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Physical Review

Normal-Fermi-Liquid Theory for Electrons in Solids

B. L. Jones, J. W. McClure

Published Mar 4, 1966• 20 citations
Publisher

Abstract

A Landau-type Fermi-liquid theory for interacting electrons moving in a fixed periodic potential is derived. Two methods are used: the Green's-function method, which gives a more physical description of the system but does not give all the desired results, and the many-body perturbation-theory approach, which is complete but is more complicated. The Green's-function formalism of Kadanoff and Baym is adapted to inhomogeneous systems by rewriting it in operator form. A kinetic equation for an energy-dependent, single-particle density matrix is then derived. The quasiparticle concept is introduced and a formal solution of the kinetic equation is given and discussed. These developments are specialized to the periodic potential and a transport equation of the Landau-Boltzmann type is derived for quasiparticles moving within a single energy band. Expressions for the density and current density are then identified from a continuity equation. Although the present work does not treat real transitions between energy bands, the Green's-function method suggests a plausible form for a Landau-like theory which includes such transitions. The perturbation-theory treatment follows the work of Luttinger and Nozi\`eres, who derived Landau's theory for systems without a lattice potential. When the perturbation theory is expressed in terms of Bloch functions, the quantities involved become matrices between different energy bands. However, it is shown that many of the key results of Luttinger and Nozi\`eres can be suitably generalized. The perturbation-theory calculation shows that when the periodic potential is present the change in quasiparticle energy can still be expressed in terms of the variation of the quasiparticle distribution function, and that the results obtained from the Green's-function approach are exact in the case of slowly varying external fields.

DOI
10.1103/physrev.143.133

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A Landau-type Fermi-liquid theory for interacting electrons moving in a fixed periodic potential is derived. Two methods are used: the Green's-function method, which gives a more physical description of the system but does not give all the desired results, and the many-body perturbation-theory approach, which is complete but is more complicated. The Green's-function formalism of Kadanoff and Baym is adapted to inhomogeneous systems by rewriting it in operator form. A kinetic equation for an energy-dependent, single-particle density matrix is then derived. The quasiparticle concept is introduced and a formal solution of the kinetic equation is given and discussed. These developments are specialized to the periodic potential and a transport equation of the Landau-Boltzmann type is derived for quasiparticles moving within a single energy band. Expressions for the density and current density are then identified from a continuity equation. Although the present work does not treat real transitions between energy bands, the Green's-function method suggests a plausible form for a Landau-like theory which includes such transitions. The perturbation-theory treatment follows the work of Luttinger and Nozi`eres, who derived Landau's theory for systems without a lattice potential. When the perturbation theory is expressed in terms of Bloch functions, the quantities involved become matrices between different energy bands. However, it is shown that many of the key results of Luttinger and Nozi`eres can be suitably generalized. The perturbation-theory calculation shows that when the periodic potential is present the change in quasiparticle energy can still be expressed in terms of the variation of the quasiparticle distribution function, and that the results obtained from the Green's-function approach are exact in the case of slowly varying external fields.
On the basis of the Kadanoff-Baym (KB) version of the time-dependent Green's function method, an Ansatz for the approximation of a spectral function is offered. The Ansatz possesses all the advantages of quasiparticle and extended quasiparticle approximations and satisfies the KB equation for a spectral function in the case of slightly nonequilibrium system when disturbances in space and time are taken into consideration in the gradient approximation. This feature opens opportunities for the microscopic derivation of the Landau kinetic equation for the quasiparticle distribution function of the normal Fermi liquid and provides the widening of these equations' temperature range of validity.
The phenomenological theory of a Fermi liquid is generalized to nonequilibrium conditions. Landau's theory is reformulated to include fluctuations of the distribution function and quasiparticle energy. The method of fluctuation in kinetic equations is used to establish the collision integral of the quasiparticle Boltzmann equation. This collision integral is expressed in terms of the parameters of Landau's theory, and includes dynamic screening effects. The results are compared with recent theories of transport in Fermi liquids.
The individual particle theory of many body systems was studied starting from a microscopic point of view. A technique which is equivalent to a generalized thermodynamics was used to show that, under the appropriate conditions of temperature and external field, the quasi-particle approach is correct for three very dissimilar systemsi the normal degenerate Fermi system, the metallic electron-phonon system, and the polaron. The fact that an approach like this works for such dissimilar systems emphasizes the underlying unity of the quasi-particle models. The concept that the real t~me non-equilibrium self-energy and the incoherent part of the density-density correlation function may be generated as functional derivatives of a generalized thermodynamic potential (~), together with local translational and rotational invariance and Galilean relativity, leads to a transformation from the microscopic particle density variables g«p,m,R,T) to those of the quasi-particle theory n (R,T). ~ - p- It was shown that, for zero temperature, such a ~ derivability is exact; at low temperature and for slowly varying fields, this ~ derivability is approximately true. This was shown by a procedure which is eqUivalent to an expansion in terms of the real scattering probability for quasiparticles. At low temperature and for slowly varying fields, such real scattering is very improbable and the expansion parameter is small. Perturbation theory was used only to determine the actual size of terms which, on physical grounds are necessarily small. As such, this approach is non-perturbative, depending only on properties of the exact selfenergies and correlation functions. In addition to demonstrating that the quasi-particle models are correct, information on the regions of validity for ~hese models is obtained. .As by-products of these derivations, microscopic expressions for the parameters of the quasi-particle theory and simple microscopic expressions for the currents in degenerate Fermi systems and the electron-phonon system are obtained.
The methods employed in the previous papers of this series for the ground-state energy of a normal Fermion system are extended to finite temperatures. The basic assumption is that the density matrix of the actual system in thermodynamic equilibrium can be derived by adiabatic transformation from the density matrix of system of noninteracting particles at the same temperature, volume, and chemical potential. However, the spectrum of the noninteracting system must be dependent on the intensive parameters. The self-consistency of the scheme is exhibited by demonstrating that the effective potential characterizing this system can be related to the self-energy operator of the actual system. Two equivalent versions of the theory are derived. In one of these the basic equations are precisely those of the Landau theory of Fermi liquids with the difference, however, that all quantities are given explicitly from first principles.
In Landau's phenomenological Fermi-liquid theory (FLT), most physical quantities are derived from the knowledge of the energy variation δE[δn] corresponding to a change δn of the quasi-particle (QP) distribution function n≡{nkσ}. We show that the internal energy E[n] (or, more precisely, the thermodynamic potential Φ[n]), expressed as a function of the QP distribution n, can be interpreted as an effective potential (in the sense of field theory), which is obtained from the free energy by a Legendre transformation. This allows to obtain explicitly δΦ (or δE) starting from a microscopic Hamiltonian and to relate the Landau f function to the forward-scattering two-particle vertex without considering the collective modes as in the standard diagrammatic derivation of FLT. Out-of-equilibrium properties are obtained by extending the definition of the effective potential to space- and time-dependent configurations. Φ[n] is then a functional of the Wigner distribution function n≡{nkσ (r,t)}. It contains information about both the static and dynamic properties of the Fermi liquid. In particular, it yields the quantum Boltzmann equation satisfied by nkσ (r, t). Finally, we show how δΦ[δn] can be derived (in the static case) using a finite-temperature renormalization-group approach. In agreement with previous results based on this technique, we find that the Landau f function is defined by the fixed-point value of the Ω-limit of the forward-scattering two-particle vertex.