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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Rabi oscillations in many-level quantum system

Alexander Alexandrovich Biryukov, B. V. Danilyuk

Published Mar 3, 2008• 3 citations
Publisher

Abstract

The object of the research are the quantum transitions of a many-level system between its stationary states under the influence of an alternating external electric field. The transition amplitudes and probabilities are calculated by the method of perturbation theory in the approximation of a classical external field. It is illustrated that in the case when the external field frequency is equal to the frequency of any quantum transition, then the probability of this transition fluctuate nearly the average value which is oscillating with Rabi frequency. Probabilities of other quantum transitions are very small and change chaotically with time.

DOI
10.1117/12.801584

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arXiv:1807.05086•Physical Review A•Oct 5, 2018•24 citations
The object of the research are the quantum transitions of a many-level system between its stationary states under the influence of an alternating external electric field. The transition amplitudes and probabilities are calculated by the method of perturbation theory in the approximation of a classical external field. It is illustrated that in the case when the external field frequency is equal to the frequency of any quantum transition, then the probability of this transition fluctuate nearly the average value which is oscillating with Rabi frequency. Probabilities of other quantum transitions are very small and change chaotically with time.
The transitions between stationary states in multilevel quantum system under the influence of an alternating external electric field are considered in this work. Herewith the strength of external electric field changes with time by the harmonic law. The analytical expressions for quantum transitions probabilities of a system are given at the third order of perturbation theory. The dependencies of quantum transitions probabilities and average energy of a system upon interaction time and frequency of field are investigated in the case when the system is a charged particle in rectangular infinitely deep potential pit.
We study the dynamics of multi-level quantum systems under the influence of electromagnetic field.Basing on the path integral approach to the quantum density matrix and transitions probability we represent functional averaging electromagnetic field influence.We demonstrate that the transition probability can be written as a path integral of real functional (the product of exponent and cosine).The numerical integration algorithm of the transitions probability in energy representation was developed.The numerical simulations of the quantum system dynamics under electromagnetic field action describe the well-known Rabi oscillations, their fluctuations and multi-photon quantum transitions.
The problem of the interaction of a quantum system having discrete states, with a classical oscillating field, is reexamined as a problem in the solution of the time-dependent Schrodinger equation with a periodic Hamiltonian. A method is presented for approximating the time-dependent Hamiltonian with a time-independent one in the weak oscillating field case. With the aid of Floquet's theorem the problem is exactly converted to one with a time-independent Hamiltonian represented by an infinite matrix. The approximation of only two states then permits finding the resonance line shape by perturbation theory for both single and multiple quantum transitions with equal ease. The simple case of only two states connected by an off diagonal sinusoidal perturbation is studied in detail, and a complete description of the average transition probability is found for the strong oscillating field case. A few more complex cases are discussed. A deeper understanding of the analysis is obtained by examining the theory with the oscillating field quantized. Experimental verification of the theory could best be obtained by the methods of atomic beam spectroscopy at radio frequencies.
The ‘phase-space’ method in quantum theory is used to derive exact expressions for the transition probabilities of a perturbed oscillator. Comparison with the approximate results obtained by perturbation methods shows that the latter must be multiplied by an exponential factor exp (− ∊/ℏω), where ∊ is the non-fluctuating part of the work done by the perturbing forces; as long as ∊ is small, exp (− ∊/ℏω) ˜ 1 and only dipole transitions have an appreciable probability. As the perturbation energy increases, however, this is no longer true, and multipole transitions become progressively more probable, the most probable ones being those for which the change in energy is approximately equal to the work done by the perturbing forces.
The multiple-linear-time-scale method is used to construct a perturbation theory for NNN-level quantum systems subjected to time-dependent perturbations. The secular and small-denominator terms which plague conventional time-dependent perturbation theory are avoided; consequently, the theory is useful for treating long-term behavior and resonant interactions. The introduction of a self-energy operator allows the shifts in energy levels to be displayed explicitly. When the perturbation is the dipole interaction with an electromagnetic field, the successive approximations yield the well-known rotating-wave approximation, corrections due to counter rotating terms, and the Bloch-Siegert frequency shift. The formalism is applicable to arbitrary pulse shapes, provided that $\ensuremath{\parallel}{H}_{1}\ensuremath{\parallel}\ensuremath{\ll}\ensuremath{\hbar}\overline{\ensuremath{\omega}}$, where $\ensuremath{\parallel}{H}_{1}\ensuremath{\parallel}$ represents the inter-action strength and $\overline{\ensuremath{\omega}}$ is a characteristic frequency of the field. Rabi oscillations induced by multiphoton resonances are automatically included, and this effect is demonstrated in the case of a square pulse with frequency approximately one half the resonance frequency for a transition between two vibrational levels of a molecule. These calculations are compared to an exact numerical solution in order to find the limits of validity of the approximation. Even at high intensities ($I\ensuremath{\sim}{10}^{14}$ W/cm2{\mathrm{cm}}^{2}cm2) the shifted resonance frequency is quite accurate; however, the approximate and exact solutions are slightly out of phase, so that the approximate solution can only be trusted for a few Rabi cycles. For much lower intensities ($I\ensuremath{\sim}{10}^{10}$ W/cm2{\mathrm{cm}}^{2}cm2), the approximate solution is valid for many thousands of Rabi cycles.
In the framework of the nonsecular perturbation theory based on the Bogoliubov averaging method, the coherent dynamics of multiphoton Raman transitions in a two-level spin system driven by an amplitude-modulated microwave field is studied. Closed-form expressions for the Rabi frequencies of these transitions are obtained beyond the rotating-wave approximation for the low-frequency driving component. It is shown that spin states dressed by the high-frequency component of the driving field are shifted due to the Bloch-Siegert-like effect caused by antiresonant interactions with the strong low-frequency driving. We predict that with increasing the order of the Raman transition, the Rabi frequency decreases and the contribution of the Bloch-Siegert shift to this frequency becomes dominant. It is found that the amplitude and phase of the Rabi oscillations strongly depend on the initial phase of the low-frequency field as well as on detuning from multiphoton resonance. The recent experimental data for the second- and third-order Raman transitions observed for the nitrogen-vacancy center in diamond (Z. Shu et al., arXiv:1804.10492) are well described in the frame of our approach. Our results may provide new possibilities for coherent control of quantum systems.