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arXiv:0808.0178 · Physical Review Letters

Quantum Interferences in Cooperative Dicke Emission from Spatial Variation of the Laser Phase

Sumanta Das, G. S. Agarwal, Marlan O. Scully

Published Oct 6, 2008• 83 citations
arXivHTMLPDF

Abstract

We report the generation of a new quantum interference effect in spontaneous emission from a resonantly driven system of two identical two-level atoms due to the spatial variation of the laser phase at the positions of the atoms. This interference affects significantly the spectral features of the emitted radiation and the quantum entanglement in the system. The interference leads to dynamic coupling of the populations and coherences in a basis, determined by the laser phase and represents a kind of vacuum mediated superexchange between the symmetric and antisymmetric states.

DOI
10.1103/physrevlett.101.153601

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We report the generation of a new quantum interference effect in spontaneous emission from a resonantly driven system of two identical two-level atoms due to the spatial variation of the laser phase at the positions of the atoms. This interference affects significantly the spectral features of the emitted radiation and the quantum entanglement in the system. The interference leads to dynamic coupling of the populations and coherences in a basis, determined by the laser phase and represents a kind of vacuum mediated superexchange between the symmetric and antisymmetric states.
We analyze the effect of the position-dependent excitation phase on the properties of entanglement between two qubits formed in atomic systems. We show that the excitation phase induces a vacuum-mediated quantum interference in the system that affects the dynamical behavior of entanglement between the qubits. It is also found that the quantum interference leads to a coherent population transfer between the symmetric and antisymmetric states that can considerably modify the dynamics of two-qubit entanglement and can even prevent finite-time disentanglement (sudden death) under certain conditions.
The transmission spectrum of a two-atom timed Dicke state is investigated in an open optical cavity. In the proposed system, two identical atoms are excited by an external single photon field. In this process, the excited atoms grasp different excitation phases for their different spatial positions. For identical coupling strength of atoms and cavity, the excitation phases get coupled via cavity and vacuum fields, and they finally induce cosine-type quantum interference on the two splitting peaks of the spectrum. However, when one of the atoms is decoupled with the cavity, the excitation phases cannot get coupled directly via the cavity but must be mediated by the vacuum fields, which leads to opposite quantum interference effects on the two splitting peaks. In addition, we find that the real and virtual vacuum-mediated excitation phase couplings generate different quantum interferences. The real vacuum-meditated coupling induces sine-type quantum interference, while it becomes cosine-type for the virtual vacuum-mediated coupling. Our study clarifies the mechanism of quantum interference in the two-atom timed Dicke state and provides a feasible scheme for investigating the effect of vacuum-mediated excitation phase coupling.
Possibility of coherent control of spontaneous emission from four- and five-level systems in the laser radiation field is studied. The four-level system consists of two levels resonantly driven by laser radiation where either of levels may decay to a separate level. For such a system we show that the presence of the second decay channel may deteriorate the destructive interference occurring because of Autler-Townes effect in case of one decay channel. The five-level system represents two two-level resonantly driven systems with the upper levels decaying to a common level. For this case, the interference between the two decay channels is partially or completely destructive or constructive depending on the initial conditions and on the mutual orientation of the transition dipole moments. It is shown that population transfer takes place by the same quantum vacuum via spontaneous emission. The populations are shown to have damping oscillatory nature.
Quantum interference and coherence effects in the interaction of atoms with the quantized electromagnetic field are investigated theoretically. A general master equation for the description of atom-field interactions is introduced. The interplay of the concepts of complementarity and interference in the time-energy domain are studied on the basis of the fluorescence light emitted by a single laser-driven atom, where the coherence of spontaneous processes gives rise to quantum interference in the spectrum of resonance fluorescence. The vacuum-induced dipole-dipole interaction in pairs of multi-level atoms is analyzed. It is shown that the interaction between orthogonal transition dipole moments of different atoms does not only influence the system dynamics crucially, but implies that the few-level approximation in general cannot be applied to near-degenerate Zeeman sublevels of the atomic level scheme. Potential applications of dipole-dipole interacting multi-level atoms for the implementation of decoherence-free subspaces and the generation of entanglement between atomic states are examined. The generation of an entangled state of the radiation field with a macroscopic number of photons is discussed on the basis of a single-atom laser.
In this paper we investigate the resonance fluorescence, the squeezing, and the absorption spectra of a laser-driven four-level atom consisting of three closely spaced upper levels decaying to a common lower level. The three upper levels are coupled by the same vacuum modes to the lower level leading to spontaneously generated coherence effects. High population inversion and extremely narrow emission lines are obtained with moderate Rabi frequencies, which are a direct consequence of decay-induced interferences. The fluorescent field is shown to exhibit two-mode squeezing in the in-phase quadrature. Squeezing in both quadratures simultaneously at different frequencies is greatly enhanced when quantum interference is accounted for. We also examine the absorption spectrum of a weak field and demonstrate that quantum interference can induce two prominent and nearly transparent holes where the slope of the refractive index is very steep. This special situation could allow the simultaneous propagation of two weak pulses with different frequencies, which could be feasibly exploited towards the realization of the entanglement of two photons.
Dicke superradiance, i.e., the enhanced spontaneous emission of coherent radiation, is often attributed to radiation emitted by synchronized dipoles coherently oscillating in phase. At the same time, Dicke derived superradiance assuming atoms in entangled Dicke states which do not display any dipole moment. To shed light on this apparent paradox, we study the intensity distribution arising from two identical two-level atoms prepared either in an entangled Dicke state or in a separable atomic state with a nonvanishing dipole moment. We find that the two configurations produce similar far-field intensity patterns, although they stem from fundamentally distinct types of coherence: while in the second case the atoms display coherence among the individual particles, leading to Young-type interference like that known from classical dipoles, atoms in Dicke states possess collective quantum coherence stemming from entanglement and quantum correlations of the state, leading to an interference pattern resulting from enhanced spontaneous emission. This demonstrates that the radiation generated by synchronized dipoles and Dicke superradiance---even if they do produce the same interference pattern---are fundamentally distinct phenomena and have to be interpreted in different ways.