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Physical Review A

Effects of Zeeman degeneracy on the steady-state properties of an atom interacting with a near-resonant laser field: Probe spectra

Bo Gao

Published May 1, 1994• 14 citations
Publisher

Abstract

The probe spectrum of a closed two-level Zeeman-degenerate atom interacting with a linearly polarized coherent laser field is studied. Results for the cycling transition of a cesium atom are presented and compared to the experimental data of Lounis et al. [Phys. Rev. Lett. 69, 3029 (1992)]. We further show that the resonance derived by Grynberg, Vallet, and Pinard [Phys. Rev. Lett. 65, 701 (1990)] is due to stimulated Raman scattering.

DOI
10.1103/physreva.49.3391

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Electromagnetically Induced Transparency in Λ-Type Zeeman Sublevels of Cesium Atoms

Tiancai Zhang

Employing two lasers as the coupling and probe fields which have opposite circular polarization (σ + and σ -), electromagnetically induced transparency (EIT) in Λ-type Zeeman sublevels of cesium 6 2S 1/2F=3-6 2P 3/2F′=2 degenerate two-level system has been demonstrated via probe absorption spectra. The effect of the intensity and detuning of different coupling. Laser on EII was also investigated in experiments. Within the Doppler background, optical pumping among Zeeman sub-levels and the population of different Zeeman sub-levels can dominate the intensity of EIT effect. And the physical reason of the rugged spectra are presented qualitatively.

