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Physical Review A

Spontaneously generated coherence effects in a laser-driven four-level atomic system

M. A. Antón, Óscar G. Calderón, F. Carreño

Published Aug 10, 2005• 80 citations
Publisher

Abstract

In this paper we investigate the resonance fluorescence, the squeezing, and the absorption spectra of a laser-driven four-level atom consisting of three closely spaced upper levels decaying to a common lower level. The three upper levels are coupled by the same vacuum modes to the lower level leading to spontaneously generated coherence effects. High population inversion and extremely narrow emission lines are obtained with moderate Rabi frequencies, which are a direct consequence of decay-induced interferences. The fluorescent field is shown to exhibit two-mode squeezing in the in-phase quadrature. Squeezing in both quadratures simultaneously at different frequencies is greatly enhanced when quantum interference is accounted for. We also examine the absorption spectrum of a weak field and demonstrate that quantum interference can induce two prominent and nearly transparent holes where the slope of the refractive index is very steep. This special situation could allow the simultaneous propagation of two weak pulses with different frequencies, which could be feasibly exploited towards the realization of the entanglement of two photons.

DOI
10.1103/physreva.72.023809

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In this paper we investigate the resonance fluorescence, the squeezing, and the absorption spectra of a laser-driven four-level atom consisting of three closely spaced upper levels decaying to a common lower level. The three upper levels are coupled by the same vacuum modes to the lower level leading to spontaneously generated coherence effects. High population inversion and extremely narrow emission lines are obtained with moderate Rabi frequencies, which are a direct consequence of decay-induced interferences. The fluorescent field is shown to exhibit two-mode squeezing in the in-phase quadrature. Squeezing in both quadratures simultaneously at different frequencies is greatly enhanced when quantum interference is accounted for. We also examine the absorption spectrum of a weak field and demonstrate that quantum interference can induce two prominent and nearly transparent holes where the slope of the refractive index is very steep. This special situation could allow the simultaneous propagation of two weak pulses with different frequencies, which could be feasibly exploited towards the realization of the entanglement of two photons.
The squeezing spectrum of the fluorescent light is investigated for a laser-driven three-level atom of the $\ensuremath{\Lambda}$ configuration when quantum interference of the decay channels is accounted for. We show that when the two atomic transitions contribute to the detected fluorescence field, squeezing at certain frequency intervals is obtained in both the weak- and the high-Rabi-frequency regimes even for equally decay rates of the transitions. Unlike in two-level atoms in free space, squeezing can be obtained in both the in-phase and out-of-phase quadrature spectra although in different spectral regions. We also show that the squeezing spectrum can be controlled by an adequate selection of the Rabi frequencies and atomic detunings. Another remarkable effect is that squeezing can be achieved with proper relative phases of the driving fields. We provide an analytical description in the dressed basis which accounts for the main features of the squeezing spectra obtained from the numerical work.
We investigate steady-state squeezing in the phase quadratures of the resonance fluorescence emitted from a coherently driven four-level atom of $\ensuremath{\Lambda}$ configuration. Quantum fluctuation spectra of the optimum-phase quadratures are calculated. We show that if quantum interference between spontaneous emission channels from closed excited states to lower levels of the atom takes place, squeezing in the optimum-phase quadrature can occur in a very wider region of the parameter space than that predicted by previous studies. We also show that the quantum interference can greatly change the atomic coherences and then lead to this interesting result.
Summary form only given. We consider a single two-level atom inside a resonant optical cavity, with cavity loss rate K, atomic fluorescence rate into noncavity modes A, and atom-field coupling g. For large atom cavity coupling (g>A, K) and weak driving fields, the fluorescence from this system exhibits a splitting of the spectral line, known as vacuum-Rabi splitting. When the cavity loss rate is the largest rate in the problem (K>A, g), the fluorescent spectrum is Lorentzian with a cavity-enhanced width. We examine the regime where A>g>K, and find that the spectrum exhibits a hole at line center as a result of quantum interference effects. This effect is formally identical to the phenomenon of electromagnetically induced transparency (EIT) in multilevel atomic systems. We discuss the relationship of these spectral holes to the presence of squeezing in the intracavity field, and present results also for the emission spectra, and incoherent spectra in transmission and fluorescence.
We investigate the effects of spontaneously generated interference on the spectrum of quantum fluctuations in phase quadratures of resonant fluorescence emitted from the transition of j = 1/2 to j = 1/2 of a monochromatically driven four-level atom with antiparallel dipole moments. It is found that the spectrum exhibits obvious characteristics of quantum interference in both cases of weak and strong laser fields. For the Zeeman-degenerate system, strong radiation squeezing in weak atomic excitation can occur at the central frequency of the spectrum, which is quite different from the case without consideration of the interference. Moreover, when we apply an external magnetic field to the atom, we find that the quantum interference can lead to a narrowing spectrum with much stronger squeezing by adjusting the magnetic field strength. These results suggest that the phase-dependent fluorescence spectrum can serve as a probe of the quantum interference effects in a realistic system such as a trapped 198Hg+ ion or charged quantum dots.
The spectrum of quantum fluctuations in phase quadratures of resonance fluorescence of a three-level V-type atom driven by a coherent field is investigated. We find that quantum interference between two decay channels of the atom can greatly modify the spectrum. We show that for weak excitation, quantum interference can greatly enhance squeezing and change the phase quadrature in which the maximum squeezing occurs. We also show that for strong and far-off-resonance excitation two deeply squeezing peaks appear at the Rabi sideband frequencies and quantum interference broadens the squeezing peaks.
The quadrature squeezing spectra in the resonance fluorescence of a V-type three-level atom driven by a coherent field and coupled to a single-mode cavity is investigated. For weak excitation, the fluorescence field exhibit squeezing in the out-of-phase quadrature. The coupling between the atom and the cavity mode can greatly enhance the squeezing centred at the laser frequency. More importantly, for strong excitation, under the effect of the cavity-atom coupling, the in-phase quadrature of fluorescence can exhibit two-mode squeezing at the two inner sideband frequencies. By working in the dressed-state representation and hiring secular approximation, we give an analytical explanation for the effect. The result shows, under appropriate conditions, the squeezing can be greatly enhanced by appropriately tuning the cavity resonant frequency.