferroelectric Optics: Optical Bistability in Nonlinear Kerr Ferroelectric Materials

Abdel-Baset M.A. Ibrahim, Mohd Kamil Abd Rahman, Junaidah Osm

Published Dec 14, 2010• 1 citation
Publisher

Abstract

Ferroelectric oxides with perovskite structure such as PbLaTiO3 (PLT), BaTiO3, PbTiO3, SrBi2Ta2O9 and LiNbO3 are very attractive class of materials which possess numerous useful properties such as high dielectric constant, large spontaneous polarization, and remarkable optical nonlinearity. Potential applications of these materials include real-time holography, correlation filtering and various novelty filter applications (Sutherland 1996 and Eaton 1991). They are also popular materials for the fabrication of nonvolatile memories (Ramesh 2001). Over the past few years, ferroelectric oxides have been widely investigated for various nonlinear optical applications (Shi 2006; Xuan 1998; Zhang 1999; Zhao 1996) especially for optical switches. Optical switches are devices invented to perform multiplexing at very fast speeds and with less delay than the customary switches works with electronic signals. A ferroelectric optical switch is expected to allow the processing of millions of signals at a speed of terahertz. To obtain optical bistability phenomenon, two ingredients are necessary, a nonlinear process and a feedback mechanism (Gibbs, 1977, 1979, and 1985). In all optical systems, the feedback can be “distributed”, “extrinsic” or “intrinsic”. In multilayer systems with alternating nonlinear materials, the feedback is “distributed”; it arises from the interaction of the propagating wave with many cross-sections of a nonlinear medium. In a Fabry-Perot (FP) resonator, the feedback is “extrinsic”; it arises as a result of reflection from the mirrors placed at its interface. In a single nonlinear layer, the feedback can be “intrinsic” or “mirrorless”; it arises in each elementary oscillator due to the strong local nonlinear response of an individual atom or molecule. In the usual or the standard analysis to study the optical bistability (Marburger 1978, Gupta 1987, Biran 1990, Danckaert 1989, Shen 1984, and Haelterman 1989) in nonlinear optics, the governing equation for optical propagation within the nonlinear medium is a nonlinear wave equation in the electric field derived from Maxwell’s equations. The usual constitutive relation between the nonlinear polarization and the electric field is then obtained by expanding the nonlinear polarization as a Taylor series in the electric field. The usefulness of this constitutive relation is that the polarization is a natural source term in the Maxwell’s

DOI
10.5772/13083

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In this complement we discuss several examples of optical phenomena in media where the refractive index depends nonlinearly on the intensity , known as optical Kerr media. This nonlinear effect exists in all materials, even isotropic ones, like glass or fused silica, but it is particularly marked in certain physical systems to be exemplified in Section 7B.1. After investigating the propagation of light through such media in Section 7B.2, we shall discuss three applications of the optical Kerr effect (which can be studied in any order). We begin by describing a bistable optical system , when this nonlinear medium is inserted in a Fabry–Perot cavity (Section 7B.3). We then study phase conjugate mirrors and examine their potential applications in adaptive optics (Section 7B.4). Finally, we discuss certain effects occurring during the propagation of an isolated wave, bounded either transversely or temporally, in a Kerr medium, and describe self-focusing effects (Section 7B.5) and self-phase-modulation effects (Section 7B.6). In particular, we shall show that nonlinear effects and dispersion effects can compensate to produce stable structures known as solitons , which maintain their shape during propagation. Examples of third-order nonlinearities Nonlinear response of two-level atoms We begin by studying a simple case of a nonlinear interaction, namely a two-level quantum system under the effects of a plane wave.

