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Optica Acta International Journal of Optics

Laser Cooling of Magnesium Ions Confined in a Penning Trap

Richard Claude Thompson, G. P. Barwood, Patrick Robert Gill

Published Apr 1, 1986• 16 citations
Publisher

Abstract

The construction of a Penning ion trap is described. The trap has been used to confine clouds of magnesium ions for periods of many hours and the ions have been cooled to sub-kelvin temperatures by the method of laser cooling. Preliminary experiments with the cooled ions are reported.
DOI
10.1080/713821957

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•May 21, 1990•0 citations
This thesis describes experimental work performed on laser cooled magnesium ions, confined in a quadrupole ion trap operating in the Penning or the combined mode. Information is gained about the dynamical motion of the ions. This is done by analyzing the time delays between scattered fluorescence photons in the case of small ion clouds (generally less than ten ions). For larger clouds (upwards of 100 ions), a fraction of the ions is "tagged" and a subsequent study made of the time evolution of the fluorescence. We have developed an innovative, non-invasive method for measuring ion oscillation frequencies which is based on analyzing photon-photon correlations present in the emitted ion fluorescence. This technique has been used to measure all three Penning trap frequencies for a wide range of dc voltage. The data have been fitted to theory and we have obtained a global fit of these data to one set of trap parameters. We also demonstrate that our technique enables us to measure space-charge shifted values of the trap resonances. This method has also been applied to the combined trap and we report experimental verification of the predicted trap resonances for a wide range of trapping parameters. These data fit well to theory. This is for all three oscillation frequencies for one set of trap parameters consistent with the data for the Penning trap. \nFurther experiments are reported concerned with the dynamics of larger ion clouds in a Penning trap. A pulsed laser is used to "tag" a small number of the ions in large ion clouds. This removes those ions from the cooling cycle by placing them in a metastable state. Subsequently, we have monitored the time evolution of the fluorescence. By analyzing these data we have been able to determine cloud rotation frequencies for large ensembles of ions.
In this work, laser-cooled ion crystals containing 1000 to 100000 singly charged magnesium ions (Mg+) were prepared in a Penning trap. The properties of the ion crystals and their structure displaying long-range ordering were analyzed by various non-destructive techniques. After creation of the Mg + ions in the form of ion bunches in an external source, the ions were injected into the Penning trap where their temperature was reduced by eight orders of magnitude within seconds using a combination of buffer gas cooling and Doppler laser cooling. The achieved temperatures in the millikelvin-regime were close to the theoretical Doppler-cooling limit and sufficiently low to induce the transition to a crystal phase exhibiting long-range ordering. The structure of these mesoscopic ion crystals is in agreement with a model describing the crystal as a set of planar shells. This allows for a derivation of properties such as the charge density or the temperature of the observed crystals. For the process of combined buffer-gas and Doppler laser cooling an analytical model has been developed, which explains the time development of the temperature and the fluorescence signal in agreement with the experimental results.
We have performed laser cooling of Mg+{}^{+}+ ions confined in a Penning trap. The externally produced ions were captured in flight, stored, and laser cooled. Laser-induced fluorescence was observed perpendicular to the cooling laser axis. Optical detection down to the single-ion level together with the electronic detection of the ion oscillations inside the Penning trap have been used to acquire information on the ion storage time, ion number, and ion temperature. Evidence for the formation of ion crystals has been observed. These investigations are an important prerequisite for the sympathetic cooling of simultaneously stored highly charged ions and the precision laser spectroscopy of forbidden transitions in these.
We report the first demonstration of the axialization of laser cooled ions in a Penning trap. Axialization involves the application of a small radial quadrupole drive which couples the cyclotron and magnetron motions. This enhances the laser cooling, allowing tighter confinement of the ions to the central axis of the trap than is otherwise possible. Using an intensified charge-coupled device (ICCD) camera we have imaged the axialization process for the first time. For a single ion, we recorded a large decrease of the magnetron amplitude corresponding to a reduction in ion temperature of approximately 2 orders of magnitude to an upper limit of order 10 mK. We have discovered dynamics specific to the laser cooled system which depend critically on the axial drive frequency and amplitude.
We have recently constructed an ion trapping and laser cooling system at Imperial College suitable for magnesium ions. This system consists of a Penning ion trap contained within an all-metal vacuum system maintained below 3 × 10−10 mbar. Also enclosed in the vacuum system are small magnesium beam ovens made of tantalum foil and resistively heated by a current of typically 6 A. The ring electrode (see Fig. 1) is kept at a negative potential with respect to the endcaps, and the magnetic field of ~1 T perpendicular to the plane of the ring causes the ions to move in closed orbits within the trap.