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Physical Review A

Absorption spectrum and gain without inversion of a driven two-level atom with arbitrary probe intensity in a squeezed vacuum

Peng Zhou, S. Swain

Published Jan 1, 1997• 44 citations
Publisher

Abstract

We examine the response of a coherently driven two-level atom interacting with a broadband squeezed vacuum to a probe beam of arbitrary intensity. The equations of motion for the reduced density matrix elements are numerically solved by nonperturbative matrix inversion methods. For large driving intensities, the absorption spectrum exhibits a number of multiphoton absorption peaks with increasing probe strength in a standard vacuum and in a squeezed vacuum with small photon numbers, while the multiphoton absorption peaks are wiped out for large squeezed photon numbers. Strong gain without inversion at line center can be obtained in the presence of the squeezed vacuum when the probe strength does not exceed the driving one. The absorption spectrum is phase sensitive. We also find the presence of remarkable, very narrow structures at line center. In general, the spectrum is symmetric when \ensuremath{\Phi}=0 and \ensuremath{\pi}; otherwise, it is asymmetric and displays a dispersivelike profile at line center.

DOI
10.1103/physreva.55.772

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Probe absorption spectra for driven atomic systems in a narrow bandwidth squeezed vacuum

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The behavior of a three level atom in a cascade configuration with the lower transition coherently driven and also coupled to a narrow bandwidth squeezed vacuum field is studied. A master equation treatment based on dressed atom states is used and expressions for probe absorption spectra are obtained via linear response theory and the quantum regression theorem. The expressions obtained also apply to the broad bandwidth squeezed vacuum case. Numerical studies of the modifications caused by the finite squeezed vacuum bandwidth to the Mollow and Autler-Townes probe absorption spectra are made for the case where the squeezed vacuum field center frequency and the driving laser frequency coincide and where upper transition relaxation terms are ignored. The squeezed vacuum source is assumed to be a degenerate parametric amplifier for the numerical calculations. Cases where the driving laser is resonant and detuned are examined. The spectral features are sensitively dependent on the phase of the squeezed vacuum field for a given driving laser phase. Dispersive features in the Mollow probe absorption spectrum can become absorptive, and vice versa. It is found in the probe absorption spectra that for certain choices of the squeezed vacuum phase lines narrower than for the broadband squeezed vacuum are obtained in the finite bandwidth situation. In both the Mollow and Autler-Townes spectra features narrower than for the normal vacuum case are obtained when the laser field is detuned, and in the Autler-Townes case this occurs for resonance also. \textcopyright{} 1996 The American Physical Society.

