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Research in Optical Sciences

Engineering Source of Multi-Photon, Multidimensional OAM Entangled States for Quantum Control of Nanostructures

Andrea Tabacchini, Mathieu L. Juan, Gabriel Molina‐Terriza

Published Jan 1, 2014• 0 citations
Publisher

Abstract

We study the topic of non-linear light-matter interaction for the generation of multi-photon entangled states. In particular, we want the quantum correlations to be inherent in the Orbital Angular Momentum (OAM) degree of freedom. Our first proposal is to generate four photons, multidimensional, spatially-entangled states, while the final goal is to make them interact with nanostructures for quantum metrology applications.

DOI
10.1364/hilas.2014.jw2a.64

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We study the topic of non-linear light-matter interaction for the generation of multi-photon entangled states. In particular, we want the quantum correlations to be inherent in the Orbital Angular Momentum (OAM) degree of freedom. Our first proposal is to generate four photons, multidimensional, spatially-entangled states, while the final goal is to make them interact with nanostructures for quantum metrology applications.
The identification of orbital angular momentum (OAM) as a fundamental property of a beam of light nearly 25 years ago has led to an extensive body of research around this topic. The possibility that single photons can carry OAM has made this degree of freedom an ideal candidate for the investigation of complex quantum phenomena and their applications. Research in this direction has ranged from experiments on complex forms of quantum entanglement to the interaction between light and quantum states of matter. Furthermore, the use of OAM in quantum information has generated a lot of excitement, as it allows for encoding large amounts of information on a single photon. Here, we explain the intuition that led to the first quantum experiment with OAM 15 years ago. We continue by reviewing some key experiments investigating fundamental questions on photonic OAM and the first steps to applying these properties in novel quantum protocols. At the end, we identify several interesting open questions that could form the subject of future investigations with OAM.This article is part of the themed issue 'Optical orbital angular momentum'.
Multi-particle entangled states are becoming more and more interesting for different applications in quantum information, such as quantum multi-particle teleportation, entangled based cryptography and quantum communication schemes based on multi-particle states, but also for fundamental reasons such as testing local realism by means of the Greenberger-Horne-Zeilinger states (GHZ) arguments . The advantage of multiparticle entanglement versus the most common two particle one lies in the fact that the greater the number of particles involved in the entangled state, the more clearly the quantum effects are exhibited. Our final goal is to exploit the multi-photon entangled states for quantum metrology. By the interaction of those states with nanostructures (mostly nanoholes, but in a future also nanospheres), we expect to reach sub-wavelength sensitivity phase measurements beating the Standard Quantum Limit as well as to detect plasmonic effects. In this thesis we present our work consisting on designing and building an experimental setup for the generation of states of 4-photon entangled in the transverse linear momentum. In the first part we explain some basics in the form of a technical introduction. We then adapt a general theoretical model to our particular case, explaining the physics of the process of generation of entangled states of photons. We proceed explaining the details of our setup, as well as the procedure of measurement. We then present the results of our tests in a "standard" 2-photon regime to show the correct functioning of the setup itself. Some more sophisticated measurements using structured light in the form of a first-order Hermite-Gaussian mode has been performed to generate entanglement in higher spatial modes are also presented. We conclude with theoretical and experimental details regarding the 4-photon experiments feasible with our setup. Our source is based on Spontaneous Parametric Down-Conversion (SPDC). In the last two decades it has been extensively studied for the generation of two-photon entangled states, since Kwiat et al. published in 1995 the new scheme based on polarization entangled photons. Most of the studies regarding entangled states involving more than two photons are indeed based on quantum correlations in the polarization or in the path of the down converted beams. The great advantage of entangling a spatial degree of freedom (as we do) is related to the dimensionality of the Hilbert space in which the state is defined. In the particular case of linear momentum, which is a continuous variable, we are dealing with infinite dimensions. Since in each dimension of the state one quanta of information can be encoded, the advantage of having multidimension entanglement for the field of quantum communication and computing is clear. The specs of our setup include a periodically-poled KTP crystals offering high conversion efficiency and cut for type-0 SPDC. The photons generated are well known to be inherently entangled in different degrees of freedom such as polarization, energy-time, linear momentum, and orbital angular momentum. Since each single SPDC event generates one photon pair, in order to reach four photon we entangle two consecutive SPDC events per each state. Furthermore, it is possible to manipulate (to enhance) the dimensionality of the entanglement by properly tailoring the pump spatial profile. The key point for the generation of four-photon entangled states is that, under some conditions, two consecutive pairs generated via SPDC cannot be described as two independent pairs but necessarily as a four-photon state showing genuine entanglement. This can happen when using a pulsed laser to generate the entangled photons; in particular, in the regime in which the coherence time of the down-converted photons τc is (much) longer than the temporal length of the pumping pulse Δt. In this condition the emission of a second pair is stimulated by the presence of the first one. That effect can be ultimately seen as a constructive multi-particle interference effect, the deep origin of which has to be sought in the boson statistic of photons.
Twisted photons offer a high-dimensional Hilbert space with the degree of freedom of orbital angular momentum (OAM). Entanglement swapping allows entangling photons that never interact. We report in this paper the hybrid entanglement swapping from multiphoton spin-entangled states to multiphoton OAM entangled states with the aid of NNN-pair hybrid spin-OAM entangled photons. Our scheme provides a feasible method for creating the two-photon OAM Bell states (N=2)(N=2)(N=2) or multiphoton multidimensional OAM Greenberger-Horne-Zeilinger states $(N\ensuremath{\ge}3)$. We highlight the advantage of multiparticle, multidimensional entangled states in some applications of quantum information protocols.
We present a compact scheme for the generation of high-dimensional states of light encoded in the transverse linear momentum of photons that carry orbital angular momentum (OAM). We use a programmable spatial light modulator in phase configuration to create correlations between these two spatial degrees of freedom. With our setup, we are able to control, independently, the relative phases and amplitudes of the spatial superposition in addition to the topological charge of the OAM. Moreover, we engineer correlations that emulate bipartite quantum states of dimensions d × m . Experimental results from the characterization of different generated states of dimensions up to 9 × 5 are in excellent agreement with the numerical simulations. Fidelity with the target state is, for all cases, above 95%.