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Springer series on atomic, optical, and plasma physics

Optical Spectroscopy

Manuel Vogel

Published Jan 1, 2024• 1 citation
Publisher
DOI
10.1007/978-3-031-55420-9_20

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Abstract Multidimensional coherent optical spectroscopy (MDCS) is an elegant and versatile tool to measure the ultrafast nonlinear optical response of materials. Of particular interest for semiconductor nanostructures, MDCS enables the separation of homogeneous and inhomogeneous linewidths, reveals the nature of coupling between resonances, and is able to identify the signatures of many-body interactions. As an extension of transient four-wave mixing (FWM) experiments, MDCS can be implemented in various geometries, in which different strategies can be used to isolate the FWM signal and measure its phase. I review and compare different practical implementations of MDCS experiments adapted to the study of semiconductor materials. The power of MDCS is illustrated by discussing experimental results obtained on semiconductor nanostructures such as quantum dots, quantum wells, microcavities, and layered semiconductors.
State of the art of optical coherent spectroscopy of doped solids that are promising as information carriers for optical processors is reviewed. Special attention is paid to optical echo spectroscopy of doped crystals classified as the Van-Vleck paramagnets where the long-lived stimulated echo is observed with the optical-memory time reaching several hours at low temperatures. Modern elaborations of optical echo processors based on this echo phenomenon are discussed. Physical principles of femtosecond echo spectroscopy and coherent four-wave mixing spectroscopy are formulated. The abilities of these methods in the diagnostics of fast processes at room temperature are illustrated using examples of a doped polymer films. The results of elaborations of a new branch of optical spectroscopy (biphoton spectroscopy) are also presented. The advantages and possible applications of this method are demonstrated using an example of two crystals (Er 3+ :YAG and Cr 3+ :Al 2 O 3 ).