We have calculated the magnetic dipolar spin-relaxation rates of magnetically trapped doubly-spin-polarized atomic deuterium gas. The results are expressed in a simple closed formula describing the dipolar-relaxation-limited stability in the Boltzmann ($T\ensuremath{\gg}{T}_{F}$), the degeneracy ($T\ensuremath{\ll}{T}_{F}$), and the crossover ($T\ensuremath{\simeq}{T}_{F}$) regimes. In the degeneracy regime we typically find lifetimes of some hours. We also discuss the dipolar decay of magnetically trapped spin-polarized fermionic alkali-metal atoms.
We study the decay of magnetically trapped doubly spin-polarized atomic hydrogen in the density and temperature regime of the Bose-Einstein phase transition and calculate the temperature and magnetic field dependence of all relevant relaxation rate constants ${G}_{\mathrm{dd}\ensuremath{\rightarrow}\ensuremath{\kappa}\ensuremath{\lambda}}$. At the transition temperature
Tc the rate constants have a discontinuous second derivative with respect to T. Below
Tc they show a pronounced decrease relative to the extrapolated above-
Tc values, the observation of which is a clear signal for the experimental realization of Bose-Einstein condensation.
We study hyperfine transitions in collisions between cold ground-state
23Na atoms, which are of crucial importance for the decay of the atomic density in magnetic traps. For comparable densities we find the initial decay by exchange collisions to be roughly a factor of 10 more rapid than that in atomic hydrogen. The doubly polarized atomic gas that thus forms spontaneously in this initial process subsequently decays by dipolar relaxation with a rate that is about a factor of 5 larger than that in atomic hydrogen. The sensitivity of the calculated rate constants associated with uncertainties in the singlet and triplet potentials is discussed.
We have studied relaxation and recombination processes in compressed, doubly polarized atomic hydrogen at temperatures from 0.13 to 0.60 K and magnetic fields from 3 to 9 T. The gas and surface dipole three-body recombination rate constants at a field of 7.6 T are measured to be, respectively,
Lg=8.9(8)\ifmmode\times\else\texttimes\fi{}${10}^{\mathrm{\ensuremath{-}}39}$
cm6 ${\mathrm{s}}^{\mathrm{\ensuremath{-}}1}$ and
Ls=1.2(4)\ifmmode\times\else\texttimes\fi{}${10}^{\mathrm{\ensuremath{-}}24}$
cm4 ${\mathrm{s}}^{\mathrm{\ensuremath{-}}1}$. They decrease slowly with field and
Ls exhibits no significant angular dependence. The three-body recombination rate due to hyperfine mixing has also been measured. Electronic and nuclear relaxation rates have been measured; the b-c electronic relaxation rate constant in the gas is
Gbc=1.03(7)\ifmmode\times\else\texttimes\fi{}${10}^{\mathrm{\ensuremath{-}}15}$
cm3 ${\mathrm{s}}^{\mathrm{\ensuremath{-}}1}$exp(-
Ebc/
kBT). The temperature and field dependence of the nuclear relaxation rate in the gas are observed to be in excellent agreement with recent theoretical calculations. Three-body surface recombination-rate measurements using $^{3}\mathrm{\ensuremath{-}}^{4}$He surfaces indicate that as little as one monolayer of
3He on the liquid
4He surface appreciably decreases the adsorption energy of atomic hydrogen. Densities achieved include 4.5\ifmmode\times\else\texttimes\fi{}
1018 atoms${\mathrm{?}}^{\mathrm{\ensuremath{-}}3}$ at 0.55 K (pure
4He walls), and 1.4\ifmmode\times\else\texttimes\fi{}
1018 atoms${\mathrm{?}}^{\mathrm{\ensuremath{-}}3}$ at 0.19 K (8 at. ? sup 3---He).
We have studied spin-polarized deuterium, ${\mathrm{D}}_{\ensuremath{\downarrow}}$, in the temperature range 0.3 to 0.7 K in a field of 40 kG using electron-spin resonance at 114 GHz. The intrinsic rates for recombination of two D atoms to form
D2 on the surface of $l\ensuremath{-}^{4}\mathrm{He}$ have been measured for both the ortho and para channels. The two rates are approximately equal and when extrapolated to zero field are 1600 times greater than the rates for
H2 formation. Doubly spin-polarized deuterium, ${\mathrm{D}}_{\ensuremath{\downarrow},↡}$, has been observed for the first time, with nuclear-spin purities > 0.98 and sample lifetimes as long as 1 h.