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Physical Review A

Optical modulation transfer by molecular modulation

Jian Wu, Heping Zeng

Published Nov 15, 2004• 0 citations
Publisher

Abstract

Modulation features in the frequency domain can be transferred from an amplitude-modulated laser field to a nonmodulated one by a strong Raman coupling, which is based on refractive index control with a strong Raman coherence established with two sufficiently intense laser fields slightly off the two-photon Raman resonance of a selected Raman mode. Numerical simulations show that modulation transfers between the driving lasers, such as transfers from ultraviolet to extreme ultraviolet and from infrared to middle infrared lasers, can be realized in gaseous Raman media. This provides an efficient way to extend the optical modulation range beyond the transparent ranges of commercial modulators. Modulation features can also be transferred from a low-intensity driving laser to a high-intensity one, which ensures a direct application to modulate lasers with high intensities beyond the damage thresholds of standard modulators.

DOI
10.1103/physreva.70.053815

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Modulation features in the frequency domain can be transferred from an amplitude-modulated laser field to a nonmodulated one by a strong Raman coupling, which is based on refractive index control with a strong Raman coherence established with two sufficiently intense laser fields slightly off the two-photon Raman resonance of a selected Raman mode. Numerical simulations show that modulation transfers between the driving lasers, such as transfers from ultraviolet to extreme ultraviolet and from infrared to middle infrared lasers, can be realized in gaseous Raman media. This provides an efficient way to extend the optical modulation range beyond the transparent ranges of commercial modulators. Modulation features can also be transferred from a low-intensity driving laser to a high-intensity one, which ensures a direct application to modulate lasers with high intensities beyond the damage thresholds of standard modulators.
We propose the extension of existing molecular modulation techniques for continuous-wave optical modulation to Raman-active microresonators. Intense pump and Stokes modes inside a microresonator prepare a high coherence of the Raman transition between two ro-vibrational states. With the coherence prepared, any laser in the optical region can be coupled to the microresonator and be modulated. We perform numerical simulations which predict that these "microresonator-based molecular modulators" could have modulation efficiencies on the order of 1% at 10 THz-scale frequencies for any optical wavelength.
We suggest that subfemtosecond pulses can be generated by using high-order stimulated Raman scattering when a Raman transition is driven by three intense single-mode laser beams with two different modulation frequencies. An oscillatory strong Raman coherence is established by the modulated molecular modulation. Numeric simulations based on the first fundamental vibrational Raman transition of gaseous and solid deuterium indicate that subfemtosecond pulses can be generated by Raman excitations with above, below, or opposite Raman detunings.
We suggest a technique where a molecular Raman transition is prepared near a maximally coherent state with continuous-wave (CW) laser beams. The key idea is to put the molecules inside a high-finesse cavity and to drive the molecular transition with two lasers whose frequency difference is slightly detuned from the Raman resonance. In this regime, the molecules become very efficient CW modulators with a modulation frequency that can be as high as 100THz100\phantom{\rule{0.3em}{0ex}}\mathrm{THz}100THz.
We have demonstrated that coherent molecular modulation can result in the collinear generation of mutually-coherent spectral sidebands that extend in frequency from the infrared to the far ultraviolet. Our technique is based on adiabatic preparation of a highly coherent molecular superposition-state, which is achieved by using narrow-linewidth lasers slightly detuned from a Raman resonance. The phases of the resultant Stokes and anti-Stokes sidebands are adjusted in order to synthesize desired single-cycle pulse trains at the target. In this article we review recent improvements and developments in this area, including: techniques for increasing the number of generated sidebands; synchronization of the pulse trains with the molecular motion in the given molecular system; laser self-focusing and spatial soliton formation due to the coherent interaction of light with oscillating molecules. In the future, this Raman source may produce sub-cycle optical pulses, and allow synthesis of waveforms where the electric field is a predetermined function of time, not limited to a quasi-sinusoidal oscillation.
An ultrafast light-intensity modulator, based on stimulated Raman scattering, is described. The intensity of a continuous wave laser is fully modulated at 17THz using hydrogen in a high-finesse cavity. The modulation frequency is determined by the molecular constant of the Raman medium, i.e., the Raman shift frequency. The modulation frequency can be changed in the tetrahertz range by replacing the Raman medium. Due to the accurate modulation frequency and the high beam coherence, this device is amenable to a variety of applications such as in basic science and also in advanced industrial technology.