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Physical Review A

Experimental study of one- and two-photon Rabi oscillations

T. Gentile, Barbara J. Hughey, Daniel Kleppner, Theodore W. Ducas

Published Nov 1, 1989• 125 citations
Publisher

Abstract

We report an experimental study of one- and two-photon Rabi oscillations and other coherent effects in microwave transitions between Rydberg states of calcium. Selective field ionization allows us to observe the time evolution of both the initial and final states with high discrimination. The experiments include measurements of the dependence of the one- and two-photon oscillation frequencies on microwave power and detuning from resonance. We have used the off-resonant behavior of the two-photon oscillation frequency to measure the ac Stark shift. In a magnetic field we have also observed the free evolution of the magnetic sublevels and the effect of Zeeman splitting on the one-photon Rabi oscillations. The theory for these experiments is presented; our results are in excellent agreement.

DOI
10.1103/physreva.40.5103

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We report an experimental study of one- and two-photon Rabi oscillations and other coherent effects in microwave transitions between Rydberg states of calcium. Selective field ionization allows us to observe the time evolution of both the initial and final states with high discrimination. The experiments include measurements of the dependence of the one- and two-photon oscillation frequencies on microwave power and detuning from resonance. We have used the off-resonant behavior of the two-photon oscillation frequency to measure the ac Stark shift. In a magnetic field we have also observed the free evolution of the magnetic sublevels and the effect of Zeeman splitting on the one-photon Rabi oscillations. The theory for these experiments is presented; our results are in excellent agreement.
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We report on high-resolution microwave spectroscopy of cesium Rydberg $(n+2){D}_{5/2}\ensuremath{\rightarrow}n{F}_{J}$ transitions in a cold atomic gas. Atoms laser-cooled and trapped in a magnetic-optical trap are prepared in the DDD Rydberg state using a two-step laser excitation scheme. A microwave field transmitted into the chamber with a microwave horn drives the Rydberg transitions, which are probed via state selective field ionization. Varying duration and power of the microwave pulse, we observe Fourier sideband spectra as well as damped, on-resonant Rabi oscillations with pulse areas up to $\ensuremath{\gtrsim}3\ensuremath{\pi}$. Furthermore, we investigate the Zeeman effect of the clearly resolved nFJn{F}_{J}nFJ​ fine-structure levels in fields up to 120 mG, where the transition into nF7/2n{F}_{7/2}nF7/2​ displays a thee-peak Zeeman pattern, while nF5/2n{F}_{5/2}nF5/2​ shows a two-peak pattern. Our theoretical models explain all observed spectral characteristics, showing good agreement with the experiment. Our measurements provide a pathway for the study of high-angular-momentum Rydberg states, initialization and coherent manipulation of such states, Rydberg-atom macrodimers, and other Rydberg-atom interactions. Furthermore, the presented methods are suitable for calibration of microwave radiation as well as for nulling and calibration of dc magnetic fields in experimental chambers for cold atoms.
We report on an experimental study of the frequency dependence of the microwave ``ionization'' probability for laser-excited Rb(np)2{)}^{2})2P3/2{\mathit{P}}_{3/2}P3/2​(\ensuremath{\Vert}MJ{\mathit{M}}_{\mathit{J}}MJ​\ensuremath{\Vert}=1/2) Rydberg atoms. Most data are for n=84. The microwave field was produced by a low-noise frequency synthesizer, and the laser-excited atoms subsequently driven by microwaves were kept in an environment cooled to 77 K in order to minimize the perturbing effects of the thermal, blackbody-radiation field. The driving frequency covered 4--14-MHz intervals around three frequencies between 8.87 and 16.14 GHz. Data are shown for 1- and 5-\ensuremath{\mu}s interaction times, which correspond to the driving frequency being resolved by the atoms to about 1 and 0.2 MHz, respectively. The turnon and turnoff parts of the microwave pulse shape were slow, lasting about 6 ns (circa 70 field oscillations). For the narrow frequency intervals used, the microwave field amplitude was calibrated in situ with use of two-photon Rabi-nutation measurements, which also directly demonstrated the spatial uniformity of the driving field amplitude and its coherence over at least a 1-\ensuremath{\mu}s time scale. Within the frequency intervals studied experimentally, we have observed no sharp, frequency-dependent structure outside of that expected from experimental counting statistics. We give physical arguments based on experimental data and previous experimental and theoretical work on microwave ``ionization'' that show that the present experiments have been in the range of the scaled frequency above 1. Thus, these experimental data examine in a continuous fashion the frequency dependence of microwave ``ionization'' in the high-scaled-frequency regime. Finally, we discuss our results in the light of published theoretical discussions of what might be expected to be the frequency dependence of the microwave ``ionization'' probability for various quantal models for the one-dimensional hydrogen atom in this high-frequency regime.
Experimental results of studying the spectrum of the microwave 37 P -37 S transition of Rydberg sodium atoms in a weak magnetic field (≤7 G) are reported. The populations of the Rydberg states were measured using the method of selective ionization with a pulsed electric field. When the magnetic field was parallel to the ionizing electric field, a good agreement between the calculated and experimental spectral shapes was observed, making it possible to determine the unknown polarization of the microwave radiation. In the case of the orthogonal configuration of the fields, the resonance structure was suppressed in the field ionization signals due to the strong influence of the magnetic field on the electron trajectories in the detection system.
Rabi oscillations have been observed in many superconducting devices, and represent prototypical logic operations for quantum bits (qubits) in a quantum computer. We use a three-level multiphoton analysis to understand the behavior of the superconducting phase qubit (current-biased Josephson junction) at high microwave drive power. Analytical and numerical results for the ac Stark shift, single-photon Rabi frequency, and two-photon Rabi frequency are compared to measurements made on a dc SQUID phase qubit with Nb/AlOx/Nb tunnel junctions. Good agreement is found between theory and experiment.
We present a two-photon microwave spectra of cesium Rydberg atoms in the room-temperature vapor cell. The three-level atom including a ground state 6S1/2 (F = 4), an excited state 6P3/2 (F′ = 5) and Rydberg state consists of Rydberg electromagnetically induced transparency (Rydberg-EIT), that is employed to detect the microwave two-photon spectra. The microwave field with frequency ν DD = 11.42865 GHz couples the transition of Rydberg energy level |68D5/2〉 → |69D5/2〉, measured two-photon spectra display a rich of information including the microwave ac Stark shifts and two-photon Autler-Townes (AT) splitting. In the strong microwave field, the two-photon spectroscopy shows the state mixture between |68D5/2〉 and |68D3/2〉 Stark lines. The microwave two-photon spectra of the |69S1/2〉 → |70S1/2〉 transition coupled with frequency ν SS = 11.73503 GHz are also presented. The Floquet theory is employed to simulate the two-photon microwave spectra, showing the good agreement with the measurements. The work suggests the new method that may be used to investigate the multi-photon field-atom interaction and as an atom-based technique for precision field measurements.