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Physical Review Letters

Quantal treatment of cold collisions in a laser field

Murray Holland, Kalle‐Antti Suominen, Keith R. Burnett

Published Apr 11, 1994• 38 citations
Publisher

Abstract

We study the kinetic energy changes taking place in collisions of atoms in a laser cooled cloud. We present a quantum approach, which can treat cold collisions at temperatures well below the Doppler limit of laser cooling. In our numerical treatment we observed an increase in the kinetic energy which depends strongly on the laser detuning and intensity.

DOI
10.1103/physrevlett.72.2367

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We study the kinetic energy changes taking place in collisions of atoms in a laser cooled cloud. We present a quantum approach, which can treat cold collisions at temperatures well below the Doppler limit of laser cooling. In our numerical treatment we observed an increase in the kinetic energy which depends strongly on the laser detuning and intensity.
We give a full quantum treatment of the radiative heating mechanism which arises in atomic clouds at low temperatures due to the collisions in the presence of a light field. The time scale of these collisions is comparable to the time scale of spontaneous decay, hence one needs to combine excitation and decay processes with the quantum motion of the colliding atoms into a single model, which we have done. Our study produces a statistical approximate to the full density matrix by combining wave-packet dynamics with the Monte Carlo state-vector method. We also present a quantitative semiclassical treatment based on the Landau-Zener model, and show that it agrees with the quantal results in certain parameter regimes. However, for low temperatures and strong laser fields the full quantum treatment is needed. We describe our numerical procedures and the statistical aspects of the Monte Carlo state-vector method in detail. Our main result is that the low-energy collisions can produce appreciable heating of the cloud.
We study laser cooling of atoms with narrow-line optical transition, i.e. in regimes when quantum nature of laser-light interactions results significant effect on atom kinetics. We demonstrate the minimum of laser cooing temperature is reached for the light field detuning close to -3 recoil frequency, i.e. is much differ from standard Doppler cooling theory is used for semiclassical description of laser cooling. We define a set of dimensionless parameters that describe the steady state solution of cold atom distribution in laser light and cooling time. The results can be used for analysis an optimal conditions of laser cooling of atoms with narrow lines Ca, Sr and Mg are of interest for optical time standards.
Based on the numerical solution of the quantum kinetic equation for the atomic density matrix, which makes it possible to accurately take into account the recoil effects in the interaction of atoms with field photons, we have studied the limits of laser cooling of atoms using closed optical transitions characterised by different recoil parameters (the ratio of the recoil energy to the natural linewidth). It is shown that for optical transitions with an insufficiently small recoil parameter, the polarisation effects, which lead to the possibility of sub-Doppler laser cooling, lose their efficiency and do not ensure an attainment of the temperature below the Doppler limit. The analysis performed allows one to outline the boundaries of the sub-Doppler theory of laser cooling of atoms.
Deep laser cooling of 24Mg^{24}\mathrm{Mg}24Mg atoms has been theoretically studied. We propose a two-stage sub-Doppler cooling strategy using electrodipole transition $3\phantom{\rule{0.16em}{0ex}}{}^{3}{P}_{2}\ensuremath{\rightarrow}3\phantom{\rule{0.16em}{0ex}}{}^{3}{D}_{3}$ ($\ensuremath{\lambda}\phantom{\rule{0.16em}{0ex}}=\phantom{\rule{0.16em}{0ex}}383.8$ nm). The first stage implies exploiting magneto-optical trap with ${\ensuremath{\sigma}}^{+}$ and ${\ensuremath{\sigma}}^{\ensuremath{-}}$ light beams, while at the second stage lin $\ensuremath{\perp}$ lin molasses is used. We focus on achieving a large number of ultracold atoms (${T}_{\mathrm{eff}}<10 \ensuremath{\mu}\mathrm{K}$) in a cold-atomic cloud. The calculations have been based on quantum treatment, taking into full account the recoil effect and beyond many widely used approximations. Steady-state values of average kinetic energy and linear momentum distributions of cold atoms have been analyzed for various light-field intensities and frequency detunings. The results of conducted quantum analysis have been significantly different from the results achieved under a semiclassical approximation based on the Fokker-Planck equation. The second cooling stage allows achieving sufficiently lower kinetic energies of the atomic cloud as well as increased fraction of ultracold atoms at certain conditions compared to the first one. We hope that the obtained results can help in overcoming current experimental problems in deep cooling of 24Mg^{24}\mathrm{Mg}24Mg atoms by means of laser field. Cold magnesium atoms cooled in a large amount to several $\ensuremath{\mu}\mathrm{K}$ are of huge interest to, for example, quantum metrology and to other many-body cold-atoms physics.