Physical Review A•Jun 1, 1996•29 citations
We examine the response of a coherently driven two-level atom interacting with a broadband squeezed vacuum to a probe beam of arbitrary intensity. The equations of motion for the reduced density matrix elements are numerically solved by nonperturbative matrix inversion methods. For large driving intensities, the absorption spectrum exhibits a number of multiphoton absorption peaks with increasing probe strength in a standard vacuum and in a squeezed vacuum with small photon numbers, while the multiphoton absorption peaks are wiped out for large squeezed photon numbers. Strong gain without inversion at line center can be obtained in the presence of the squeezed vacuum when the probe strength does not exceed the driving one. The absorption spectrum is phase sensitive. We also find the presence of remarkable, very narrow structures at line center. In general, the spectrum is symmetric when \ensuremath{\Phi}=0 and \ensuremath{\pi}; otherwise, it is asymmetric and displays a dispersivelike profile at line center.
We study the absorption spectra of a weak probe beam that interacts with a driven two-level atom in the presence of a squeezed vacuum. In particular, we focus on the behavior of the central resonance of the probe absorption spectra in the region of intermediate driving intensities and in the large squeezed photon number limit. Squeezing-induced pimples, hole-burning, and dispersive profiles at line center are displayed. These unusual spectral features are highly sensitive to the squeezing phase and to the Rabi frequency of the driving field. We present analytical conditions for the occurrence of these effects and find that they all take place in the vicinity of the critical point dividing the different dynamical regimes, probe absorption and amplification, of the atomic radiation. We also investigate analytically and numerically the two-time correlation functions of the atomic polarization and find that the cross correlations of the two dipole quadratures contribute symmetric (absorptionlike) spectral features to the absorption spectra, whereas the self-correlations contribute asymmetric (dispersionlike) spectral profiles, which disappear for the particular phase values Φ = 0, π. The physical origin of the unusual spectral profiles at line center is also discussed in terms of the coherent population oscillations.
A comprehensive study is made of the absorption spectrum of a weak-probe beam irradiating a two-level atom damped by a broadband squeezed vacuum and driven by a strong laser field. We show that for a resonant driving field whose phase does not coincide with the principal directions of the squeezing ellipse, the absorption spectrum is asymmetric and exhibits absorption-emission profiles at the Rabi sidebands. We find that this feature arises from unequal populations of the dressed states of the system, which occur when all components of the Bloch vector are coupled to the driving field. A symmetric spectrum with dispersionlike profiles at the Rabi sidebands is revealed for an off-resonant driving field. Furthermore, the spectrum may exhibit an emission profile at the central frequency, signifying an amplification of the probe beam. We point out that the amplification at the central component is not attributed to population inversion in both the atomic bare states and in the dressed atomic states. We find that the amplification originates from the coherent population oscillations and is impossible in the absence of the squeezed vacuum. In addition, we examine how these features are affected by the detuning of the driving field and an imperfect squeezed vacuum.
The resonance fluorescence system of a coherently driven two-level atom in the presence of a broadband squeezed vacuum field whose central frequency is not in resonance with either the driving field frequency or the atomic transition frequency is analyzed. Solutions of the Bloch equations of the system are presented in terms of continued fractions for arbitrary strength of the coherent driving field. Numerical results are presented for the first-harmonic quadrature components of the absorption spectrum and the fluorescent intensity. The effects of the squeezed vacuum field detuning on the absorption spectrum result in hole burning or a dip structure in the weak-field case and two absorption–amplification peaks in the strong-field case. Results are sensitive to the relative phase of the squeezed vacuum.
We present numerical and analytical results for the Mollow probe absorption spectrum of a coherently driven two-level system in a narrow bandwidth squeezed vacuum field. The spectra are calculated for the case where the Rabi frequency of the driving field is much larger than the natural linewidth and the squeezed vacuum carrier frequency is detuned from the driving laser frequency. The driving laser is on resonance. We show that in a detuned squeezed vacuum the standard Mollow features are each split into triplets. The central components of each triplet are weakly dependent on the squeezing phase but the sidebands strongly depend on the phase and can have dispersive or absorptive/emissive profiles. We also derive approximate analytical expressions for the spectral features and find that the multi-peak structure of the spectrum can be interpreted either via the eigenfrequencies of a generalized Floquet Hamiltonian or in terms of three-photon transitions between dressed states involving a probe field photon and a correlated photon pair from the squeezed vacuum field.
The behavior of a three level atom in a cascade configuration with the lower transition coherently driven and also coupled to a narrow bandwidth squeezed vacuum field is studied. A master equation treatment based on dressed atom states is used and expressions for probe absorption spectra are obtained via linear response theory and the quantum regression theorem. The expressions obtained also apply to the broad bandwidth squeezed vacuum case. Numerical studies of the modifications caused by the finite squeezed vacuum bandwidth to the Mollow and Autler-Townes probe absorption spectra are made for the case where the squeezed vacuum field center frequency and the driving laser frequency coincide and where upper transition relaxation terms are ignored. The squeezed vacuum source is assumed to be a degenerate parametric amplifier for the numerical calculations. Cases where the driving laser is resonant and detuned are examined. The spectral features are sensitively dependent on the phase of the squeezed vacuum field for a given driving laser phase. Dispersive features in the Mollow probe absorption spectrum can become absorptive, and vice versa. It is found in the probe absorption spectra that for certain choices of the squeezed vacuum phase lines narrower than for the broadband squeezed vacuum are obtained in the finite bandwidth situation. In both the Mollow and Autler-Townes spectra features narrower than for the normal vacuum case are obtained when the laser field is detuned, and in the Autler-Townes case this occurs for resonance also. \textcopyright{} 1996 The American Physical Society.