Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)

Two-photon spectra of quantum systems

Elena del Valle, Alejandro González-Tudela, Fabrice P. Laussy, C. Tejedor, Michael J. Hartmann

Published May 1, 2013• 0 citations
Publisher

Abstract

Summary form only given. We present our recent theory [1] of frequency-filtered and time-resolved N-photon correlations or N-photon spectra, g(N)Γ(ω1, T1;... ; ωNTN). There are an extension of the standard Nth order temporal correlation functions, g(N)(T1;... ;TN) (that measure the probability of emission of N photons at times T1,..., TN), into the frequency domain. Heisenberg uncertainty principle requires the introduction of the detector or filter frequency resolution, Γ, in the theory.

DOI
10.1109/cleoe-iqec.2013.6801656

Related papers

Two-photon spectra of quantum emitters

Alejandro González-Tudela, Materia Condensada, Fabrice P. Laussy +3 more

Abstract. We apply our recently developed theory of frequency-filtered and time-resolved N-photon correlations [1] to study the two-photon spectra of a variety of systems of increasing complexity: single mode emitters with two limiting statistics (one harmonic oscillator or a two-level system) and the various combinations that arise from their coupling. We consider both the linear and nonlinear regimes under incoherent excitation. We find that even the simplest systems display a rich dynamics of emission, not accessible by simple single photon spectroscopy. In the strong coupling regime, novel two-photon emission processes involving virtual states are revealed. Furthermore, two general results are unraveled by two-photon correlations with narrow linewidth detectors: i) filtering induced bunching and ii) breakdown of the semi-classical theory. We show how to overcome this shortcoming in a fully-quantized picture. PACS numbers: 42.50.Ar,42.50.Lc,05.10.Gg,42.25.Kb,42.79.Pw ar X iv

•Jan 1, 2013•96 citations

Two-photon spectra of quantum emitters

Alejandro Gonzalez-Tudela, Fabrice P. Laussy, Carlos Tejedor +2 more

We apply our recently developed theory of frequency-filtered and time-resolved N -photon correlations (del Valle et al 2012 Phys. Rev. Lett. 109 183601) to study the two-photon spectra of a variety of systems of increasing complexity: single-mode emitters with two limiting statistics (one harmonic oscillator or a two-level system) and the various combinations that arise from their coupling. We consider both the linear and nonlinear regimes under incoherent excitation. We find that even the simplest systems display a rich dynamics of emission, not accessible by simple single-photon spectroscopy. In the strong coupling regime, two-photon emission processes involving virtual states are revealed. Furthermore, two general results are unravelled by two-photon correlations with narrow linewidth detectors: (i) filtering-induced bunching and (ii) breakdown of the semi-classical theory. We show how to overcome the latter in a fully quantized picture.

arXiv:1211.5592•New Journal of Physics•Mar 22, 2013•103 citations

Theory of Frequency-Filtered and Time-Resolved N -Photon Correlations

Elena del Valle, Alejandro González-Tudela, Fabrice P. Laussy +2 more

A theory of correlations between N photons of given frequencies and detected at given time delays is presented. These correlation functions are usually too cumbersome to be computed explicitly. We show that they are obtained exactly through intensity correlations between two-level sensors in the limit of their vanishing coupling to the system. This allows the computation of correlation functions hitherto unreachable. The uncertainties in time and frequency of the detection, which are necessary variables to describe the system, are intrinsic to the theory. We illustrate the power of our formalism with the example of the Jaynes-Cummings model, by showing how higher order photon correlations can bring new insights into the dynamics of open quantum systems.

arXiv:1203.6016•Physical Review Letters•Oct 31, 2012•152 citations

Achieving two-dimensional optical spectroscopy with temporal and spectral resolution using quantum entangled three photons

