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The Journal of Chemical Physics

Ising Chain with Several Phase Transitions

W. K. Theumann, J. S. Ho ye

Published Nov 1, 1971• 21 citations
Publisher

Abstract

The one-dimensional spin-½ Ising model with very long-range ferromagnetic interaction and first and second neighbor antiferromagnetic interactions is solved exactly in a direct magnetic field. A study of the finite temperature behavior confirms the existence of up to four first-order phase transitions ending in classical critical points. We find a confluence of three critical lines at a ``tricritical'' point with exponents β=14 , δ=5, γ=γ′=1,α=0, and α′=12. We find also a confluence of four critical lines at a ``tetracritical'' point with exponents β=14, δ=7, γ=γ′=1, α=0, and α′=23. We show the existence of triple lines and ``quadruple'' lines, along which three or four phases are simultaneously in contact with each other, respectively. For some special values of the interaction strengths, five phases are in contact with each other at a ``quintuple'' point. We remark that our ``multiple'' lines and ``multicritical'' points are not ``true'' multiple lines and multicritical points but that they would be so in a somewhat extended model. This model satisfies a generalized form of the ordinary phase rule of Gibbs. In distinction to various models considered recently, our model does not exhibit a singular phase-boundary diameter.

DOI
10.1063/1.1676731

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The one-dimensional spin-½ Ising model with very long-range ferromagnetic interaction and first and second neighbor antiferromagnetic interactions is solved exactly in a direct magnetic field. A study of the finite temperature behavior confirms the existence of up to four first-order phase transitions ending in classical critical points. We find a confluence of three critical lines at a tricritical'' point with exponents β=14 , δ=5, γ=γ′=1,α=0, and α′=12. We find also a confluence of four critical lines at a tetracritical'' point with exponents β=14, δ=7, γ=γ′=1, α=0, and α′=23. We show the existence of triple lines and quadruple'' lines, along which three or four phases are simultaneously in contact with each other, respectively. For some special values of the interaction strengths, five phases are in contact with each other at a quintuple'' point. We remark that our multiple'' lines and multicritical'' points are not ``true'' multiple lines and multicritical points but that they would be so in a somewhat extended model. This model satisfies a generalized form of the ordinary phase rule of Gibbs. In distinction to various models considered recently, our model does not exhibit a singular phase-boundary diameter.
The one-dimensional spin-\textonehalf{} Ising model is solved exactly with very long-range, equivalent-neighbor ferromagnetic interactions of strength JLR{J}_{\mathrm{LR}}JLR​ superimposed on nearest-neighbor anti-ferromagnetic interactions of strength $\ensuremath{-}{J}_{\mathrm{sr}}$. For $\ensuremath{-}\frac{{J}_{\mathrm{lr}}}{{J}_{\mathrm{sr}}} >R=3.1532$... there is a critical point of classical type in zero field. For $2\ensuremath{-}\frac{{J}_{\mathrm{lr}}}{{J}_{\mathrm{sr}}}=R$ the critical exponents take the values $\ensuremath{\beta}=\frac{1}{4}$, $\ensuremath{\gamma}=1={\ensuremath{\gamma}}^{\ensuremath{'}}$, $\ensuremath{\delta}=5$, and $0=\ensuremath{\alpha}\ensuremath{\ne}{\ensuremath{\alpha}}^{\ensuremath{'}}=\frac{1}{2}$. For $2<\ensuremath{-}\frac{{J}_{\mathrm{lr}}}{{J}_{\mathrm{sr}}}<R$ the transition in zero field is of first order, and the critical points which occur in finite field are of classical type. For $0<\ensuremath{-}\frac{{J}_{\mathrm{lr}}}{{J}_{\mathrm{sr}}}<2$ there is no phase transition in zero field, although there are classical critical points in a field.
We have studied the phase diagrams of the one-dimensional spin-1 Blume-Capel model with anisotropy constant D, in which equivalent-neighbor ferromagnetic interactions of strength -J are superimposed on nearest-neighbor antiferromagnetic interactions of strength K. A rich critical behavior is found due to the competing interactions. At zero temperature two ordered phases exist in the D/J-K/J plane, namely the ferromagnetic (F) and the antiferromagnetic one (AF). For lower values of D/J(D/J<0.25) these two ordered phases are separated by the point K_{c}=0.25J. For 0.25<D/J≤0.50, the paramagnetic phase P emerges in a region separated between the lines determined by D/J=0.5-K/J and D/J=K/J. For D/J>0.5, only phases AF and F exist and are separated by a line given by D/J=K/J. At finite temperatures, we found that the ferromagnetic region of the phase diagram in the k_{B}T/J-D/J plane is enriched by another ferromagnetic phase F^{^{'}} above a first-order line for 0.195<K/J<0.250. This first-order line, which separates phases F and F^{^{'}}, begins at a coexistence point, where phases F,F^{^{'}}, and P coexist, and ends at an ordered critical point. Similarly, we found that the phase F^{^{'}} is present in the phase diagram in the k_{B}T/J-K/J plane for 0.228<D/J<0.286.
