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Physical Review Letters

Correlation of high-frequency phase fluctuations in electromagnetically induced transparency

Michael Fleischhauer

Published Feb 14, 1994• 96 citations
Publisher

Abstract

A quantum analysis of the interaction of two propagating, quasimonochromatic fields with three-level \ensuremath{\Lambda}-type atoms is presented. It is shown that the recently predicted effect of pulse matching [S. Harris, Phys. Rev. Lett. 70, 552 (1993)]--the generation of fields with matched Fourier components--is due to the nonadiabatic response of the medium. This effect leads to a correlation of the high-frequency phase fluctuations of the fields, and may therefore be used to reduce the noise in short-time measurements of phase differences.

DOI
10.1103/physrevlett.72.989

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Laser Physics Letters•Jun 6, 2014•3 citations
A quantum analysis of the interaction of two propagating, quasimonochromatic fields with three-level \ensuremath{\Lambda}-type atoms is presented. It is shown that the recently predicted effect of pulse matching [S. Harris, Phys. Rev. Lett. 70, 552 (1993)]--the generation of fields with matched Fourier components--is due to the nonadiabatic response of the medium. This effect leads to a correlation of the high-frequency phase fluctuations of the fields, and may therefore be used to reduce the noise in short-time measurements of phase differences.
The interaction of a bichromatic quantized field with three-level \ensuremath{\Lambda}-type atoms is analyzed on the basis of c-number Langevin equations. In the presence of ground-state coherence one particular combination of field modes is selectively absorbed leading to a correlation of the output fields. This correlation manifests itself in a matching of Fourier components of the field modes and in a strong reduction of the diffusion of the difference phase. This correlation phenomenon is studied for the case of externally generated coherence as well as for coherence produced by population trapping in conjunction with a nonadiabatic atomic response.
Summary form only given. The destructive quantum interference of resonantly excited transitions within a lambda-system in case of two photon resonance leads to a medium, which is coherently prepared in a superpositional dark state. The corresponding distinct enhancement of radiation transmission is well known as electromagnetically induced transparency. Interaction of quantized fields with such a medium yields a correlation of quantum phase fluctuations of the fields even for independent cw lasers. The experiments are done on the Na D/sub 1/ line by means of a temperature stabilized sodium vapor cell. One frequency component is modulated by a broad spectrum of phase fluctuations of about 50 MHz width by means of an electrooptical phase modulator driven by a noise generator. A transfer of noise to the other frequency components within a lambda- or a closed double-lambda transition scheme during transmission through the dark state medium is observed using the heterodyne spectroscopy. The verified exponential decay of the width of the beat signal in dependence on the medium optical density proofs the noise transfer and hence the correlation of phase fluctuations between the corresponding frequency components. This behaviour as well as the different limits of decay for lambda- (towards the transparency linewidth) and closed double-lambda (towards zero) scheme is in good qualitative agreement with the theory.
Summary form only given. The destructive quantum interference of resonantly excited transitions within a lambda-system in case of two photon resonance leads to a medium, which is coherently prepared in a superpositional dark state. The corresponding distinct enhancement of radiation transmission is well known as electromagnetically induced transparency. Interaction of quantized fields with such a medium yields a correlation of quantum phase fluctuations of the fields even for independent cw lasers. The experiments are done on the Na D/sub 1/ line by means of a temperature stabilized sodium vapor cell. One frequency component is modulated by a broad spectrum of phase fluctuations of about 50 MHz width by means of an electrooptical phase modulator driven by a noise generator. A transfer of noise to the other frequency components within a lambda- or a closed double-lambda transition scheme during transmission through the dark state medium is observed using the heterodyne spectroscopy. The verified exponential decay of the width of the beat signal in dependence on the medium optical density proofs the noise transfer and hence the correlation of phase fluctuations between the corresponding frequency components. This behaviour as well as the different limits of decay for lambda- (towards the transparency linewidth) and closed double-lambda (towards zero) scheme is in good qualitative agreement with the theory.
Quantum coherence and interference in atomic systems can lead to interesting optical phenomena such as nonabsorbing resonances, lasing without inversion, generating an ultrahigh index of refraction without absorption, propagation of light pulses without losses. In the last-named is given the title transparency. Up to now it is known some types of transparency in multi-level resonant media. One of them is electromagnetically induced transparency (EIT). The phenomenon of EIT in the propagation of laser radiation through an absorbing medium has been recently investigated and explained in terms of quantum coherence and interference for multi-level atomic system. For instance in the (Lambda) -system, if the atomic medium is prepared in a quantum superposition of states, matched pulses, i.e., a pair of optical pulses whose amplitude and phase have a well defined relation, propagate without absorption. The mechanism of coherent population trapping is responsible for EIT in a (Lambda) -system. There is another, well known mechanism for creating transparency in a two-state atom: self-induced transparency, or SIT. Here, a single pulse whose area (the integral of its Rabi frequency over time) is 2(pi) is applied to the medium. Such a pulse causes the atoms to cycle smoothly from the ground to the excited state and then back again. In principle, such a pulse can propagate over long distances. SIT can be generalized to multi-level systems and multiple quasi-monochromatic fields. Generalization of SIT in a (Lambda) -system was obtained in reference 2. In this report we present a new type of transparency (combined transparency). This type describes propagation of laser pulse through a (Lambda) -type medium where the initial atomic state is prepared in the form of spatially varying coherent superposition of low-energetic states (initial coherency gradient). The common envelope behaves as usual 2(pi) hyperbolic secant pulse, but the ratio between the components of frequencies transitions 1> yields 3> and 2> yields 3> changes due to coherent Raman scattering so (phi) equals atan(E1/E2) equals (pi) /2-Gz, where z is the coordinate, G is the constant determined by both the incident pulse parameters and the initial coherence between the atomic states. Our solution demonstrates a direct connection of EIT in adiabatic regime to the SIT effects. This type of a transparency is given the title screw-type transparency, because for the given form of incident pulse (pitch of screw) medium is transparent, if medium's the initial coherence gradient is correspondingly prepared (thread on a engine nut). Besides a transparency, this phenomenon contains a transformation of the incident pulse frequency during the process of the propagation. This property of the phenomena can be result in a complete conversion of the frequency.
We study the dynamics of the phase pulses of laser radiation with two resonant frequency components propagating in an atomic three-level Λ type medium under coherent population trapping. Using the density matrix adiabatic approach we show that the effect of a very large slowing down occurs not only for amplitude pulses, but also for phase pulses. The group velocity of phase pulses can be controlled by the amplitudes of resonant fields. The analytical solution describing the mutual influence of the phase modulation of one field component on another is obtained.