Yuta Fujihashi, Akihito Ishizaki

Recent advances in techniques for generating quantum light have stimulated research on novel spectroscopic measurements using quantum entangled photons. One such spectroscopy technique utilizes non-classical correlations among entangled photons to enable measurements with enhanced sensitivity and selectivity. Here, we investigate the spectroscopic measurement utilizing entangled three photons. In this measurement, time-resolved entangled photon spectroscopy with monochromatic pumping [A. Ishizaki, J. Chem. Phys. 153, 051102 (2020)] is integrated with the frequency-dispersed two-photon counting technique, which suppresses undesired accidental photon counts in the detector and thus allows one to separate the weak desired signal. This time-resolved frequency-dispersed two-photon counting signal, which is a function of two frequencies, is shown to provide the same information as that of coherent two-dimensional optical spectra. The spectral distribution of the phase-matching function works as a frequency filter to selectively resolve a specific region of the two-dimensional spectra, whereas the excited-state dynamics under investigation are temporally resolved in the time region longer than the entanglement time. The signal is not subject to Fourier limitations on the joint temporal and spectral resolution, and therefore, it is expected to be useful for investigating complex molecular systems in which multiple electronic states are present within a narrow energy range.

arXiv:2103.04534•The Journal of Chemical Physics•Jul 22, 2021•12 citations

Optimization of photon correlations by frequency filtering

Alejandro González-Tudela, Elena del Valle, Fabrice P. Laussy

Photon correlations are a cornerstone of quantum optics. Recent works [E. del Valle, New J. Phys. 15, 025019 (2013); A. Gonzalez-Tudela et al., New J. Phys. 15, 033036 (2013); C. Sanchez Mu\~noz et al., Phys. Rev. A 90, 052111 (2014)] have shown that by keeping track of the frequency of the photons, rich landscapes of correlations are revealed. Stronger correlations are usually found where the system emission is weak. Here, we characterize both the strength and signal of such correlations, through the introduction of the ``frequency-resolved Mandel parameter.'' We study a plethora of nonlinear quantum systems, showing how one can substantially optimize correlations by combining parameters such as pumping, filtering windows and time delay.

arXiv:1501.01799•Physical Review A•Apr 6, 2015•50 citations

Two-photon emission spectrum of a two-level atom in an ideal cavity

Lin-sheng He, Xun‐Li Feng

The time-dependent two-photon emission spectra of a two-level atom interacting with a single-mode radiation field in an ideal cavity have been studied. The expressions of the system operators as a function of time have been derived based on the two-photon Jaynes-Cummings model and Heisenberg equation. As a result, the theoretical curves of the time-dependent two-photon emission spectra have been given. The features of two-photon emission spectra depend not only on the photon statistical distribution of the initial field, such as the thermal field, the squeezed vacuum field, and the coherent field, but also on the passband width of the filter detector \ensuremath{\Gamma}. The two-photon emission spectra exhibit multi- peaked structures when \ensuremath{\Gamma}(two-photon coupling constant).