Cambridge University Press eBooks•Sep 2, 2010•0 citations
Ferroelectric oxides with perovskite structure such as PbLaTiO3 (PLT), BaTiO3, PbTiO3, SrBi2Ta2O9 and LiNbO3 are very attractive class of materials which possess numerous useful properties such as high dielectric constant, large spontaneous polarization, and remarkable optical nonlinearity. Potential applications of these materials include real-time holography, correlation filtering and various novelty filter applications (Sutherland 1996 and Eaton 1991). They are also popular materials for the fabrication of nonvolatile memories (Ramesh 2001). Over the past few years, ferroelectric oxides have been widely investigated for various nonlinear optical applications (Shi 2006; Xuan 1998; Zhang 1999; Zhao 1996) especially for optical switches. Optical switches are devices invented to perform multiplexing at very fast speeds and with less delay than the customary switches works with electronic signals. A ferroelectric optical switch is expected to allow the processing of millions of signals at a speed of terahertz. To obtain optical bistability phenomenon, two ingredients are necessary, a nonlinear process and a feedback mechanism (Gibbs, 1977, 1979, and 1985). In all optical systems, the feedback can be “distributed”, “extrinsic” or “intrinsic”. In multilayer systems with alternating nonlinear materials, the feedback is “distributed”; it arises from the interaction of the propagating wave with many cross-sections of a nonlinear medium. In a Fabry-Perot (FP) resonator, the feedback is “extrinsic”; it arises as a result of reflection from the mirrors placed at its interface. In a single nonlinear layer, the feedback can be “intrinsic” or “mirrorless”; it arises in each elementary oscillator due to the strong local nonlinear response of an individual atom or molecule. In the usual or the standard analysis to study the optical bistability (Marburger 1978, Gupta 1987, Biran 1990, Danckaert 1989, Shen 1984, and Haelterman 1989) in nonlinear optics, the governing equation for optical propagation within the nonlinear medium is a nonlinear wave equation in the electric field derived from Maxwell’s equations. The usual constitutive relation between the nonlinear polarization and the electric field is then obtained by expanding the nonlinear polarization as a Taylor series in the electric field. The usefulness of this constitutive relation is that the polarization is a natural source term in the Maxwell’s
We study the nonlinear optical bistability and multistability of a nonlinear ferroelectric (FE) Fabry-Perot (FP) interferometer assumed coated with partial dielectric mirrors on its interfaces. The FE material is considered to have an intensity-dependent refractive index where the third order nonlinear susceptibility χ ilmn (3) acts like Kerr coefficient. The nonlinear response of the FE medium is modeled by the Landau-Khalatnikov (LK) dynamical equation. Within a single frequency approximation, the nonlinear wave equation is written in terms of polarization P rather than the electric field E as the dependent variable. The resulting nonlinear polarization equation is numerically integrated across the FP film using the fourth order Runge-Kutta method. The behavior of the resulting polarization and transmission as a function of the field input intensity is investigated.
In the last chapter, we examined the effect of cubic nonlinearity on selfrefraction of an optical beam. We have also seen that the presence of a quadratic nonlinearity can also contribute to change in the profile of a Gaussian beam in a crystal. In this chapter we will see how the effect of nonlinearity, alongwith the proper feedback, can give rise to optical bistability and hysteresis. This is not unexpected as hysteresis and bistability are also observed in nonlinear electronic circuits with feedback, such as in the Schmitt trigger, as well as in hybrid optical devices, such as an acoustooptic device with feedback (Banerjee and Poon, 1991). In what follows, we will examine two different types of optically bistable devices based on optical nonlinearities. The first is a nonlinear ring resonator comprising a two-level gain medium as the nonlinear element. We will treat both absorptive and dispersive bistability. Absorptive bistability is the case when the incident optical frequency is close to or equal to the transition frequency of the atoms from one level to another. In this case, the absorption coefficient becomes a nonlinear function of the incident intensity. On the other hand, if the frequencies are far apart, the medium behaves like a Kerr-type material and the system exhibits what is called dispersive bistability. In this case the material can be modeled by an effective n2 or v (3), meaning that the refractive index becomes a nonlinear function of the optical intensity. The second configurationwewill examine is a linear-nonlinear interface. In this case, the interface provides the feedback due to refractive index mismatch. In fact, the reflection coefficient (as well as the transmission coefficient) is modified due to the nonlinearity, which, as we shall see later, is responsible for demonstrating optical switching and bistability.
The nonlinear phenomenon known as optical bistability, which enables optical systems to maintain two stable output states for a single input, is thoroughly examined in this review article. Through a detailed analysis of two important devices—the Simple Fiber Ring (SFR) resonator and the Nonlinear Optical Loop Mirror (NOLM)—it investigates the basic concepts of optical bistability, namely nonlinearity and feedback. Numerical simulations demonstrating dynamic dynamics and stability conditions bolster a strong theoretical framework. Recent advancements in bistable optical technologies, including developments in epsilon-near-zero materials, silicon photonics, hybrid plasmonic structures, neuromorphic photonics, and AI-driven photonic processors are also discussed. Furthermore, this review highlights emerging applications of optical bistability in optical logic circuits, high-speed communication, and quantum information processing. This review work is a useful tool for researchers and engineers creating next-generation optical systems because it connects theoretical insights with cutting-edge technological developments.
In this study, we investigate the optical bistability and multistability in a pure single Kerr nonlinear layer of dielectric material using the Maxwell-Duffing approach. We employ the Duffing anharmonic oscillator as an alternative constitutive relation to express the electric field as a nonlinear function of the induced polarization. Utilizing both the electromagnetic wave equation and the Duffing constitutive relation, we obtain a nonlinear polarization equation propagates through the nonlinear layer under the slowly varying envelope approximation. With the application of boundary conditions at both interfaces, expressions for the incident, reflected, and transmitted intensities of the light wave are obtained as nonlinear functions of the polarization and other controlling parameters. For realistic input parameters, our numerical results demonstrated the existence of an intrinsic optical bistability (IOB) in a pure single dielectric layer. Furthermore, the threshold value of the observed IOB depends essentially on the value Eth, i.e., the minimum value required to invoke the third-order nonlinearity inside the material. For operating frequency near the sharp resonance region, Eth was found to be ≈105 V/cm; this is equivalent to a threshold value of the optical intensity ≈1010 W/cm2. With the developments in THz sources, it is nowadays possible to observe this IOB experimentally by tuning the operating frequency near the sharp resonance region of the material. Steps to get the threshold value of Eth are also advised.
In this complement we discuss several examples of optical phenomena in media where the refractive index depends nonlinearly on the intensity , known as optical Kerr media. This nonlinear effect exists in all materials, even isotropic ones, like glass or fused silica, but it is particularly marked in certain physical systems to be exemplified in Section 7B.1. After investigating the propagation of light through such media in Section 7B.2, we shall discuss three applications of the optical Kerr effect (which can be studied in any order). We begin by describing a bistable optical system , when this nonlinear medium is inserted in a Fabry–Perot cavity (Section 7B.3). We then study phase conjugate mirrors and examine their potential applications in adaptive optics (Section 7B.4). Finally, we discuss certain effects occurring during the propagation of an isolated wave, bounded either transversely or temporally, in a Kerr medium, and describe self-focusing effects (Section 7B.5) and self-phase-modulation effects (Section 7B.6). In particular, we shall show that nonlinear effects and dispersion effects can compensate to produce stable structures known as solitons , which maintain their shape during propagation. Examples of third-order nonlinearities Nonlinear response of two-level atoms We begin by studying a simple case of a nonlinear interaction, namely a two-level quantum system under the effects of a plane wave.