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arXiv:1811.12115 · Physical Review Letters

Probing the Roton Excitation Spectrum of a Stable Dipolar Bose Gas

Daniel Petter, G. Natale, Rick van Bijnen, A. Patscheider, Manfred J. Mark, Lauriane Chomaz, Francesca Ferlaino

Published May 8, 2019• 135 citations
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Abstract

We measure the excitation spectrum of a stable dipolar Bose-Einstein condensate over a wide momentum range via Bragg spectroscopy. We precisely control the relative strength ε_{dd} of the dipolar to the contact interactions and observe that the spectrum increasingly deviates from the linear phononic behavior for increasing ε_{dd}. Reaching the dipolar-dominated regime ε_{dd}>1, we observe the emergence of a roton minimum in the spectrum and its softening towards instability. We characterize how the excitation energy and the strength of the density-density correlations at the roton momentum vary with ε_{dd}. Our findings are in excellent agreement with numerical calculations based on mean-field Bogoliubov theory. When including beyond-mean-field corrections, in the form of a Lee-Huang-Yang potential, we observe a quantitative deviation from the experiment, questioning the validity of such a description in the roton regime.

DOI
10.1103/physrevlett.122.183401

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We measure the excitation spectrum of a stable dipolar Bose-Einstein condensate over a wide momentum range via Bragg spectroscopy. We precisely control the relative strength ε_{dd} of the dipolar to the contact interactions and observe that the spectrum increasingly deviates from the linear phononic behavior for increasing ε_{dd}. Reaching the dipolar-dominated regime ε_{dd}>1, we observe the emergence of a roton minimum in the spectrum and its softening towards instability. We characterize how the excitation energy and the strength of the density-density correlations at the roton momentum vary with ε_{dd}. Our findings are in excellent agreement with numerical calculations based on mean-field Bogoliubov theory. When including beyond-mean-field corrections, in the form of a Lee-Huang-Yang potential, we observe a quantitative deviation from the experiment, questioning the validity of such a description in the roton regime.
Roton-type excitations usually emerge from strong correlations or long-range interactions, as in superfluid helium or dipolar ultracold atoms. However, in a weakly short-range interacting quantum gas, the recently synthesized spin-orbit (SO) coupling can lead to various unconventional phases of superfluidity and give rise to an excitation spectrum of roton-maxon character. Using Bragg spectroscopy, we study a SO-coupled Bose-Einstein condensate of ^{87}Rb atoms and show that the excitation spectrum in a "magnetized" phase clearly possesses a two-branch and roton-maxon structure. As Raman coupling strength Ω is decreased, a roton-mode softening is observed, as a precursor of the phase transition to a stripe phase that spontaneously breaks spatially translational symmetry. The measured roton gaps agree well with theoretical calculations. Furthermore, we determine sound velocities both in the magnetized and in the nonmagnetized phases, and a phonon-mode softening is observed around the phase transition in between. The validity of the f-sum rule is examined.
We observe signatures of radial and angular roton excitations around a droplet crystallization transition in dipolar Bose-Einstein condensates. In situ measurements are used to characterize the density fluctuations near this transition. The static structure factor is extracted and used to identify the radial and angular roton excitations by their characteristic symmetries. These fluctuations peak as a function of the interaction strength indicating the crystallization transition of the system. We compare our observations to a theoretically calculated excitation spectrum allowing us to connect the crystallization mechanism with the softening of the angular roton modes.
We discuss fluctuations in a dilute two-dimensional Bose-condensed dipolar gas, which has a roton-maxon character of the excitation spectrum. We calculate the density-density correlation function, fluctuation corrections to the chemical potential, compressibility, and normal (superfluid) fraction. It is shown that the presence of the roton strongly enhances fluctuations of the density, and we establish the validity criterion of the Bogoliubov approach. At T=0T=0T=0 the condensate depletion becomes significant if the roton minimum is sufficiently close to 0. At finite temperatures exceeding the roton energy, the effect of thermal fluctuations is stronger and it may lead to a large normal fraction of the gas and compressibility.
In a recent experiment, it has been found that by tuning the interaction strength of a dipolar Bose-Einstein Condensate confined in a quasi-1D geometry orthogonal to the polarization direction, the roton gap vanishes, while density modulations are induced in the trapped gas. This suggests the possibility of realizing a supersolid in dipolar quantum gases. Inspired by this experiment, we simulate a dipolar BEC in a ring geometry by confining the dipoles in a ”tube” orthogonal to the polarization direction and enforcing periodic boundary conditions. Our calculations are based on a Density Functional approach where the total energy density functional includes the beyond-mean-field correction of Lee-Huang-Yang, which partially accounts for quantum fluctuations. We study the ground state properties of the system by evolving in imaginary time the EulerLagrange equation derived from the variational principle. We also study the excitation spectrum of the system by solving the corresponding Bogoliubov-de Gennes equations. We find that the calculated excitation spectrum shows indeed a roton minimum, and the roton gap can become vanishingly small by reducing the effective scattering length. As the roton gap disappears, we find that the system spontaneously develops in its ground-state a periodic structure formed by denser clusters of atomic dipoles immersed in a dilute superfluid background. We find that this structure shows the hallmarks of a supersolid system, i.e. (i) a finite non-classical translational inertia and (ii) the appearance, besides the phonon mode, of the Nambu-Goldstone gapless mode corresponding to fluctuations in the phase, and related to the spontaneous breaking of the gauge symmetry.