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Journal of Magnetism and Magnetic Materials

Impulsive optical spin orientation by Zeeman state mixing in ruby

Y. Takagi, Ryuichiro Minamihara, T. Makino

Published Sep 5, 2012• 1 citation
Publisher
DOI
10.1016/j.jmmm.2012.08.047

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The Zeeman effect of R-absorption lines in ruby was observed in a high pulsed magnetic field up to 520 kOe using an optical multichannel analyzer. The experiment was done under a thermal equilibrium condition ( T =130 K) and the Zeeman line intensity is satisfactorily explained. When a magnetic field is applied perpendicular to the C 3 -axis, the excited \barE and 2\barA states show a level mixing and the observed pattern indicates a clear Paschen-Back effect The observed g // -values of the excited states are -2.49±0.05 and 1.49±0.05 for \barE and 2\barA, respectively. g ⊥ -values for these levels were estimated to be smaller than 0.1 at 500 kOe.
Laser-induced fluorescence line narrowing of the ruby R1{R}_{1}R1​ Zeeman spectra at 693.4 nm is reported using a continuous, stable, single-frequency ruby laser for resonant excitation. A resolution in excess of 107{10}^{7}107 corresponding to a linewidth of \ensuremath{\sim} 30 MHz has been achieved. The linewidths are anisotropic with respect to the relative magnetic-field-crystal-axis orientation and, at low Cr concentrations, are expected to be determined by Cr-Al superhyperfine interactions.