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Indian Journal of Physics

Effects of spontaneous decay on absorptive lineshape in closely spaced transitions of an open four level system

Saswata Ghosh, Swapan Mandal

Published Aug 1, 2010• 0 citations
Publisher
DOI
10.1007/s12648-010-0092-1

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Under the Doppler free condition, a four-level system with three coherently prepared closely spaced upper levels coupled to a single electromagnetic field is being investigated for the absorptive and dispersive lineshapes. By using a perturbation method, the optical Bloch equations for the present four-level system are solved analytically to obtain the induced polarization and hence the spectral lineshapes. The field induced and field independent coherences appear automatically in the analytical expressions of the imaginary and real parts of the complex polarization. These field independent and field dependent coherences are the outcome of the quantum interference between the probability amplitudes of finding the atom in those energy levels. The phase sensitive field induced polarizations are extensively studied for two special conditions of the ground level populations. The influence of the closely spaced transitions on the quantum coherence and hence the subsequent effects on absorption despite inversion, electromagnetically induced transparency and on the ultrahigh index of refraction are discussed.
Two electromagnetic fields (the stronger called the pump and the weaker called the signal) are allowed to interact with a four-level double λ-type system with two pairs of closely spaced levels. The present four-level system could also be viewed as an example of a double resonant system. Under the Doppler-free condition and using a semiclassical formulation of atom–field interaction, we derive the optical Bloch equations involving the said four-level system coupled to two external fields. These coupled optical Bloch equations are unsolvable in closed analytical form. In order to obtain the absorptive lineshapes, we use the usual perturbation method for getting the approximate analytical solution to the coupled optical Bloch equations for the density matrix elements. Through the off-diagonal complex density matrix elements, the introduction of phase angles between the levels participating in dipole-allowed transitions is automatic. It is shown that these phases are appreciable if the applied electromagnetic field is strong. For on-resonance pump conditions, we obtain the usual Rabi splitting. The effects of two-photon resonances are clearly shown for off-resonance pump conditions.