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Physics Letters A

Radiative lifetimes of superradiant populated Ba Rydberg levels

C. Leonard, R.-H. Rinkleff

Published Oct 1, 1985• 4 citations
Publisher
DOI
10.1016/0375-9601(85)90504-3

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We report the observation of unusual doubly excited states of barium: Ba (5dj, 21c). One of the valence electrons of Ba is prepared in an oriented circular Rydberg state (n = 21, l = m = 20, denoted 21c) by the adiabatic crossed-fields method. The other electron is excited to a 6pj state which decays radiatively to a 5dj metastable level. The measured autoionization lifetime of Ba (5d5/2, 21c) is T ~ 1 μ s , whereas for Ba (5d3/2, 21c), τ is estimated to be longer than 400 μs. This very large difference of lifetimes between the fine-structure states of the inner electron has been analysed.