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Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)

Nonlinear magneto-optical effects and quantum coherences in cold rubidium atoms in an optical dipole trap

Adam M. Wojciechowski, Krystian Sycz, Artur Stabrawa, Marcin Piotrowski, Jerzy Zachorowski, Wojciech Gawlik

Published May 1, 2013• 0 citations
Publisher

Abstract

We report on our experiments on nonlinear magneto-optical effects in laser-cooled, near-degenerate rubidium samples. Atoms are laser-cooled and subsequently transferred to the crossed-beam optical dipole trap (ODT), formed by a tight focusing of 1560-nm laser beams. The trap not only provides long relaxation time but also allows us to investigate the quantum degeneracy regime. Moreover, the tight confinement of atoms enables magnetic field probing with a high spatial resolution of a few tens of micrometers.

DOI
10.1109/cleoe-iqec.2013.6801785

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•Jan 1, 1996•1 citation
We report on our experiments on nonlinear magneto-optical effects in laser-cooled, near-degenerate rubidium samples. Atoms are laser-cooled and subsequently transferred to the crossed-beam optical dipole trap (ODT), formed by a tight focusing of 1560-nm laser beams. The trap not only provides long relaxation time but also allows us to investigate the quantum degeneracy regime. Moreover, the tight confinement of atoms enables magnetic field probing with a high spatial resolution of a few tens of micrometers.
We discuss our experimental results on forced evaporative cooling of cold rubidium 87 Rb atoms to quantum degeneracy in an Optical Dipole Trap. The atoms are first trapped and cooled in a magneto-optical trap (MOT) loaded from a continuous beam of cold atoms [1]. More than 10 10 atoms are trapped in the MOT and then about 10 8 atoms are transferred to a Quasi-Electrostatic Trap (QUEST) formed by tightly focused CO2 laser (λ = 10.6μ m ) beams intersecting at their foci in an orthogonal configuration in the horizontal plane. Before loading the atoms into the dipole trap, the phase-space density of the atomic ensemble was increased making use of sub-doppler cooling at large detuning and the temporal dark MOT technique. In a MOT the phase-space density of the atomic ensemble is six orders of magnitude less than what is required to achieve quantum degeneracy. After transferring atoms into the dipole trap efficiently, phase-space density increases by a factor of 10 3 . Further increase in phase-space density to quantum degeneracy is achieved by forced evaporative cooling of atoms in the dipole trap. The evaporative cooling process involves a gradual reduction of the trap depth by ramping down the trapping laser intensity over a second. The temperature of the cold atomic cloud was measured by time-of-flight (TOF) technique. The spatial distribution of the atoms is measured using absorption imaging. We report results of evaporative cooling in a single beam and in a crossed double-beam dipole traps. Due to the large initial phase space density, and large initial number of atoms trapped, the quantum phase transition occurs after about 600 ms of evaporative cooling in our optimized crossed dipole trap.
The interaction of light with atoms and molecules is of fundamental interest in many branches of science. In atomic physics, this interaction can be used to cool and spatially confine (trap) atoms. These traps can be used as the starting point for other experiments, but the dynamics of the cooling and trapping processes is itself of interest. In order to better understand the physics of trapping atoms in an optical dipole force trap, we have conducted a series of spectroscopic measurements of ultracold rubidium atoms in such a trap. The trap was created at the focus of a Nd:YAG laser beam with wavelength 1064nm and nearly Gaussian spatial mode. For rubidium, the trap light is red-detuned and the atoms are confined to the highest intensity in the beam. In order to probe the atoms confined in the trap, we have performed spectroscopy on the 5S1/2 → 5P3/2 transition. Because the polarizability of the ground and excited states is not the same at the trap wavelength, the spectra exhibit both a shift and inhomogeneous broadening. We have investigated the spectra for both linear and circular polarized traps. We also studied the application of a second laser to couple the excited state (5P3/2) to another higher excited state (5D5/2) to reduce the inhomogeneous broadening of the 5S1/2 → 5P 3/2 transition. Finally, two-photon spectroscopy was performed on atoms in the dipole force trap and compared to spectra taken in a magneto optical trap (MOT). Autler-Townes splitting was clearly observed in the MOT and appears to have been observed in the dipole force trap also.
