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Physical Review Letters

Collective Effects in the Self-Interference of a Single Photon Emitted by Two Atoms

Ho Trung Dung, Kikuo Ujihara

Published Jan 10, 2000• 15 citations
Publisher

Abstract

Collective effects in the spontaneous emission pattern of two identical two-level atoms a fixed distance apart and sharing initially a single excitation are investigated. It is shown that the interference can take place even when it is known for certain which atom is excited initially. This interference is due solely to the atomic coherence established through multiple photon absorptions and reemissions and will disappear if it is ignored. The interference patterns with and without collective effects are compared for symmetric and antisymmetric initial states. The dark center from an antisymmetric state is shown both analytically and numerically.

DOI
10.1103/physrevlett.84.254

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Collective effects in the spontaneous emission pattern of two identical two-level atoms a fixed distance apart and sharing initially a single excitation are investigated. It is shown that the interference can take place even when it is known for certain which atom is excited initially. This interference is due solely to the atomic coherence established through multiple photon absorptions and reemissions and will disappear if it is ignored. The interference patterns with and without collective effects are compared for symmetric and antisymmetric initial states. The dark center from an antisymmetric state is shown both analytically and numerically.
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We report the generation of a new quantum interference effect in spontaneous emission from a resonantly driven system of two identical two-level atoms due to the spatial variation of the laser phase at the positions of the atoms. This interference affects significantly the spectral features of the emitted radiation and the quantum entanglement in the system. The interference leads to dynamic coupling of the populations and coherences in a basis, determined by the laser phase and represents a kind of vacuum mediated superexchange between the symmetric and antisymmetric states.
The role of the collective antisymmetric state in entanglement creation by spontaneous emission in a system of two non-overlapping two-level atoms has been investigated. Populations of the collective atomic states and the Wootters entanglement measure (concurrence) for two sets of initial atomic conditions are calculated and illustrated graphically. Calculations include the dipole-dipole interaction and a spatial separation between the atoms that the antisymmetric state of the system is included throughout even for small interatomic separations. It is shown that spontaneous emission can lead to a transient entanglement between the atoms even if the atoms were prepared initially in an unentangled state. It is found that the ability of spontaneous emission to create transient entanglement relies on the absence of population in the collective symmetric state of the system. For the initial state of only one atom excited, entanglement builds up rapidly in time and reaches a maximum for parameter values corresponding roughly to zero population in the symmetric state. On the other hand, for the initial condition of both atoms excited, the atoms remain unentangled until the symmetric state is depopulated. A simple physical interpretation of these results is given in terms of the diagonal states of the density matrix of the system. We also study entanglement creation in a system of two non-identical atoms of different transition frequencies. It is found that the entanglement between the atoms can be enhanced compared to that for identical atoms, and can decay with two different time scales resulting from the coherent transfer of the population from the symmetric to the antisymmetric state. In addition, it was found that a decaying initial entanglement between the atoms can display a revival behaviour.
We present an analysis of the spontaneous emission by two identical two-level atoms a distance R apart, both of which are initially in the upper state. This analysis applies for two interacting atoms emitting both in a free space and in a cavity structure. In this paper we use the Heisenberg picture. We work under the dipole approximation and the rotating-wave approximation. We assume that all the field modes are initially in the vacuum state and the two atoms A and B are in the upper state. We will concentrate on the motion of the product of the dipole operators of two atoms. Because we have two excitations at t=0, and because we work under rotating-wave approximation, we will always have two excitations, i.e., two excited atoms, or one excited atom plus one photon, or two unexcited atoms with two photons.
The possibility of realization of collective resonance fluorescence of extended systems of atoms in the strong travel and standing laser waves it is demonstrated. The influence of regular arrangement of the atoms in interaction with the laser pulls on the fluorescence intensity is analyzed. Taking in to account that such interference can be realize in two distant atomic ensembles we analyzed the collective interference phenomena between the fluorescent fields in the farther field detection region. These effects depend on the exchange integrals between systems of atoms through vacuum fluorescence field. The fluorescence spectrum of these atoms is found. About similar coherence interference experiment of spontaneous emission of light from two distant solid-state ensembles of atoms that are coherently excited by a short laser pulse it is reported in the papers [1,2]. For example, in paper [1] it is observed the entanglement between two distant atomic ensembles located in distinct apparatuses on different tables. Quantum interference in the detection of a photon emitted by one of the samples projects the otherwise independent ensembles into an entangled state with one joint excitation stored remotely in 105 atoms at each site. The experiment [2] relate about the ensembles of erbium ions doped into two LiNbO3 crystals with channel wave guides, which are placed in the two arms of a Mach-Zehnder interferometer. The light that is spontaneously emitted after the excitation pulse shows first-order interference. By a strong collective enhancement of the emission, the atoms behave as ideal two-level quantum systems and no which-path information is left in the atomic ensembles after emission of a photon. Influence of geometry of the sample on the coherent phenomena between two distant systems of atoms in this report is presented.