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Physical Review Letters

Ferromagnetic spin-wave theory in the multiband Hubbard model having a flat band

Koichi Kusakabe, Hideo Aoki

Published Jan 3, 1994• 73 citations
Publisher

Abstract

The peculiar effect of electron correlation in multiband systems is illustrated for the recently proposed ferromagnetism in a Hubbard model having flat bands. Depsite the flatness of the band, an acoustic spin-wave mode with a finite stiffness exists along with optical modes below a Stoner gap. The relevant energy (gap and stiffness) transmutes from the Hubbard U in the weak-coupling limit to t (transfer integral) in the strong-coupling limit. This implies a stable itinerant ferromagnetism with finite band widths.

DOI
10.1103/physrevlett.72.144

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The peculiar effect of electron correlation in multiband systems is illustrated for the recently proposed ferromagnetism in a Hubbard model having flat bands. Depsite the flatness of the band, an acoustic spin-wave mode with a finite stiffness exists along with optical modes below a Stoner gap. The relevant energy (gap and stiffness) transmutes from the Hubbard U in the weak-coupling limit to t (transfer integral) in the strong-coupling limit. This implies a stable itinerant ferromagnetism with finite band widths.
It is believed that strong ferromagnetic interactions in some solids are generated by subtle interplay between quantum many-body effects and spin-independent Coulomb interactions between electrons. It is a challenging problem to verify this scenario in the Hubbard model, which is an idealized model for strongly interacting electrons in a solid. Nagaoka's ferromagnetism is a well-known rigorous example of ferromagnetism in the Hubbard model. It deals with the limiting situation in which there is one fewer electron than in the half-filling and the on-site Coulomb interaction is infinitely large. There are relatively new rigorous examples of ferromagnetism in Hubbard models called flat-band ferromagnetism. Flat-band ferromagnetism takes place in carefully prepared models in which the lowest bands (in the single-electron spectra) are “flat.” Usually, these two approaches are regarded as two complimentary routes to ferromagnetism in the Hubbard model. In the present paper we describe Nagaoka's ferromagnetism and flat-band ferromagnetism in detail, giving all the necessary background as well as complete (but elementary) mathematical proofs. By studying an intermediate model called the long-range hopping model, we also demonstrate that there is indeed a deep relation between these two seemingly different approaches to ferromagnetism. We further discuss some attempts to go beyond these approaches. We briefly discuss recent rigorous example of ferromagnetism in the Hubbard model which has neither infinitely large parameters nor completely flat bands. We give preliminary discussion regarding possible experimental realizations of the (nearly-)flat-band ferromagnetism. Finally, we focus on some theoretical attempts to understand metallic ferromagnetism. We discuss three artificial one-dimensional models in which the existence of metallic ferromagnetism can be easily proved. We have tried to make the present paper as self-contained as possible, keeping in mind readers who are new to the field. Although the present paper is written as a review, it contains some material which appears for the first time.
Kagome metals exhibit a rich interplay of topology, electronic correlations, and lattice dynamics. Recent discoveries of Kagome materials with a flat band near the Fermi level have revealed a variety of correlated electronic phases. However, elucidating their microscopic origin remains challenging, as realistic descriptions require accounting for multiple orbitals and competing interactions on an equal footing. To disentangle correlation effects from material-specific details and identify the essential physics of the flat-band regime, we study the single-orbital Kagome-Hubbard model at flat-band fillings using dynamical mean-field theory. We find strong signatures of flat-band ferromagnetism, consistent with exact and mean-field ground-state results. Moreover, we uncover an unconventional quasi-ordered phase in which a partially filled spin-polarized flat band pinned at the Fermi level gives rise to persistent local spin fluctuations down to zero temperature, in striking contrast to the classical behavior expected for a conventional ferromagnet. Our results demonstrate that these anomalous fluctuations are an intrinsic consequence of the flat-band degeneracy and establish a minimal framework for understanding correlation effects in flat-band Kagome systems.
Recently certain Hubbard models with flat lowest bands were proved to exhibit ferromagnetism. Here we study perturbed models with nearly flat bands. We prove that the ferromagnetic state is stable against a single-spin flip for sufficiently large Coulomb interaction UUU, but is unstable for small U>0U>0U>0. This is the first time that the (local) stability of ferromagnetism is proved in nonsingular Hubbard models, in which we must overcome competition between the kinetic energy and the Coulomb interaction.
Ferromagnetism in the Hubbard model is investigated on sc, bcc, and fcc lattices using a systematic inverse-degeneracy (1∕N)(1∕\mathcal{N})(1∕N) expansion which incorporates self-energy and vertex corrections such that spin-rotation symmetry and the Goldstone mode are explicitly preserved. First-order quantum corrections to magnon energies are evaluated for several cases, providing a comprehensive picture of the interplay of lattice, band dispersion, and interaction effects on the stability of the ferromagnetic state with respect to both long- and short-wavelength fluctuations. Our results support the belief that ferromagnetism is a generic feature of the Hubbard model at intermediate and strong coupling provided the density of states (DOS) is sufficiently asymmetric and strongly peaked near the band edge, as for the fcc lattice with finite ${t}^{\ensuremath{'}}$. For short-wavelength modes, the behavior of a characteristic energy scale ${\ensuremath{\omega}}^{*}\ensuremath{\sim}{T}_{c}$ (magnon DOS peak energy) is in excellent agreement with the Tc{T}_{c}Tc​ vs nnn behavior within dynamical mean field theory, with respect to both the stable range of densities (0.20<n<0.85)(0.20<n<0.85)(0.20<n<0.85) as well as the optimal density n=0.65n=0.65n=0.65. However, our finding of vanishing spin stiffness near optimal density highlights the role of long-wavelength fluctuations in further reducing the stable range of densities.