This thesis reports on the design, setup, and operation of a new atom trap apparatus, which is developed to confine few rubidium atoms in ultrahigh vacuum by means of taylored and dynamically variable light potentials (dipole traps), thus making the atoms available for spectroscopy and controlled manipulations. To maintain low background pressure, atoms of a vapour cell are transferred into a cold atomic beam by laser cooling techniques, and accumulated by a magneto-optic trap (MOT) in a separate part of the vacuum system. The laser cooled atoms are then transferred into dipole traps made of focused far-off-resonant laser fields in single or crossed-beam geometry, which are superimposed with the center of the MOT. Gaussian as well as hollow Laguerre-Gaussian (LG01) beam profiles are used with red-detuned and blue-detuned light. Microfabricated dielectric phase objects allow the efficient and robust mode conversion of Gaussian into Laguerre-Gaussian laser beams. Trap geometries can easily be changed due to the highly flexible experimental setup. The dipole trap laser beams have powers up to several hundred milliwatts and are focused to around 10 m. At a detuning of several tens of nanometers from the atomic resonance, the resulting traps are a few millikelvin deep, and the trapped atoms exhibit motional frequencies near 30 kHz, trap light scattering rates of a few hundred photons per second per atom, and storage times of several seconds. The number of dipole-trapped atoms ranges from more than ten thousand to below ten. The dipole-trapped atoms are detected either by a photon counting system with efficient straylight discrimination, or by recapture into the MOT, which is imaged onto a sensitive photodiode and a CCD-camera. Due to the strong AC-Stark shift imposed by the high-intensity trapping light, energy-selective resonant excitation and detection of the stored atoms is possible. The measured energy distribution is consistent with a harmonic potential shape and allows for the determination of temperatures and heating rates. From initial measurements, the thermal energy is found to be about 10 % of the trap depth. Using a crossed-beam geometry with red-detuned laser light, efficient transfer of atoms between the beams is observed. Optimum transfer occurs when the two beams cross at a radial offset, which can qualitatively be understood when the particle energy and geometrical properties of the two-beam trapping potential are considered. Numerical simulations reproduce the general features of the measured transfer efficiency vs. radial beam offset. This experiment is a first step towards dynamically variable potentials. Atoms have been radially confined in a blue-detuned hollow beam, and their decay time has been determined. This configuration is currently extended to a three-dimensionally confining blue-detuned dipole trap. For advanced laser cooling, state manipulation and spectroscopy of trapped atoms, a system of two diode lasers has been set up which are phase-coherently locked with a difference frequency near 6.834 GHz, to drive Raman transitions between the hyperfine-split ground states of 87Rb atoms. Resonances of such a transition have been recorded in a buffer gas loaded rubidium vapour cell with linewidths below 100 Hz.
Spectral characteristics of rubidium atoms confined in a dark magneto-optical trap (DMOT) are measured, including probe absorption spectra and atom density as a function of the cooling and repumping laser frequencies. The trap can capture and cool more than 2.5 × 10 8 rubidium atoms, confining them in a hyperfine state weakly perturbed by the laser beams used to form the trap. The optical density of the trapped atomic cloud approaches 9. A qualitative model of the DMOT operation is presented, based on the experimental results obtained.
This thesis describes theoretical and experimental work concerning radiation forces on atoms, with particular reference to rubidium atoms confined in a magneto-optical trap. After a short history of the field of laser cooling, a review of the semiclassical theory of mechanical interactions between two-level atoms and electromagnetic radiation is given. Different formulations of the semiclassical theory are discussed, including a new formulation in terms of momentum transfer amongst the plane wave modes of the electromagnetic field. Two important applications of light forces on atoms, namely 'optical molasses' and the 'magneto-optical trap', are then described with emphasis on experimental parameters. Three sub-Doppler cooling mechanisms, 'sisyphus cooling', 'motion-induced orientation cooling' and the 'magnetically-assisted sisyphus effect', are described and their role in optical molasses and the magneto-optical trap is discussed. A new study of the polarisation gradients which occur in 3-D monochromatic light fields is presented and quantifies their relative presence in different light field configurations. Polarisation gradient parameters are developed and shown to be directly related to the relativistic spin tensor of the light field. Implications of this polarisation gradient study for laser cooling work are discussed. The design, construction from scratch, operation and testing of a magneto-optical trap for rubidium are described, including novel designs for two vacuum cells. Preliminary experiments to characterise the trap are described and results are presented; they primarily concern the number and distribution of atoms in the trap. Finally. the theory of time domain spectroscopy is reviewed. The construction and testing of a pulsed dye laser for study of coherent transients in samples of laser-cooled atoms and a proposed experiment to measure the temperature of cold atoms using coherent transients are described. Factors expected to influence the shape of coherent transients in cold atoms are discussed.