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arXiv:1203.6016 · Physical Review Letters

Theory of Frequency-Filtered and Time-Resolved N -Photon Correlations

Elena del Valle, Alejandro González-Tudela, Fabrice P. Laussy, C. Tejedor, Michael J. Hartmann

Published Oct 31, 2012• 152 citations
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Abstract

A theory of correlations between N photons of given frequencies and detected at given time delays is presented. These correlation functions are usually too cumbersome to be computed explicitly. We show that they are obtained exactly through intensity correlations between two-level sensors in the limit of their vanishing coupling to the system. This allows the computation of correlation functions hitherto unreachable. The uncertainties in time and frequency of the detection, which are necessary variables to describe the system, are intrinsic to the theory. We illustrate the power of our formalism with the example of the Jaynes-Cummings model, by showing how higher order photon correlations can bring new insights into the dynamics of open quantum systems.

DOI
10.1103/physrevlett.109.183601

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A theory of correlations between N photons of given frequencies and detected at given time delays is presented. These correlation functions are usually too cumbersome to be computed explicitly. We show that they are obtained exactly through intensity correlations between two-level sensors in the limit of their vanishing coupling to the system. This allows the computation of correlation functions hitherto unreachable. The uncertainties in time and frequency of the detection, which are necessary variables to describe the system, are intrinsic to the theory. We illustrate the power of our formalism with the example of the Jaynes-Cummings model, by showing how higher order photon correlations can bring new insights into the dynamics of open quantum systems.
We propose an alternative formulation of the sensor method presented in Phys. Rev. Lett. 109, 183601 (2012) for the calculation of frequency-filtered and time-resolved photon correlations. Our approach is based on an algebraic expansion of the joint steady state of quantum emitter and sensors with respect to the emitter-sensor coupling parameter $\ensuremath{\epsilon}$. This allows us to express photon correlations in terms of the open quantum dynamics of the emitting system only and ensures that computation of correlations are independent on the choice of a small value of $\ensuremath{\epsilon}$. Moreover, using time-dependent perturbation theory, we are able to express the frequency- and time-resolved second-order photon correlation as the addition of three components, each of which gives insight into the physical processes dominating the correlation at different time scales. We consider a bioinspired vibronic dimer model to illustrate the agreement between the original formulation and our approach.
Photon correlations are a cornerstone of quantum optics. Recent works [E. del Valle, New J. Phys. 15, 025019 (2013); A. Gonzalez-Tudela et al., New J. Phys. 15, 033036 (2013); C. Sanchez Mu\~noz et al., Phys. Rev. A 90, 052111 (2014)] have shown that by keeping track of the frequency of the photons, rich landscapes of correlations are revealed. Stronger correlations are usually found where the system emission is weak. Here, we characterize both the strength and signal of such correlations, through the introduction of the ``frequency-resolved Mandel parameter.'' We study a plethora of nonlinear quantum systems, showing how one can substantially optimize correlations by combining parameters such as pumping, filtering windows and time delay.
Frequency-filtered photon correlations have been proven to be extremely useful in grasping how the detection process alters photon statistics. Harnessing the spectral correlations also permits refinement of the emission and unraveling of previously hidden strong correlations in a plethora of quantum-optical systems under continuous-wave excitation. In this work, we investigate such correlations for time-dependent excitation and develop a methodology to compute efficiently time-integrated correlations, which are at the heart of the photon-counting theory, and subsequently apply it to analyze the photon emission of pulsed systems. By combining this formalism with the —which facilitates frequency-resolved correlations—we demonstrate how spectral filtering enhances single-photon purity and suppresses multiphoton noise in time-bin-encoded quantum states. Specifically, filtering the central spectral peak of a dynamically driven two-level system boosts temporal coherence and improves the fidelity of time-bin entanglement preparation, even under conditions favoring multiphoton emission. These results establish spectral filtering as a critical tool for tailoring photon statistics in pulsed quantum light sources.
The problems concerning the influence of spectral filters on the quantum properties of light have recently attracted great attention in connection with quantum cryptography and quantum data transmission. In this paper, we consider the influence of a spectral filter on the second-order coherence function of a field of a resonator mode and a two-level atom in the framework of the Jaynes-Cummings model. Since the Heisenberg equations for the operators of the field of the resonator mode and the atom can be solved exactly, it is possible to obtain exact analytical Fourier transformation of the dynamics of operators of the resonator mode and two-level atom. We demonstrate that the second-order coherence function of the resonator mode and the two-level atom is equal to zero for all possible frequencies in the spectrum of operator oscillations. We find the interbeam second-order coherence function between different frequencies of the Fourier spectrum and show that in the limit of a large number of quanta, it can take the values in the range from zero to two. Thus, non-classical correlations are formed between certain frequencies in the Fourier spectrum of emitted light. We demonstrate that in the limit of a large number of quanta in the resonator mode, when the filter sums up the frequencies near the resonator eigenfrequency, the second-order coherence function of the field of the resonator mode is not affected by the interaction with the two-level atom.
We develop a formalism based on a time-dependent wave-function ansatz to study correlations of photons emitted from a collection of two-level quantum emitters. We show how to simulate the system dynamics and evaluate the intensity of the scattered photons and the second-order correlation function g(2)g^{(2)}g(2) in terms of the amplitudes of the different components of the wave function. Our approach is efficient for considering systems that contain up to two excitations. To demonstrate this we first consider the example of spectral filtering of photons emitted from a single quantum emitter. We show how our formalism can be used to study spectral filtering of the two-photon component of the emitted light from a single quantum emitter for various kinds of filters. Furthermore, as a general application of our formalism, we show how it can be used to study photon-photon correlations in an optically dense ensemble of two-level quantum emitters. In particular we lay out the details of simulating correlated photon transport in such ensembles reported recently by S. Mahmoodian {\it et.al.} [Phys. Rev. Lett. {\bf 121}, 143601 (2018)]. Compared to other existing techniques, the advantage of our formalism is that it is applicable to any generic spectral filter and quantum many-body systems involving a large number of quantum emitters while requiring only a modest computational resource.