An array of N closely spaced dipole coupled quantum emitters exhibits super- and subradiance with characteristic tailorable spatial radiation patterns. Optimizing the emitter geometry and distance with respect to the spatial profile of a near resonant optical cavity mode allows us to increase the ratio between light scattering into the cavity mode and free space emission by several orders of magnitude. This leads to distinct scaling of the collective coherent emitter-field coupling vs the free space decay as a function of the emitter number. In particular, for subradiant states, the effective cooperativity increases much faster than the typical linear ∝N scaling for independent emitters. This extraordinary collective enhancement is manifested both in the amplitude and the phase profile of narrow collective antiresonances appearing at the cavity output port in transmission spectroscopy.An array of N closely spaced dipole coupled quantum emitters exhibits super- and subradiance with characteristic tailorable spatial radiation patterns. Optimizing the emitter geometry and distance with respect to the spatial profile of a near resonant optical cavity mode allows us to increase the ratio between light scattering into the cavity mode and free space emission by several orders of magnitude. This leads to distinct scaling of the collective coherent emitter-field coupling vs the free space decay as a function of the emitter number. In particular, for subradiant states, the effective cooperativity increases much faster than the typical linear ∝N scaling for independent emitters. This extraordinary collective enhancement is manifested both in the amplitude and the phase profile of narrow collective antiresonances appearing at the cavity output port in transmission spectroscopy.

arXiv:1703.06039Physical Review LettersAug 31, 201774 citations

Theory of the Collective Many-body Subradiance in Waveguide Quantum Electrodynamics

Xin Wang, Junjun He, Zeyang Liao

We present an analytical theory for the most subradiant modes in a finite one-dimensional emitter array coupled to either an ideal or a nonideal waveguide. Using an effective non-Hermitian Hamiltonian together with a Bragg-edge open-boundary ansatz, we derive compact expressions for the full complex collective eigenvalues, including both the linewidths and the collective energy shifts. The linewidths of the most subradiant states exhibit the characteristic $N^{-3}$ scaling in both cases, while in the deep-subwavelength regime they display even--odd oscillations due to boundary interference. In contrast, the collective energy shift approaches a separation-dependent asymptotic value with a leading finite-size correction scaling as $N^{-2}$ . These results highlight the distinct physical origins of the imaginary and real parts of the subradiant eigenvalue: Bragg-edge destructive interference controls the linewidth, whereas near-field dipole--dipole interactions dominate the collective shift. Our theory provides a transparent framework beyond the ideal-waveguide limit and opens potential applications in subradiant spectroscopy and waveguide-QED-based sensing.We present an analytical theory for the most subradiant modes in a finite one-dimensional emitter array coupled to either an ideal or a nonideal waveguide. Using an effective non-Hermitian Hamiltonian together with a Bragg-edge open-boundary ansatz, we derive compact expressions for the full complex collective eigenvalues, including both the linewidths and the collective energy shifts. The linewidths of the most subradiant states exhibit the characteristic $N^{-3}$ scaling in both cases, while in the deep-subwavelength regime they display even--odd oscillations due to boundary interference. In contrast, the collective energy shift approaches a separation-dependent asymptotic value with a leading finite-size correction scaling as $N^{-2}$. These results highlight the distinct physical origins of the imaginary and real parts of the subradiant eigenvalue: Bragg-edge destructive interference controls the linewidth, whereas near-field dipole--dipole interactions dominate the collective shift. Our theory provides a transparent framework beyond the ideal-waveguide limit and opens potential applications in subradiant spectroscopy and waveguide-QED-based sensing.

quant-pharXiv:2604.03954Apr 7, 20260 citations

Optical Spectroscopy

Manuel Vogel

Springer series on atomic, optical, and plasma physicsJan 1, 20241 citation

Quantum Coherence and Collective Phenomena: From Spectroscopy to Accelerating Detectors

Tuguldur Begzjav

During the last half century, quantum coherence has been of great interest due to its own right and also due to its broad range of applications in many areas of physics. The reason for that is the technological progress made last century, specially, the invention of coherent light sources and their commercialization. Indeed, coherent laser sources allow us to coherently excite atoms and molecules, as a consequence, to study variety of coherent and collective phenomena in atomic physics, for instance, coherent optical spectroscopy, superradiance, superflourescence, lasing without inversion and so forth. Interestingly, recent studies in biological systems also seem to exhibit coherent processes, in particular, photosynthetic transport and avian compass.\n\nIn this dissertation, we present some of the theory and applications of the quantum coherence. This study considers (i) application of quantum coherence to enhance output signals of coherent anti-Stokes Raman spectroscopy of optically active media (chiral molecules), (ii) a way to find general formulas of single- and double-excited subradiant Dicke states using symmetry group theory, (iii) an impact of Fano-Agarwal coupling and other virtual processes arising from non-rotating wave approximation on the decay of super and subradiant timed Dicke states, and finally (iv) quantum coherence and collective phenomena of relativistically and uniformly accelerating atoms.\n\nApplications of the results presented in the dissertation may be a new method for resolving chirality of molecules using coherent anti-Stokes Raman spectroscopy - Raman optical activity, and a sidewise excitation method for single- and double-excited subradiant states. The obtained results also advance our theoretical understanding of quantum coherence specially theory of super and subradiance.During the last half century, quantum coherence has been of great interest due to its own right and also due to its broad range of applications in many areas of physics. The reason for that is the technological progress made last century, specially, the invention of coherent light sources and their commercialization. Indeed, coherent laser sources allow us to coherently excite atoms and molecules, as a consequence, to study variety of coherent and collective phenomena in atomic physics, for instance, coherent optical spectroscopy, superradiance, superflourescence, lasing without inversion and so forth. Interestingly, recent studies in biological systems also seem to exhibit coherent processes, in particular, photosynthetic transport and avian compass.\n\nIn this dissertation, we present some of the theory and applications of the quantum coherence. This study considers (i) application of quantum coherence to enhance output signals of coherent anti-Stokes Raman spectroscopy of optically active media (chiral molecules), (ii) a way to find general formulas of single- and double-excited subradiant Dicke states using symmetry group theory, (iii) an impact of Fano-Agarwal coupling and other virtual processes arising from non-rotating wave approximation on the decay of super and subradiant timed Dicke states, and finally (iv) quantum coherence and collective phenomena of relativistically and uniformly accelerating atoms.\n\nApplications of the results presented in the dissertation may be a new method for resolving chirality of molecules using coherent anti-Stokes Raman spectroscopy - Raman optical activity, and a sidewise excitation method for single- and double-excited subradiant states. The obtained results also advance our theoretical understanding of quantum coherence specially theory of super and subradiance.

May 19, 20200 citations

N^{-3}

scaling in both cases, while in the deep-subwavelength regime they display even--odd oscillations due to boundary interference. In contrast, the collective energy shift approaches a separation-dependent asymptotic value with a leading finite-size correction scaling as

N^{-2}

. These results highlight the distinct physical origins of the imaginary and real parts of the subradiant eigenvalue: Bragg-edge destructive interference controls the linewidth, whereas near-field dipole--dipole interactions dominate the collective shift. Our theory provides a transparent framework beyond the ideal-waveguide limit and opens potential applications in subradiant spectroscopy and waveguide-QED-based sensing.