A quantum-mechanical model of multi-photon lasers is proposed for arbitrary degeneracy of the multi-photon processes of photon emission and absorption governing the interaction between the active medium and the radiation field. Equations of motion are derived for the mean values of the intensive, slowly varying operators essential to the description of the dynamics. Stationary solutions are found and their stability is studied proving the existence of a non-equilibrium first-order phase transition. The critical value of the inversion parameter required for laser action is shown to vary by a jump depending on the degree of degeneracy of the multi-photon processes of emission and absorption considered.
The quantum theory of the three-energy-level two-mode laser in which all the levels are being pumped is investigated and the master equation of the laser operation is obtained. It contains two variables,
n1, the photon number of the first mode, and
n2, the photon number of the second mode. There appear four terms in the master equation which represent two-photon processes between the two modes, the absorption of a photon from one mode, and emission of a photon to the other. They are absent in the single-mode case and in the two-mode case with pumping only to the upper level. The master equation can be represented by a diagram of probability in two dimensions which can be extended to infinity, and each arrow of it represents a term on the right-hand side of the master equation. By summing each variable (
n1 or
n2) of the master equation, two equations can be obtained. Each equation contains only one variable, and can be expressed by a diagram of probability flow in one dimension. By considering the correspondence between macroscopic equilibrium and microscopic detailed balance the equations of motion in the steady state are obtained. By introducing a parameter
H, the equation of motion is simplified and a formal solution can be deduced which is dependent on
H. It appears that the parameter
H cannot be fully determined, but some properties of it can be deduced which prove that the introduction of
H is reasonable. The operation characteristics of the laser under different conditions are discussed on the basis of the formal solution: among them are the threshold condition, the condition for one-mode operation, and the change of the photon-statistical distribution. We especially discuss the laser output power curves under two-mode operation above threshold. The curve of one mode, which oscillates first, shows a bending-down phenomenon as the excitation increases when the other mode goes beyond its threshold as demonstrated experimentally by Otsuka. This phenomenon is explained qualitatively and is attributed to the two-photon processes between the two modes.
A quantum-mechanical model for a multiphoton laser is proposed by an obvious generalization of the usual one-photon laser model. The authors consider a class of lasers which preserve detailed balance. This condition is ensured by assuming a multiphoton loss mechanism for the laser light of the same order as the multiphoton gain from the stimulated emission process. Solutions for the stationary density operator of the light field are obtained by a straightforward generalization of the techniques of Scully and Lamb. The multiphoton laser around threshold exhibits behaviour analogous to a second-order phase transition. A non-thermal distribution of multiphoton laser light is achieved above threshold.
We study the dynamics of the solution of a non-linear quantum master equation describing a simple laser under the mean field approximation. The quantum system is formed by a single mode optical cavity and a set of two level atoms that are coupled to two reservoirs. First, we establish the existence of a unique regular stationary state for the non-linear evolution equation under consideration. Second, we examine the free interaction solutions, i.e., the solutions to the non-linear quantum master equation that coincide with unitary evolutions generated by the Hamiltonian resulting from neglecting the interactions between the laser mode, atoms and the bath. We obtain that a family of non-constant free interaction solutions is born at the regular stationary state as a relevant parameter, which is denoted by $C_\mathfrak{b} $, passes through the critical value
1. These free interaction solutions yield the periodic solutions of the Maxwell Bloch equations modeling our physical system in the framework of the semiclassical laser theory. Third, in case $ C_\mathfrak{b} < 1$ we deduce that the system converges exponentially fast to the equilibrium, and so the regular stationary state is a globally asymptotically stable equilibrium solution. Thus, the quantum system has a Hopf bifurcation at $C_\mathfrak{b} =1 $.
The quantum theory of two-level atom single-mode laser system of Sargent, Scully and Lamb is extended to two-mode laser in a three-level atomic system with common lower level, and master equation is obtained for the system with all the three levels being pumped. There appear four terms in the master equation that are absent in the single-mode case and those interpreted as 2-photon processes play an especial role in the present case. The master equation is represented by a probability flow diagram in two-dimensions with the photon numbers n1 and n2 of the two-mode as variables. The probability flow diagram can be extended to infinity, and each arrow of it represents a term of the right hand side of master equation. By taking sum over one of the variables n1 or n2, the master equation is reduced to two equations, each of them can be represented by an one-dimensional probability flow diagram. The equation of motion under steady state is obtained by considering the correspondence between the macroscopic balance and the microscopic balance.A parameter H is introduced to reduce the equation of motion and to facilitate the mathematical procedure and a formal solution is thus obtained. Using the equation of motion and its formal solution various operation characteristics are discussed. Among them are: the threshold condition for each mode; the condition of only one mode operation; the variation of photon statistics between single-mode operation and two-mode operation and the variation of photon statistics with lower level being pumped and not pumped.
A quantum-statistical analysis of multi-photon lasers including the effect of detuning and atomic motion is presented. The equations are solved to fourth order in the atom-field coupling constant. Systems in detailed balance (with multi-photon loss mechanism) as well as systems without detailed balance (with single-photon loss mechanism) are considered separately. Treatments for the single-mode and multi-mode processes are given. Expressions for threshold conditions, peak photon number and the half width of photon distribution are obtained. The variation of mean output photon number, the effect of detuning, the coherence characteristics, etc. are studied and results are illustrated for two- and three-photon lasers as examples.