Physical Review A•May 1, 1994•26 citations
Summary form only given. We present our recent theory [1] of frequency-filtered and time-resolved N-photon correlations or N-photon spectra, g(N)Γ(ω1, T1;... ; ωNTN). There are an extension of the standard Nth order temporal correlation functions, g(N)(T1;... ;TN) (that measure the probability of emission of N photons at times T1,..., TN), into the frequency domain. Heisenberg uncertainty principle requires the introduction of the detector or filter frequency resolution, Γ, in the theory.
Abstract. We apply our recently developed theory of frequency-filtered and time-resolved N-photon correlations [1] to study the two-photon spectra of a variety of systems of increasing complexity: single mode emitters with two limiting statistics (one harmonic oscillator or a two-level system) and the various combinations that arise from their coupling. We consider both the linear and nonlinear regimes under incoherent excitation. We find that even the simplest systems display a rich dynamics of emission, not accessible by simple single photon spectroscopy. In the strong coupling regime, novel two-photon emission processes involving virtual states are revealed. Furthermore, two general results are unraveled by two-photon correlations with narrow linewidth detectors: i) filtering induced bunching and ii) breakdown of the semi-classical theory. We show how to overcome this shortcoming in a fully-quantized picture. PACS numbers: 42.50.Ar,42.50.Lc,05.10.Gg,42.25.Kb,42.79.Pw ar X iv
We apply our recently developed theory of frequency-filtered and time-resolved N -photon correlations (del Valle et al 2012 Phys. Rev. Lett. 109 183601) to study the two-photon spectra of a variety of systems of increasing complexity: single-mode emitters with two limiting statistics (one harmonic oscillator or a two-level system) and the various combinations that arise from their coupling. We consider both the linear and nonlinear regimes under incoherent excitation. We find that even the simplest systems display a rich dynamics of emission, not accessible by simple single-photon spectroscopy. In the strong coupling regime, two-photon emission processes involving virtual states are revealed. Furthermore, two general results are unravelled by two-photon correlations with narrow linewidth detectors: (i) filtering-induced bunching and (ii) breakdown of the semi-classical theory. We show how to overcome the latter in a fully quantized picture.
A theory of correlations between N photons of given frequencies and detected at given time delays is presented. These correlation functions are usually too cumbersome to be computed explicitly. We show that they are obtained exactly through intensity correlations between two-level sensors in the limit of their vanishing coupling to the system. This allows the computation of correlation functions hitherto unreachable. The uncertainties in time and frequency of the detection, which are necessary variables to describe the system, are intrinsic to the theory. We illustrate the power of our formalism with the example of the Jaynes-Cummings model, by showing how higher order photon correlations can bring new insights into the dynamics of open quantum systems.
Recent advances in techniques for generating quantum light have stimulated research on novel spectroscopic measurements using quantum entangled photons. One such spectroscopy technique utilizes non-classical correlations among entangled photons to enable measurements with enhanced sensitivity and selectivity. Here, we investigate the spectroscopic measurement utilizing entangled three photons. In this measurement, time-resolved entangled photon spectroscopy with monochromatic pumping [A. Ishizaki, J. Chem. Phys. 153, 051102 (2020)] is integrated with the frequency-dispersed two-photon counting technique, which suppresses undesired accidental photon counts in the detector and thus allows one to separate the weak desired signal. This time-resolved frequency-dispersed two-photon counting signal, which is a function of two frequencies, is shown to provide the same information as that of coherent two-dimensional optical spectra. The spectral distribution of the phase-matching function works as a frequency filter to selectively resolve a specific region of the two-dimensional spectra, whereas the excited-state dynamics under investigation are temporally resolved in the time region longer than the entanglement time. The signal is not subject to Fourier limitations on the joint temporal and spectral resolution, and therefore, it is expected to be useful for investigating complex molecular systems in which multiple electronic states are present within a narrow energy range.
Photon correlations are a cornerstone of quantum optics. Recent works [E. del Valle, New J. Phys. 15, 025019 (2013); A. Gonzalez-Tudela et al., New J. Phys. 15, 033036 (2013); C. Sanchez Mu\~noz et al., Phys. Rev. A 90, 052111 (2014)] have shown that by keeping track of the frequency of the photons, rich landscapes of correlations are revealed. Stronger correlations are usually found where the system emission is weak. Here, we characterize both the strength and signal of such correlations, through the introduction of the ``frequency-resolved Mandel parameter.'' We study a plethora of nonlinear quantum systems, showing how one can substantially optimize correlations by combining parameters such as pumping, filtering windows and time delay.
The time-dependent two-photon emission spectra of a two-level atom interacting with a single-mode radiation field in an ideal cavity have been studied. The expressions of the system operators as a function of time have been derived based on the two-photon Jaynes-Cummings model and Heisenberg equation. As a result, the theoretical curves of the time-dependent two-photon emission spectra have been given. The features of two-photon emission spectra depend not only on the photon statistical distribution of the initial field, such as the thermal field, the squeezed vacuum field, and the coherent field, but also on the passband width of the filter detector \ensuremath{\Gamma}. The two-photon emission spectra exhibit multi- peaked structures when \ensuremath{\Gamma}(two-photon coupling constant).