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Journal of Physics A Mathematical Nuclear and General

Theory of radiation reaction and atom self-energies: all-order perturbation theory of the generalized non-relativistic Lamb shift

R. Bullough, P. J. Caudrey, A.‐S. F. Obada

Published Sep 1, 1974• 12 citations
Publisher

Abstract

A natural all-order decorrelation procedure is described for the interaction of a single two-level atom with all modes of the radiation field which replaces the semi-classical boson approximation for the atom by an exact fermion treatment. In consequence the vacuum Lamb shift appears as twice the Bethe shift for each level separately instead of the limiting neo-classical shift obtained in the Bose theory. Stimulated emission and absorption modify the Einstein A-coefficient and the vacuum shift is extended to include a field dependent shift. The all-order decorrelated perturbation theory yields an equation of motion for the single-atom dipole moment which includes those reported from operator radiation reaction theory recently; but it also generalizes these by including the effects of stimulated processes. The method is extended to a many-atom case in which it becomes necessary to modify the procedure slightly.

DOI
10.1088/0305-4470/7/13/019

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A natural all-order decorrelation procedure is described for the interaction of a single two-level atom with all modes of the radiation field which replaces the semi-classical boson approximation for the atom by an exact fermion treatment. In consequence the vacuum Lamb shift appears as twice the Bethe shift for each level separately instead of the limiting neo-classical shift obtained in the Bose theory. Stimulated emission and absorption modify the Einstein A-coefficient and the vacuum shift is extended to include a field dependent shift. The all-order decorrelated perturbation theory yields an equation of motion for the single-atom dipole moment which includes those reported from operator radiation reaction theory recently; but it also generalizes these by including the effects of stimulated processes. The method is extended to a many-atom case in which it becomes necessary to modify the procedure slightly.
Reports a natural all-order decorrelation procedure for the interaction of a single two-level atom with all modes of the radiation field which replaces the semiclassical boson approximation for the atom by an exact fermion treatment. In consequence, the spontaneous emission of the semiclassical theory is extended to include stimulated emission, a semiclassical Lamb-type shift is explicitly replaced by a shift satisfying the Bethe formula manifestly due to vacuum fluctuations, and there can be two intensity-dependent terms, one of which generalizes the Bethe formula.
An improved form of semiclassical radiation theory is developed which includes the effect of the atom's radiation field back on the atom. This formalism is applied to the problem of a single "two-level atom" interacting with a monochromatic field. The resulting equations are solved without resorting to time-dependent perturbation theory, and are found to predict the behavior of the system over times long compared with the lifetime for spontaneous transitions. Not only stimulated emission and absorption, but also spontaneous emission with the proper Einstein AAA coefficient, and a frequency shift which agrees at least semiquantitatively with the Lamb shift are described. In addition, several nonlinear effects involving the interference between spontaneous and stimulated radiation are described, and new experiments which might detect such effects are suggested.
An improved form of semiclassical radiation theory is developed which includes the effect of the atom's radiation field back on the atom. This formalism is applied to the problem of a single two-level atom interacting with a monochromatic field. The resulting equations are solved without resorting to time-dependent perturbation theory, and are found to predict the behavior of the system over times long compared with the lifetime for spontaneous transitions. Not only stimulated emission and absorption, but also spontaneous emission with the proper Einstein AAA coefficient, and a frequency shift which agrees at least semiquantitatively with the Lamb shift are described. In addition, several nonlinear effects involving the interference between spontaneous and stimulated radiation are described, and new experiments which might detect such effects are suggested.
The field generalizes in a natural way the c-number theory of radiation reaction and frequency shifts due to Lorentz. By a trivial extension the operator field can be applied to the more complicated cases of a single multi-level atom and the super-radiant problem of N atoms on the same site where these are coupled either to the vacuum or the vacuum and additional imposed quantized fields. By further extension it also applies to the case of N atoms on different sites. Explicit expressions for positive and negative frequency parts of the total operator field are given in terms of arbitrary dipole operator sources and are apparently valid for times t>> omega s -1 >> omega max -1 where omega s is the atomic resonance and omega max a cut-off used systematically throughout the theory.
The interaction of an atomic system with an unquantized electromagnetic field is studied by means of the Heisenberg-operator equations of motion. The electromagnetic fields created by the atom are taken into account by assuming that the charge and probability current densities are the actual charge and current source terms in Maxwell's equation. When Ehrenfest's theorem is written to order (1/c)2{)}^{2})2, the equations of motion are found to have a constant of motion that can be interpreted as stating that the sum of the atomic energy, energy of interaction, and energy stored in the electromagnetic field is constant. This constant of integration can be expressed as an expectation of a new semiclassical Hamiltonian that now includes the effects of the atomic self-fields to order 1/c2{\mathit{c}}^{2}c2. This Hamiltonian is related to the classical Darwin Lagrangian. Since the new approximate Hamiltonian is the sum of an atomic and a field Hamiltonian, it provides a formulation of semiclassical radiation theory that is formally close to the usual formulation of quantum electrodynamics. A Schr\"odinger equation can be derived by applying the variational principle to the expectation of the new Hamiltonian. The result is a nonlinear integro-differential equation, in \ensuremath{\Psi}, which is somewhat similar to Hartree's self-consistent equation for a multielectron atom.When the Heisenberg equations are written to include the next-higher-order terms, 1/c3{\mathit{c}}^{3}c3, it is found that the total energy of the atom and the electromagnetic field in the vicinity of the atom decreases at a rate that is given by the Larmor power formula (2e2{\mathit{e}}^{2}e2/3c3{\mathit{c}}^{3}c3)(d〈v〉/dt)2{)}^{2})2, where 〈v〉 is the quantum-mechanical expectation of the electron's velocity operator. This approximate formulation of semiclassical radiation theory is applied to semiclassical calculations of atomic radiative shifts. It is then shown that, if some retardation effects are included to all orders of 1/c in the vector potential, the semiclassical analysis provides a formula for radiative energy-level shifts that are time dependent and that contain coefficients similar to the starting point of the Bethe calculation of the Lamb shift. The incorporation of mass renormalization in semiclassical theory is then discussed.
A general perturbation procedure is described for writing down the contributions to any order for the probability of a quantum system described by a time-independent Hamiltonian making a transition from an arbitrary initial state to an arbitrary final state. The results are expressed in terms of certain propagators which involve continued fractions, so that some processes are summed to all orders. The general theory is then applied to a single multilevel atom interacting with any number of modes of the electromagnetic field in the electric dipole approximation. The fundamental theory is considered primarily but a detailed discussion is given of spontaneous and stimulated emission. Expressions for the lineshape are derived incorporating the generalized Lamb shifts and damping constants.