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Physical Review A

Berry’s geometrical phases in ESR in the presence of a stochastic process

Dan Gamliel, Jack H. Freed

Published Apr 1, 1989• 58 citations
Publisher

Abstract

Berry's [Proc. R. Soc. London, Ser. A 392, 45 (1984)] geometrical phase is discussed in the context of dissipative evolution of an interacting spin system, governed by the stochastic Liouville equation. An analytical treatment is given for a possible ESR experiment on an interacting electron-nucleus system, modulated by two-site jumps. Geometrical phases are shown to be relevant to systems of this type, when their Hamiltonian changes slowly with time. A method for obtaining higher-order corrections to the adiabatic approximation is demonstrated. It is found that if the jumps are slow relative to the rate of change of the Hamiltonian, their effect reduces to familiar line broadening, and the geometrical phases may be observed experimentally. Equations are also set up for a similar ESR experiment on an electron-nucleus system undergoing isotropic rotational diffusion, and a brief discussion of the equations follows.

DOI
10.1103/physreva.39.3238

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Berry's [Proc. R. Soc. London, Ser. A 392, 45 (1984)] geometrical phase is discussed in the context of dissipative evolution of an interacting spin system, governed by the stochastic Liouville equation. An analytical treatment is given for a possible ESR experiment on an interacting electron-nucleus system, modulated by two-site jumps. Geometrical phases are shown to be relevant to systems of this type, when their Hamiltonian changes slowly with time. A method for obtaining higher-order corrections to the adiabatic approximation is demonstrated. It is found that if the jumps are slow relative to the rate of change of the Hamiltonian, their effect reduces to familiar line broadening, and the geometrical phases may be observed experimentally. Equations are also set up for a similar ESR experiment on an electron-nucleus system undergoing isotropic rotational diffusion, and a brief discussion of the equations follows.
We examine the role of Berry's geometrical phase [Proc. R. Soc. London, Ser. A 392, 45 (1984)] in the coherent excitation of atoms. The dynamics of a two-level atom prepared in a superposition of its eigenstates will be modified in a nontrivial fashion by the Berry phase. We extend Berry's formalism to treat the Liouville equation for the density matrix. This extension allows us to discuss statistical mixtures and to incorporate Berry's phase within the well-known Bloch-vector description of optical resonance. Furthermore, our density-matrix formalism provides the means of investigating Berry's phase in open, dissipative systems.
The generic Berry phase scenario in which a two-level system is coupled to a second system whose dynamical coordinate is slowly varying is generalized to allow for stochastic evolution of the slow system. The stochastic behavior is produced by coupling the slow system to a heat reservoir, which is modeled by a bath of harmonic oscillators initially in equilibrium at temperature TTT, and whose spectral density has a bandwidth that is small compared to the energy-level spacing of the fast system. The well-known energy-level shifts produced by Berry's phase in the fast system, in conjunction with the stochastic motion of the slow system, leads to a broadening of the fast system energy levels. In the limit of strong damping and sufficiently low temperature, we determine the degree of level broadening analytically, and show that the slow system dynamics satisfies a Langevin equation in which Lorentz-like and electriclike forces appear as a consequence of geometrical effects. We also determine the average energy level shift produced in the fast system by this mechanism.
According to Berry, quantum states of a hamiltonian which varies adiabatically through a circuit C in parameter space may acquire geometrical phase factors exp (iγ(C)) in addition to the normal dynamical phase factors exp ((-i/ħ) ∝ E(t) dt). We present N.M.R. experiments in the rotating frame which bear out these predictions for simple conical circuits, and point out that they are related to familiar behaviour based on the classical Bloch equations and on Haeberlen-Waugh coherent averaging theory. Extensions to coupled spins and electric quadrupolar effects are discussed.
Geometric phases in quantum mechanics play an extraordinary role in broadening our understanding of fundamental significance of geometry in nature. One of the best known examples is the Berry phase [M.V. Berry (1984), Proc. Royal. Soc. London A, 392:45], which naturally emerges in quantum adiabatic evolution. So far the applicability and measurements of the Berry phase were mostly limited to systems of weakly interacting quasi-particles, where interference experiments are feasible. Here we show how one can go beyond this limitation and observe the Berry curvature, and hence the Berry phase, in generic systems as a nonadiabatic response of physical observables to the rate of change of an external parameter. These results can be interpreted as a dynamical quantum Hall effect in a parameter space. The conventional quantum Hall effect is a particular example of the general relation if one views the electric field as a rate of change of the vector potential. We illustrate our findings by analyzing the response of interacting spin chains to a rotating magnetic field. We observe the quantization of this response, which we term the rotational quantum Hall effect.
In this work, we make a review of the literature that the so-called Berry’s geometric phase. A recent issue, which has been employed in various areas of physics. For this, we use, in a number of references, in which many were critical to the theoretical foundation of this work. At first, we focus on the study of the time evolution of quantum systems governed by Hamiltonians operators whose time dependence is manifested by a set of parameters called classical fields. The adiabatic approximation, is justified mathematically when demonstrated the adiabatic theorem. Under these conditions, we obtain geometric phases - Berry’s phase - associated with these systems in different representations, each displaying its particularity. Finally, as a particular case of geometric phase, we studi from the viewpoint of duality transformations of Maxwell’s equations, the dual Aharonov-Bohm effect, extracting the geometric Berry’s phase associated with the dynamics of the magnetic monopole in the presence of the electric vector potential
A precise definition of an adiabaticity parameter \ensuremath{\nu} of a time-dependent Hamiltonian is proposed. A variation of the time-dependent perturbation theory is presented which yields a series expansion of the evolution operator U(\ensuremath{\tau})=${\ensuremath{\sum}}_{\mathrm{\ensuremath{\ell}}}$${\mathrm{U}}^{(\mathrm{\ensuremath{\ell}})}$(\ensuremath{\tau}) with ${\mathrm{U}}^{(\mathrm{\ensuremath{\ell}})}$(\ensuremath{\tau}) being at least of the order ${\ensuremath{\nu}}^{\mathrm{\ensuremath{\ell}}}$. In particular, U(0){\mathrm{U}}^{(0)}U(0)(\ensuremath{\tau}) corresponds to the adiabatic approximation and yields Berry's adiabatic phase. It is shown that this series expansion has nothing to do with the 1/\ensuremath{\tau} expansion of U(\ensuremath{\tau}). It is also shown that the nonadiabatic part of the evolution operator is generated by a transformed Hamiltonian which is off-diagonal in the eigenbasis of the initial Hamiltonian. This suggests the introduction of an adiabatic product expansion for U(\ensuremath{\tau}) which turns out to yield exact expressions for U(\ensuremath{\tau}) for a large number of quantum systems. In particular, a simple application of the adiabatic product expansion is used to show that for the Hamiltonian describing the dynamics of a magnetic dipole in an arbitrarily changing magnetic field, there exists another Hamiltonian with the same eigenvectors for which the Schr\"odinger equation is exactly solvable. Some related issues concerning geometric phases and their physical significance are also discussed.