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Physical Review Letters

Roton-Roton Crossover in Strongly Correlated Dipolar Bose-Einstein Condensates

Diana Hufnagl, Rainer Kaltseis, V. Apaja, Robert E. Zillich

Published Aug 4, 2011• 26 citations
Publisher

Abstract

We study the pair correlations and excitations of a dipolar Bose gas layer. The anisotropy of the dipole-dipole interaction allows us to tune the strength of pair correlations from strong to weak perpendicular and weak to strong parallel to the layer by increasing the perpendicular trap frequency. This change is accompanied by a roton-roton crossover in the spectrum of collective excitations, from a roton caused by the head-to-tail attraction of dipoles to a roton caused by the side-by-side repulsion, while there is no roton excitation for intermediate trap frequencies. We discuss the nature of these two kinds of rotons and the relation to instabilities of dipolar Bose gases. In both regimes of trap frequencies where rotons occur, we observe strong damping of collective excitations by decay into two rotons.

DOI
10.1103/physrevlett.107.065303

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We study the pair correlations and excitations of a dipolar Bose gas layer. The anisotropy of the dipole-dipole interaction allows us to tune the strength of pair correlations from strong to weak perpendicular and weak to strong parallel to the layer by increasing the perpendicular trap frequency. This change is accompanied by a roton-roton crossover in the spectrum of collective excitations, from a roton caused by the head-to-tail attraction of dipoles to a roton caused by the side-by-side repulsion, while there is no roton excitation for intermediate trap frequencies. We discuss the nature of these two kinds of rotons and the relation to instabilities of dipolar Bose gases. In both regimes of trap frequencies where rotons occur, we observe strong damping of collective excitations by decay into two rotons.
We study correlation effects and excitations in a dipolar Bose gas bilayer which is modeled by a one-dimensional double-well trap that determines the width of an individual layer, the distance between the two layers, and the height of the barrier between them. For the ground-state calculations we use the hypernetted-chain Euler-Lagrange method, and for the calculation of the excitations we use the correlated basis function method. We observe instabilities both for wide, well-separated layers dominated by intralayer attraction of the dipoles, and for narrow layers that are close to each other dominated by interlayer attraction. The behavior of the pair distribution function leads to the interpretation that the monomer phase becomes unstable when pairing of two dipoles becomes energetically favorable between or within layers, respectively. In both cases we observe a tendency towards ``rotonization,'' i.e., the appearance of a soft mode with finite momentum in the excitation spectrum. The dynamic structure function is not simply characterized by a single excitation mode but has a nontrivial multipeak structure that is not captured by the Bijl-Feynman approximation. The dipole-dipole interaction between different layers leads to additional damping compared to the damping obtained for uncoupled layers.
We predict the effect of the roton instability for a two-dimensional weakly interacting gas of tilted dipoles in a single homogeneous quantum layer. Being typical for strongly correlated systems, the roton phenomena appear to occur in a weakly interacting gas. It is important that in contrast to a system of normal to the layer dipoles, breaking of the rotational symmetry for a system of tilted dipoles leads to the convergence of the condensate depletion even up to the threshold of the roton instability, with mean-field approach being valid. Predicted effects can be observed in a wide class of dipolar systems. We suggest observing predicted phenomena for systems of ultracold atoms and polar molecules in optical lattices, and estimate optimal experimental parameters.
We study the effects of quasiparticle interactions in a quasi-two-dimensional (quasi-2D), zero-temperature Bose-Einstein condensate of dipolar atoms, which can exhibit a roton-maxon feature in its quasiparticle spectrum. Our focus is the Beliaev damping process, in which a quasiparticle collides with the condensate and resonantly decays into a pair of quasiparticles. Remarkably, the rate for this process exhibits a highly nontrivial dependence on the quasiparticle momentum and the dipolar interaction strength. For weak interactions, low-energy phonons experience no damping, and higher-energy quasiparticles undergo anomalously weak damping. In contrast, the Beliaev damping rates become anomalously large for stronger dipolar interactions, as rotons become energetically accessible as final states. When the dipoles are tilted off the axis of symmetry, the damping rates acquire an anisotropic character. Surprisingly, this anisotropy does not simply track the anisotropy of the dipolar interactions, rather, the mechanisms for damping are qualitatively modified in the anisotropic case. Our study reveals the unconventional nature of Beliaev damping in dipolar condensates, and has important implications for ongoing studies of equilibrium and nonequilibrium dynamics in these systems. Further, our results are relevant for other 2D superfluids with roton excitations, including spin-orbit-coupled Bose gases, magnon condensates, and 4He^{4}\mathrm{He}4He films.
We study the merging and splitting of quasi-two-dimensional Bose-Einstein condensates with strong dipolar interactions. We observe that if the dipoles have a non-zero component in the plane of the condensate, the dynamics of merging or splitting along two orthogonal directions, parallel and perpendicular to the projection of dipoles on the plane of the condensate are different. The anisotropic merging and splitting of the condensate is a manifestation of the anisotropy of the roton-like mode in the dipolar system. The difference in dynamics disappears if the dipoles are oriented at right angles to the plane of the condensate as in this case the Bogoliubov dispersion, despite having roton-like features, is isotropic.
We measure the excitation spectrum of a stable dipolar Bose-Einstein condensate over a wide momentum range via Bragg spectroscopy. We precisely control the relative strength ε_{dd} of the dipolar to the contact interactions and observe that the spectrum increasingly deviates from the linear phononic behavior for increasing ε_{dd}. Reaching the dipolar-dominated regime ε_{dd}>1, we observe the emergence of a roton minimum in the spectrum and its softening towards instability. We characterize how the excitation energy and the strength of the density-density correlations at the roton momentum vary with ε_{dd}. Our findings are in excellent agreement with numerical calculations based on mean-field Bogoliubov theory. When including beyond-mean-field corrections, in the form of a Lee-Huang-Yang potential, we observe a quantitative deviation from the experiment, questioning the validity of such a description in the roton regime.