In the framework of mean field approximation, we consider a spin system consisting of two interacting sub-ensembles. The intra-ensemble interactions are ferromagnetic, while the inter-ensemble interactions are antiferromagnetic. We define the effective number of the nearest neighbors and show that if the two sub-ensembles have the same effective number of the nearest neighbors, the classical form of critical exponents (α=0, β=1/2, γ=γ'=1, δ=3) gives way to the non-classical form (α=0, β=3/2, γ=γ'=0, δ=1), and the scaling function changes simultaneously. We demonstrate that this system allows for two second-order phase transitions and two first-order phase transitions. We observe that an external magnetic field does not destroy the phase transitions but only shifts their critical points, allowing for control of the system's parameters. We discuss the regime when the magnetization as a function of the magnetic field develops a low-magnetization plateau and show that the height of this plateau abruptly rises to the value of one when the magnetic field reaches a critical value. Our analytical results are supported by a Monte Carlo simulation of a three-dimensional layered model.
We study the ground-state properties of a spin-1/2 model on a chain containing four-spin Ising-like interactions in the presence of both transverse and longitudinal magnetic fields. We use entanglement entropy and finite-size scaling methods to obtain the phase diagrams of the model. Our numerical calculations reveal a rich variety of phases and the existence of multicritical points in the system. We identify phases with both ferromagnetic and antiferromagnetic orderings. We also find periodically modulated orderings formed by a cluster of like spins followed by another cluster of opposite like spins. The quantum phases in the model are found to be separated by either first- or second-order transition lines.
We describe the essential features of the mean-field phase diagram for the spin-1 Ising model with general nearest-neighbor interaction when sublattice ordering is made explicit. The phase diagram (in five-dimensional field space) can be classified into 84 zones where uniform with ordered phase coexistence is identified and multicritical behavior is determined. This generalized Ising model was studied extensively, in its ferromagnetic version, by Furman, Dattagupta, and Griffiths towards the end of the last decade. Here we complement that study with the antiferromagnetic phase behavior associated with the same model. Two different mappings between uniform and ordered phase existence conditions facilitated our task and indicated the interconnections that exist between ferromagnetic and antiferromagnetic properties in the model. Known features, like the ``shield'' region, appear reproduced in other energy-parameter locations, but also new features occur, such as additional tricritical and fourth-order critical lines connected by sixth-order critical points.
We study the phase diagram of the four dimensional Ising model with first and second neighbour couplings, specially in the antiferromagnetic region, by using Mean Field and Monte Carlo methods. From the later, all the transition lines seem to be first order except that between ferromagnetic and disordered phases in a region including the first-neighbour Ising transition point. 1 Antiferromagnetism has been considered in a great variety of models in order to find properties not present in the purely ferromagnetic (FM) system. Mostly they have been models in two and three dimensions. For instance, in several works on High Temperature Superconductivity the transition from paramagnetic (PM) to non-pure FM ordered phases has been studied [1, 2, 3, 4]. On the other hand, in relation to the finite temperature phase transition in pure gauge SU(3), the d = 3 three state Potts model with negative second neighbour couplings was unsuccessfully considered to find a new critical behaviour [5, 6]. In four dimensions, in diluted systems recently new critical exponents have been