Chinese Journal of Lasers•Jan 1, 2005•0 citations
The probe spectrum of a closed two-level Zeeman-degenerate atom interacting with a linearly polarized coherent laser field is studied. Results for the cycling transition of a cesium atom are presented and compared to the experimental data of Lounis et al. [Phys. Rev. Lett. 69, 3029 (1992)]. We further show that the resonance derived by Grynberg, Vallet, and Pinard [Phys. Rev. Lett. 65, 701 (1990)] is due to stimulated Raman scattering.
Effects of the atomic Zeeman degeneracy on the resonance fluorescence spectrum of a closed two-level atom with arbitrary ground-state angular momentum Jg{\mathit{J}}_{\mathit{g}}Jg​ and excited-state, angular momentum Je{\mathit{J}}_{\mathit{e}}Je​ are studied in detail. Especially interesting are the narrow structures due to the spontaneous Raman scattering and the incoherent Rayleigh scattering. Results for the cycling transition of a Cs atom are presented as part of the examples.
The analytic solution of the steady-state density matrix is presented for a closed two-level atom with an arbitrary ground-state angular momentum Jg{\mathit{J}}_{\mathit{g}}Jg​ and an excited-state angular momentum Je{\mathit{J}}_{\mathit{e}}Je​ interacting with a linearly polarized laser field. From this solution, analytic formulas for the total rate of laser-atom scattering, the rate of coherent scattering, and radiative forces are derived. Interestingly, it is found that population inversion in true atomic states, as opposed to the population inversion in the dressed states, can occur under certain conditions. A method is proposed to take advantage of this inversion for light amplification. The mathematical formulation is built around the concept of the resolvent operator in Liouville space, with some conclusions that are generally applicable to any system with a unique steady state.
Resonance fluorescence due to intense laser fields from a Zeeman degenerate atom being perturbed by collisional interactions is calculated in the impact regime by using the quantum-fluctuation-regression theorem. Various interesting effects are found. For example, the scattered intensity spectrum for a J=0J=0J=0 to J=1J=1J=1 transition for polarization parallel to the laser polarization is essentially an asymmetric triplet, whereas for a perpendicular polarization due to collisions the spectrum is essentially a doublet (whose frequencies do not correspond with any of those of the triplet). Further, the width of the fluorescent component (whose frequency is close to the unperturbed frequency) actually decreases with increasing laser power.
We study the pump and probe absorption spectra, as a function of the probe detuning, in a degenerate two-level atomic system, for the case where the probe intensity is high enough to affect the pump absorption. The theory is valid for any ${F}_{g}\ensuremath{\rightarrow}{F}_{e}$ alkali-metal transition interacting with an arbitrarily intense pump and probe (with general Rabi frequencies ${\ensuremath{\Omega}}_{1,2}$) which are perpendicularly polarized with either ${\ensuremath{\sigma}}_{\ifmmode\pm\else\textpm\fi{}}$ or $\ensuremath{\pi}$ polarization. We have constructed a computer program that can calculate the spectra without requiring one to write out the Bloch equations explicitly. We show that, when the pump is ${\ensuremath{\sigma}}_{\ifmmode\pm\else\textpm\fi{}}$ polarized and the probe $\ensuremath{\pi}$ polarized, or vice versa, the pump and probe absorptions depend on the Zeeman coherences between the nearest-neighboring ground or excited Zeeman sublevels, whereas when the pump is ${\ensuremath{\sigma}}_{+}$ polarized and the probe ${\ensuremath{\sigma}}_{\ensuremath{-}}$ polarized, or vice versa, the Zeeman coherences that directly determine the absorption are between next-nearest neighbors. We report calculations of the pump and probe absorption spectra for the cycling ${F}_{g}=2\ensuremath{\rightarrow}{F}_{e}=3$ transition in the D2{D}_{2}D2​ line of 87Rb^{87}\text{R}\text{b}87Rb, interacting with a resonant ${\ensuremath{\sigma}}_{+}$-polarized pump and either a $\ensuremath{\pi}$- or a ${\ensuremath{\sigma}}_{\ensuremath{-}}$- polarized probe. The probe and pump absorption spectra are analyzed by considering the contributions that derive from the individual ${m}_{g}\ensuremath{\rightarrow}{m}_{e}$ transitions. We then show how these contributions depend on the ground- and excited-state populations and Zeeman coherences, and investigate the role played by transfer of coherence from the excited to the ground hyperfine state. We show that the pump and probe absorption spectra are mirror images of each other when ${\ensuremath{\Omega}}_{1}\ensuremath{\ge}{\ensuremath{\Omega}}_{2}>\ensuremath{\Gamma}$, and have the same behavior at line center and complementary behavior in the wings, when ${\ensuremath{\Omega}}_{1}\ensuremath{\ge}{\ensuremath{\Omega}}_{2}<\ensuremath{\Gamma}$ ($\ensuremath{\Gamma}$ is the rate of spontaneous decay from Fe{F}_{e}Fe​ to Fg{F}_{g}Fg​).
We present a general formalism for studying the interaction between laser fields and degenerate-Zeeman-sublevel atoms correct up to the first order in the weak probe field. We derive from this theory the equations of motion for a \ensuremath{\Lambda}-type system involving S1/2{\mathit{S}}_{1/2}S1/2​, F=2\ensuremath{\leftrightarrows}P1/2{\mathit{P}}_{1/2}P1/2​, F\ensuremath{'}=1\ensuremath{\leftrightarrows}S1/2{\mathit{S}}_{1/2}S1/2​, F=1 transitions in 87Rb^{87}\mathrm{Rb}87Rb atoms. These equations are used to numerically investigate the coherent population trapping (CPT) schemes in the S1/2{\mathit{S}}_{1/2}S1/2​, F=2\ensuremath{\leftrightarrows}P1/2{\mathit{P}}_{1/2}P1/2​, F\ensuremath{'}=1 transition induced by a linearly polarized pumping field and the electromagnetically induced transparency exhibited in the weak probe spectrum in the S1/2{\mathit{S}}_{1/2}S1/2​, F=1\ensuremath{\leftrightarrows}P1/2{\mathit{P}}_{1/2}P1/2​, F\ensuremath{'}=1 transition. We discuss the effects of the CPT on the probe spectrum with and without the Doppler broadenings by comparing the probe spectrum derived from the real system with that derived from an ideal \ensuremath{\Lambda}-type system. We show that the atoms in the CPT states are shielded from interacting with the probe field while those in the absorbent states make contributions to the weak probe by the Raman anti-Stokes process, and the effect of the real system on the probe field becomes equivalent to the ideal \ensuremath{\Lambda} system only in the strong CPT parameter regime. \textcopyright{} 1996 The American Physical Society.
Employing two lasers as the coupling and probe fields which have opposite circular polarization (σ + and σ -), electromagnetically induced transparency (EIT) in Λ-type Zeeman sublevels of cesium 6 2S 1/2F=3-6 2P 3/2F′=2 degenerate two-level system has been demonstrated via probe absorption spectra. The effect of the intensity and detuning of different coupling. Laser on EII was also investigated in experiments. Within the Doppler background, optical pumping among Zeeman sub-levels and the population of different Zeeman sub-levels can dominate the intensity of EIT effect. And the physical reason of the rugged spectra are presented qualitatively.